We demonstrate the sensitivity of transverse-field muon spin rotation (TF-muSR) to static charge-density-wave (CDW) order in the bulk of 2H-NbSe2. In the presence of CDW order the quadrupolar interaction of the 93Nb nuclei with the local electric-fie
ld gradient is modified, and this in turn affects the magnetic dipolar coupling of the positive muon to these nuclei. For a weak magnetic field applied parallel to the c-axis, we observe a small enhancement of the muon depolarization rate at temperatures below the established CDW phase transition. Aligning the applied field perpendicular to the c-axis, we observe a sensivity to static CDW order in regions of the sample extending up to nearly 3 times the CDW transition temperature. The results suggest that the muon is mobile over the temperature range explored above the superconducting transition temperature (Tc), and becomes trapped in the vicinity of defects.
We have performed muon spin rotation/relaxation (muSR) measurements on single crystals of the chiral helimagnet Cr1/3NbS2 at zero to low magnetic field. The transition from the paramagnetic to helical magnetically ordered phase at zero field is marke
d by the onset of a coherent oscillation of the zero-field muon spin polarization below a critical temperature Tc. An enhancement of the muon spin precession frequency is observed below T ~ 50K, where anomalous behavior has been observed in bulk transport measurements. The enhanced precession frequency indicates a low-temperature modification of the helical magnetic structure. A Landau free energy analysis suggests that the low-temperature change in the magnetic structure is caused by a structural change, whereas the magnetic order above Tc is the result of an attractive interaction between the ferromagnetic moment induced by the applied field and the magnetic moments of the helical structure. We also suggest a longer periodicity of helicity below T ~ 50K, which can be verified by neutron scattering.
