We investigate the dynamically polarized nuclear-spin system in Fe/emph{n}-GaAs heterostructures using the response of the electron-spin system to nuclear magnetic resonance (NMR) in lateral spin-valve devices. The hyperfine interaction is known to a
ct more strongly on donor-bound electron states than on those in the conduction band. We provide a quantitative model of the temperature dependence of the occupation of donor sites. With this model we calculate the ratios of the hyperfine and quadrupolar nuclear relaxation rates of each isotope. For all temperatures measured, quadrupolar relaxation limits the spatial extent of nuclear spin-polarization to within a Bohr radius of the donor sites and is directly responsible for the isotope dependence of the measured NMR signal amplitude. The hyperfine interaction is also responsible for the $2text{ kHz}$ Knight shift of the nuclear resonance frequency that is measured as a function of the electron spin accumulation. The Knight shift is shown to provide a measurement of the electron spin-polarization that agrees qualitatively with standard spin transport measurements.
A single photon counting system has been developed for efficient detection of forward emitted fluorescence photons at the Experimental Storage Ring (ESR) at GSI. The system employs a movable parabolic mirror with a central slit that can be positioned
around the ion beam and a selected low noise photomultiplier for detection of the collected photons. Compared to the previously used system of mirror segments installed inside the ESR the collection efficiency for forward-emitted photons is improved by more than a factor of 5. No adverse effects on the stored ion beam have been observed during operation besides a small drop in the ion current of about 5% during movement of the mirror into the beam position. The new detection system has been used in the LIBELLE experiment at ESR and enabled for the first time the detection of the ground-state hyperfine M1 transition in lithium-like bismuth (209Bi80+) in a laser-spectroscopy measurement.
