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Quasiparticle properties in the superconducting state are masked by the superfluid and are not directly accessible to infrared spectroscopy. We show how one can use a Kramers--Kronig transformation to separate the quasiparticle from superfluid respon se and extract intrinsic quasiparticle properties in the superconducting state. We also address the issue of a narrow quasiparticle peak observed in microwave measurements, and demonstrate how it can be combined with infrared measurements to obtain unified picture of electrodynamic properties of cuprate superconductors.
Using infrared spectroscopy, we investigate bottom gated ABA-stacked trilayer graphene subject to an additional environment-induced p-type doping. We find that the Slonczewski-Weiss-McClure tight-binding model and the Kubo formula reproduce the gate voltage-modulated reflectivity spectra very accurately. This allows us to determine the charge densities and the potentials of the {pi}-band electrons on all graphene layers separately and to extract the interlayer permittivity due to higher energy bands.
Far-infrared diagonal and Hall conductivities of multilayer epitaxial graphene on the C-face of SiC were measured using magneto-optical absorption and Faraday rotation in magnetic fields up to 7 T and temperatures between 5 and 300 K. Multiple compon ents are identified in the spectra, which include: (i) a quasi-classical cyclotron resonance (CR), originating from the highly doped graphene layer closest to SiC, (ii) transitions between low-index Landau levels (LLs), which stem from weakly doped layers and (iii) a broad optical absorption background. Electron and hole type LL transitions are optically distinguished and shown to coexist. An electron-hole asymmetry of the Fermi velocity of about 2% was found within one graphene layer, while the Fermi velocity varies by about 10% across the layers. The optical intensity of the LL transitions is several times smaller than what is theoretically expected for isolated graphene monolayers without electron-electron and electron-phonon interactions.
We present a detailed analysis of resonant inelastic scattering (RIXS) from Fe$_{1.087}$Te with unprecedented energy resolution. In contrast to the sharp peaks typically seen in insulating systems at the transition metal $L_3$ edge, we observe spectr a which show different characteristic features. For low energy transfer, we experimentally observe theoretically predicted many-body effects of resonant Raman scattering from a non-interacting gas of fermions. Furthermore, we find that limitations to this many-body electron-only theory are realized at high Raman shift, where an exponential lineshape reveals an energy scale not present in these considerations. This regime, identified as emission, requires considerations of lattice degrees of freedom to understand the lineshape. We argue that both observations are intrinsic general features of many-body physics of metals.
Single crystals of Fe(1+x)Te(1-y)Se(y) have been grown with a controlled Fe excess and Se doping, and the crystal structure has been refined for various compositions. The systematic investigation of magnetic and superconducting properties as a functi on of the structural parameters shows how the material can be driven into various ground states, depending on doping and the structural modifications. Our results prove that the occupation of the additional Fe site, Fe2, enhances the spin localization. By reducing the excess Fe, the antiferromagnetic ordering is weakened, and the superconducting ground state is favored. We have found that both Fe excess and Se doping in synergy determine the properties of the material and an improved 3-dimensional phase diagram is proposed.
We present infrared spectra (0.1-1 eV) of electrostatically gated bilayer graphene as a function of doping and compare it with tight binding calculations. All major spectral features corresponding to the expected interband transitions are identified in the spectra: a strong peak due to transitions between parallel split-off bands and two onset-like features due to transitions between valence and conduction bands. A strong gate voltage dependence of these structures and a significant electron-hole asymmetry is observed that we use to extract several band parameters. Surprisingly, the structures related to the gate-induced bandgap are much less pronounced in the experiment than predicted by the tight binding model.
Classically the interaction between light and matter is given by the Maxwell relations. These are briefly reviewed and will be used as a basis to discuss several techniques that are used in optical spectroscopy. We then discuss the quantum mechanical description of the optical conductivity based on the Kubo formalism. This is used as a basis to understand how strong correlation effects can be observed using optical techniques. We will discuss the use of sum rules in the interpretation of optical experiments. Finally, we describe the effect of including interactions between electronic and collective degrees of freedom on optical spectra.
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