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The primary aim of experimental nuclear astrophysics is to determine the rates of nuclear reactions taking place in stars in various astrophysical conditions. These reaction rates are important ingredient for understanding the elemental abundance dis tribution in our solar system and the galaxy. The reaction rates are determined from the cross sections which need to be measured at energies as close to the astrophysically relevant ones as possible. In many cases the final nucleus of an astrophysically important reaction is radioactive which allows the cross section to be determined based on the off-line measurement of the number of produced isotopes. In general, this technique is referred to as the activation method, which often has substantial advantages over in-beam particle- or gamma-detection measurements. In this paper the activation method is reviewed from the viewpoint of nuclear astrophysics. Important aspects of the activation method are given through several reaction studies for charged particle, neutron and gamma-induced reactions. Various techniques for the measurement of the produced activity are detailed. As a special case of activation, the technique of Accelerator Mass Spectrometry in cross section measurements is also reviewed.
The cross section of the $^{23}$Na($n, gamma$)$^{24}$Na reaction has been measured via the activation method at the Karlsruhe 3.7 MV Van de Graaff accelerator. NaCl samples were exposed to quasistellar neutron spectra at $kT=5.1$ and 25 keV produced via the $^{18}$O($p, n$)$^{18}$F and $^{7}$Li($p, n$)$^{7}$Be reactions, respectively. The derived capture cross sections $langlesigmarangle_{rm kT=5 keV}=9.1pm0.3$ mb and $langlesigmarangle_{rm kT=25 keV}=2.03 pm 0.05$ mb are significantly lower than reported in literature. These results were used to substantially revise the radiative width of the first $^{23}$Na resonance and to establish an improved set of Maxwellian average cross sections. The implications of the lower capture cross section for current models of $s$-process nucleosynthesis are discussed.
The $^{92}$Mo($alpha,n$)$^{95}$Ru, $^{94}$Mo($alpha,n$)$^{97}$Ru, and $^{112}$Sn($alpha,gamma$)$^{116}$Te cross sections were measured at the upper end of the $p$-process Gamow window between 8.2 MeV and 11.1 MeV. Our results are slightly lower than global Hauser-Feshbach calculations from the code NON-SMOKER, but still within the uncertainty of the prediction. The $^{112}$Sn($alpha,gamma$)$^{116}$Te cross section agrees well with a recently measured thick-target cross section in the same energy range. For the $^{92,94}$Mo($alpha,n$) reactions the present data close to the reaction thresholds could eliminate previous uncertainties within a factor of 20, and we can present now useful comparisons to statistical model calculations with different optical potentials.
The nucleosynthesis of elements beyond iron is dominated by the s and r processes. However, a small amount of stable isotopes on the proton-rich side cannot be made by neutron capture and are thought to be produced by photodisintegration reactions on existing seed nuclei in the so-called p process. So far most of the p-process reactions are not yet accessible by experimental techniques and have to be inferred from statistical Hauser-Feshbach model calculations. The parametrization of these models has to be constrained by measurements on stable proton-rich nuclei. A series of (n,$gamma$) activation measurements on p nuclei, related by detailed balance to the respective photodisintegrations, were carried out at the Karlsruhe Van de Graaff accelerator using the $^7$Li(p,n)$^7$Be source for simulating a Maxwellian neutron distribution of kT= 25 keV. We present here preliminary results of our extended measuring program in the mass range between A=74 and A=132, including first experimental (n,$gamma$) cross sections of $^{74}$Se, $^{84}$Sr, $^{120}$Te and $^{132}$Ba, and an improved value for $^{130}$Ba. In all cases we find perfect agreement with the recommended MACS predictions from the Bao et al. compilation.
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