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We present experimental results from a new scheme for magneto-optically trapping strontium monofluoride (SrF) molecules, which provides increased confinement compared to our original work. The improved trap employs a new approach to magneto-optical t rapping presented by M. Tarbutt, emph{arXiv preprint} 1409.0244, which provided insight for the first time into the source of the restoring force in magneto-optical traps (MOTs) where the cycling transition includes dark Zeeman sublevels (known as type-II MOTs). We measure a radial spring constant $20times$ greater than in our original work with SrF, comparable to the spring constants reported in atomic type-II MOTs. We achieve a trap lifetime $tau_{rm{MOT}}=136(2)$~ms, over $2times$ longer than originally reported for SrF. Finally, we demonstrate further cooling of the trapped molecules by briefly increasing the trapping lasers detunings. Our trapping scheme remains a straightforward extension of atomic techniques and marks a step towards the direct production of large, dense, ultracold molecular gases via laser cooling.
Laser cooling and trapping are central to modern atomic physics. The workhorse technique in cold-atom physics is the magneto-optical trap (MOT), which combines laser cooling with a restoring force from radiation pressure. For a variety of atomic spec ies, MOTs can capture and cool large numbers of particles to ultracold temperatures (<1 mK); this has enabled the study of a wide range of phenomena from optical clocks to ultracold collisions whilst also serving as the ubiquitous starting point for further cooling into the regime of quantum degeneracy. Magneto-optical trapping of molecules could provide a similarly powerful starting point for the study and manipulation of ultracold molecular gases. Here, we demonstrate three-dimensional magneto-optical trapping of a diatomic molecule, strontium monofluoride (SrF), at a temperature of approximately 2.5 mK. This method is expected to be viable for a significant number of diatomic species. Such chemical diversity is desired for the wide array of existing and proposed experiments which employ molecules for applications ranging from precision measurement, to quantum simulation and quantum information, to ultracold chemistry.
We report the production of a high phase-space density mixture of $^{87}$Rb and $^{133}$Cs atoms in a levitated crossed optical dipole trap as the first step towards the creation of ultracold RbCs molecules via magneto-association. We present a simpl e and robust experimental setup designed for the sympathetic cooling of $^{133}$Cs via interspecies elastic collisions with $^{87}$Rb. Working with the $|F=1, m_F=+1 >$ and the $|3, +3 >$ states of $^{87}$Rb and $^{133}$Cs respectively, we measure a high interspecies three-body inelastic collision rate $sim 10^{-25}-10^{-26} rm{cm}^{6}rm{s}^{-1}$ which hinders the sympathetic cooling. Nevertheless by careful tailoring of the evaporation we can produce phase-space densities near quantum degeneracy for both species simultaneously. In addition we report the observation of an interspecies Feshbach resonance at 181.7(5) G and demonstrate the creation of Cs$_{2}$ molecules via magneto-association on the 4g(4) resonance at 19.8 G. These results represent important steps towards the creation of ultracold RbCs molecules in our apparatus.
We report an apparatus and method capable of producing Bose-Einstein condensates (BECs) of ~1x10^6 87Rb atoms, and ultimately designed for sympathetic cooling of 133Cs and the creation of ultracold RbCs molecules. The method combines several elements : i) the large recapture of a magnetic quadrupole trap from a magneto-optical trap, ii) efficient forced RF evaporation in such a magnetic trap, iii) the gain in phase-space density obtained when loading the magnetically trapped atoms into a far red-detuned optical dipole trap and iv) efficient evaporation to BEC within the dipole trap. We demonstrate that the system is capable of sympathetically cooling the |F=1,m_F=-1> and |1,0> sublevels with |1,+1> atoms. Finally we discuss the applicability of the method to sympathetic cooling of 133Cs with 87Rb.
We report the formation of a dual-species Bose-Einstein condensate of $^{87}$Rb and $^{133}$Cs in the same trapping potential. Our method exploits the efficient sympathetic cooling of $^{133}$Cs via elastic collisions with $^{87}$Rb, initially in a m agnetic quadrupole trap and subsequently in a levitated optical trap. The two condensates each contain up to $2times10^{4}$ atoms and exhibit a striking phase separation, revealing the mixture to be immiscible due to strong repulsive interspecies interactions. Sacrificing all the $^{87}$Rb during the cooling, we create single species $^{133}$Cs condensates of up to $6times10^{4}$ atoms.
We report modulation transfer spectroscopy on the D2 transitions in 85Rb and 87Rb using a simple home-built electro-optic modulator (EOM). We show that both the gradient and amplitude of modulation transfer spectroscopy signals, for the 87Rb F=2 to F =3 and the 85Rb F=3 to F=4 transitions, can be significantly enhanced by expanding the beams, improving the signals for laser frequency stabilization. The signal gradient for these transitions is increased by a factor of 3 and the peak to peak amplitude was increased by a factor of 2. The modulation transfer signal for the 85Rb F=2 to F transitions is also presented to highlight how this technique can generate a single, clear line for laser frequency stabilization even in cases where there are a number of closely spaced hyperfine transitions.
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