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In a certain regime of low carrier densities and strong correlations, electrons can crystallize into a periodic arrangement of charge known as Wigner crystal. Such phases are particularly interesting in one dimension (1D) as they display a variety of charge and spin ground states which may be harnessed in quantum devices as high-fidelity transmitters of spin information. Recent theoretical studies suggest that the strong Coulomb interactions in Mott insulators and other flat band systems, may provide an attractive higher temperature platform for Wigner crystallization, but due to materials and device constraints experimental realization has proven difficult. In this work we use scanning tunneling microscopy at liquid helium temperatures to directly image the formation of a 1D Wigner crystal in a Mott insulator, TaS$_2$. Charge density wave domain walls in TaS$_2$ create band bending and provide ideal conditions of low densities and strong interactions in 1D. STM spectroscopic maps show that once the lower Hubbard band crosses the Fermi energy, the charges rearrange to minimize Coulomb energy, forming zigzag patterns expected for a 1D Wigner crystal. The zigzag charge patterns show characteristic noise signatures signifying charge or spin fluctuations induced by the tunneling electrons, which is expected for this more fragile condensed state. The observation of a Wigner crystal at orders of magnitude higher temperatures enabled by the large Coulomb energy scales combined with the low density of electrons, makes TaS$_2$ a promising system for exploiting the charge and spin order in 1D Wigner crystals.
Recent experiments [arXiv: 1808.07865] on twisted bilayer graphene (TBLG) show that under hydrostatic pressure, an insulating state at quarter-filling of the moire superlattice (i.e., one charge per supercell) emerges, in sharp contrast with the prev ious ambient pressure measurements of Cao et al. where the quarter--filling state (QFS) is a metal [Nature 556, 43 & 80 (2018)]. In fact, the insulating state at the other commensurate fillings of two and three charges per supercell is also enhanced under applied pressure. Based on realistic computations of the band structure for TBLG which show that the bandwidth first shrinks and then expands with increasing hydrostatic pressure, we compute the ratio of the potential to the kinetic energy, $r_s$. We find an experimentally relevant window of pressure for which $r_s$ crosses the threshold for a triangular Wigner crystal, thereby corroborating our previous work [Nano Lett. (2018)] that the insulating states in TBLG are due to Wigner rather than Mott physics. A key prediction of this work is that the window for the onset of the hierarchy of Wigner states that obtains at commensurate fillings is dome-shaped as a function of the applied pressure, which can be probed experimentally. Theoretically, we find a peak for crystallization around $1.5$ GPa relative to the experimental optimal pressure of $1.33$ GPa for the observation of the insulating states. Consequently, TBLG provides a new platform for the exploration of Wigner physics and its relationship with superconductivity.
59 - Bikash Padhi , Chandan Setty , 2018
We devise a model to explain why twisted bi-layer graphene (TBLG) exhibits insulating behavior when $ u=2,3$ charges occupy a unit moire cell, a feature attributed to Mottness, but not for $ u=1$, clearly inconsistent with Mott insulation. We compute $r_s=E_U/E_K$, where $E_U$ and $E_K$ are the potential and kinetic energies, respectively, and show that (i) the Mott criterion lies at a density $10^4$ higher than in the experiments and (ii) a transition to a series of Wigner crystalline states exists as a function of $ u$. We find, for $ u=1$, $r_s$ fails to cross the threshold ($r_s = 37$) for the triangular lattice and metallic transport ensues. However, for $ u=2$ and $ u=3$, the thresholds, $r_s=22$, and $r_s=17$, respectively are satisfied for a transition to Wigner crystals (WCs) with a honeycomb ($ u=2$) and kagome ($ u=3$) structure. We believe, such crystalline states form the correct starting point for analyzing superconductivity.
We address the question of the mismatch between the zero momentum limits of the transverse and longitudinal dielectric functions for a fixed direction of the driving field observed in the cuprates. This question translates to whether or not the order in which the longitudinal and transverse momentum transfers are taken to zero commute. While the two limits commute for both isotropic and anisotropic Drude metals, we argue that a scaleless vertex interaction that depends solely on the angle between scattered electron momenta is sufficient to achieve non-commutativity of the two limits even for a system that is inherently isotropic. We demonstrate this claim for a simple case of the Drude conductivity modified by electron-boson interactions through appropriate vertex corrections, and outline possible consequences of our result to optical and electron energy loss spectroscopy (EELS) measurements close to zero momentum transfer
346 - Bikash Padhi 2016
In this article we present a pedagogical discussion of some of the optomechanical properties of a high finesse cavity loaded with ultracold atoms in laser induced synthetic gauge fields of different types. Essentially, the subject matter of this arti cle is an amalgam of two sub-fields of atomic molecular and optical (AMO) physics namely, the cavity optomechanics with ultracold atoms and ultracold atoms in synthetic gauge field. After providing a brief introduction to either of these fields we shall show how and what properties of these trapped ultracold atoms can be studied by looking at the cavity (optomechanical or transmission) spectrum. In presence of abelian synthetic gauge field we discuss the cold-atom analogue of Shubnikov de Haas oscillation and its detection through cavity spectrum. Then, in the presence of a non-abelian synthetic gauge field (spin-orbit coupling), we see when the electromagnetic field inside the cavity is quantized, it provides a quantum optical lattice for the atoms, leading to the formation of different quantum magnetic phases. We also discuss how these phases can be explored by studying the cavity transmission spectrum.
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