The extreme back-angle evaporation spectra of alpha, lithium, beryllium, boron and carbon from different compound nuclei near A=100 (EX=76-210 MeV) have been compared with the predictions of standard statistical model codes such as CASCADE and GEMINI
. It was found that the shapes of the alpha spectra agree well with the predictions of the statistical models. However the spectra of lithium, beryllium, boron and carbon show significantly gentler slopes implying higher temperature of the residual nuclei, even though the spectra satisfy all other empirical criteria of statistical emissions. The observed slope anomaly was found to be largest for lithium and decreases at higher excitation energy. These results could not be understood by adjusting the parameters of the statistical models or from reaction dynamics and might require examining the statistical model from a quantum mechanical perspective.
The eigenstate energies of an atom increase under spatial confinement and this effect should also increase the electron density of the orbital electrons at the nucleus thus increasing the decay rate of an electron-capturing radioactive nucleus. We ha
ve observed that the orbital electron capture rates of 109In and 110Sn increased by (1.00+-0.17)% and (0.48+-0.25)% respectively when implanted in the small Au lattice versus large Pb lattice. These results have been understood because of the higher compression experienced by the large radioactive atoms due to the spatial confinement in the smaller Au lattice.
