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$^{121,123}Sb$ nuclear quadrupole resonance (NQR) was applied to $Fe(Sb_{1-x}Te_x)_2$ in the low doping regime (emph{x = 0, 0.01} and emph{0.05}) as a microscopic zero field probe to study the evolution of emph{3d} magnetism and the emergence of meta llic behavior. Whereas the NQR spectra itself reflects the degree of local disorder via the width of the individual NQR lines, the spin lattice relaxation rate (SLRR) $1/T_1(T)$ probes the fluctuations at the $Sb$ - site. The fluctuations originate either from conduction electrons or from magnetic moments. In contrast to the semi metal $FeSb_2$ with a clear signature of the charge and spin gap formation in $1/T_1(T)T ( sim exp/ (Delta k_BT) ) $, the 1% $Te$ doped system exhibits almost metallic conductivity and a almost filled gap. A weak divergence of the SLRR coefficient $1/T_1(T)T sim T^{-n} sim T^{-0.2}$ points towards the presence of electronic correlations towards low temperatures wheras the textit{5%} $Te$ doped sample exhibits a much larger divergence in the SLRR coefficient showing $1/T_1(T)T sim T^{-0.72} $. According to the specific heat divergence a power law with $n = 2 m = 0.56$ is expected for the SLRR. Furthermore $Te$-doped $FeSb_2$ as a disordered paramagnetic metal might be a platform for the electronic Griffith phase scenario. NQR evidences a substantial asymmetric broadening of the $^{121,123}Sb$ NQR spectrum for the emph{5%} sample. This has purely electronic origin in agreement with the electronic Griffith phase and stems probably from an enhanced $Sb$-$Te$ bond polarization and electronic density shift towards the $Te$ atom inside $Sb$-$Te$ dumbbell.
64 - A.A. Gippius , A.S. Moskvin , 2010
The incommensurate (IC) spin ordering in quasi-1D edge-shared cuprate NaCu_2O_2 has been studied by ^{23}Na nuclear magnetic resonance spectroscopy in an external magnetic field near 6 Tesla applied along the main crystallographic axes. The NMR lines hape evolution above and below T_Napprox12 K yields a clear signature of an IC static modulation of the local magnetic field consistent with a Cu^{2+} spin spiral polarized in the bc-plane rather than in the ab-plane as reported from earlier neutron diffraction data.
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