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We use inelastic neutron scattering to show that the spin waves in the iron chalcogenide Fe$_{1.05}$Te display novel dispersion clearly different from those in the related iron pnictide systems. By fitting the spin waves to a Heisenberg Hamiltonian, we extract magnetic exchange couplings that are dramatically different from both predictions by density functional calculations and measurements on the iron pnictide CaFe$_2$As$_2$. While the nearest-neighbor exchange couplings in CaFe$_2$As$_2$ and Fe$_{1.05}$Te are quite different, their next-nearest-neighbor exchange couplings are similar. These results suggest that superconductivity in the pnictides and chalcogenides share a common magnetic origin that is intimately associated with the next-nearest-neighbor magnetic coupling between the irons.
54 - T. Tabuchi , Z. Li , G.F. Chen 2010
We report systematic ^{75}As-NQR and ^{139}La-NMR studies on nickel-pnictide superconductors LaNiAsO_{1-x}F_x (x=0, 0.06, 0.10 and 0.12). The spin lattice relaxation rate 1/T_1 decreases below T_c with a well-defined coherence peak and follows an exp onential decay at low temperatures. This result indicates that the superconducting gap is fully opened, and is strikingly different from that observed in iron-pnictide analogs. In the normal state, 1/T_1T is constant in the temperature range T_c sim 4 K < T <10 K for all compounds and up to T=250 K for x=0 and 0.06, which indicates weak electron correlations and is also different from the iron analog. We argue that the differences between the iron and nickel pnictides arise from the different electronic band structure. Our results highlight the importance of the peculiar Fermi-surface topology in iron-pnictides.
We report on band-dependent quasiparticle dynamics in Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ ($T_c = 37 K$) measured using ultrafast pump-probe spectroscopy. In the superconducting state, we observe two distinct relaxation processes: a fast component whose decay rate increases linearly with excitation density and a slow component with an excitation density independent decay rate. We argue that these two components reflect the recombination of quasiparticles in the two hole bands through intraband and interband processes. We also find that the thermal recombination rate of quasiparticles increases quadratically with temperature. The temperature and excitation density dependence of the decays indicates fully gapped hole bands and nodal or very anisotropic electron bands.
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