We predicted and observed for the first time the quasi-specular albedo of cold neutrons at small incidence angles from a powder of nanoparticles. This albedo (reflection) is due to multiple neutron small-angle scattering. The reflection angle as well
as the half-width of angular distribution of reflected neutrons is approximately equal to the incidence angle. The measured reflection probability was equal to ~30% within the detector angular size that corresponds to 40-50% total calculated probability of quasi-specular reflection.
We study possibility of efficient reflection of very cold neutrons (VCN) from powders of nanoparticles. In particular, we measured the scattering of VCN at a powder of diamond nanoparticles as a function of powder sample thickness, neutron velocity a
nd scattering angle. We observed extremely intense scattering of VCN even off thin powder samples. This agrees qualitatively with the model of independent nanoparticles at rest. We show that this intense scattering would allow us to use nanoparticle powders very efficiently as the very first reflectors for neutrons with energies within a complete VCN range up to $10^{-4}$ eV.
