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We study the non-linear interaction of a cold sample of strontium-88 atoms coupled to a single mode of a low finesse optical cavity in the so-called bad cavity limit and investigate the implications for applications to laser stabilization. The atoms are probed on the weak inter-combination line $lvert 5s^{2} , ^1 textrm{S}_0 rangle ,-, lvert 5s5p , ^3 textrm{P}_1 rangle$ at 689 nm in a strongly saturated regime. Our measured observables include the atomic induced phase shift and absorption of the light field transmitted through the cavity represented by the complex cavity transmission coefficient. We demonstrate high signal-to-noise-ratio measurements of both quadratures - the cavity transmitted phase and absorption - by employing FM spectroscopy (NICE-OHMS). We also show that when FM spectroscopy is employed in connection with a cavity locked to the probe light, observables are substantially modified compared to the free space situation where no cavity is present. Furthermore, the non-linear dynamics of the phase dispersion slope is experimentally investigated and the optimal conditions for laser stabilization are established. Our experimental results are compared to state-of-the-art cavity QED theoretical calculations.
We consider the phase stability of a local oscillator (or laser) locked to a cavity QED system comprised of atoms with an ultra-narrow optical transition. The atoms are cooled to millikelvin temperatures and then released into the optical cavity. Alt hough the atomic motion introduces Doppler broadening, the standing wave nature of the cavity causes saturated absorption features to appear, which are much narrower than the Doppler width. These features can be used to achieve an extremely high degree of phase stabilization, competitive with the current state-of-the-art. Furthermore, the inhomogeneity introduced by finite atomic velocities can cause optical bistability to disappear, resulting in no regions of dynamic instability and thus enabling a new regime accessible to experiments where optimum stabilization may be achieved.
As an alternative to state-of-the-art laser frequency stabilisation using ultra-stable cavities, it has been proposed to exploit the non-linear effects from coupling of atoms with a narrow transition to an optical cavity. Here we have constructed suc h a system and observed non-linear phase shifts of a narrow optical line by strong coupling of a sample of strontium-88 atoms to an optical cavity. The sample temperature of a few mK provides a domain where the Doppler energy scale is several orders of magnitude larger than the narrow linewidth of the optical transition. This makes the system sensitive to velocity dependent multi-photon scattering events (Dopplerons) that affect the cavity field transmission and phase. By varying the number of atoms and the intra-cavity power we systematically study this non-linear phase signature which displays roughly the same features as for much lower temperature samples. This demonstration in a relatively simple system opens new possibilities for alternative routes to laser stabilization at the sub 100 mHz level and superradiant laser sources involving narrow line atoms. The understanding of relevant motional effects obtained here has direct implications for other atomic clocks when used in relation with ultranarrow clock transitions.
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