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We have characterized spin-squeezed states produced at a temperature of $26^circ{mathrm C}$ on a Nuclear Magnetic Resonance (NMR) quadrupolar system. The implementation is carried out in an ensemble of $^{133}$Cs nuclei with spin $I=7/2$ of a lyotrop ic liquid crystal sample. We identify the source of spin squeezing due to the interaction between the quadrupole moment of the nuclei and the electric field gradients internally present in the molecules. We use the spin angular momentum representation to describe formally the nonlinear operators that produce the spin squeezing. The quantitative and qualitatively characterization of the spin squeezing phenomena is performed through a squeezing parameter and squeezing angle developed for the two-mode BEC system, and, as well, by the Wigner quasi-probability distribution function. The generality of the present experimental scheme indicates its potential applications on solid state physics.
The Josephson Junction model is applied to the experimental implementation of classical bifurcation in a quadrupolar Nuclear Magnetic Resonance system. There are two regimes, one linear and one nonlinear which are implemented by the radio-frequency t erm and the quadrupolar term of the Hamiltonian of a spin system respectively. Those terms provide an explanation of the symmetry breaking due to bifurcation. Bifurcation depends on the coexistence of both regimes at the same time in different proportions. The experiment is performed on a lyotropic liquid crystal sample of an ordered ensemble of $^{133}$Cs nuclei with spin $I=7/2$ at room temperature. Our experimental results confirm that bifurcation happens independently of the spin value and of the physical system. With this experimental spin scenario, we confirm that a quadrupolar nuclei system could be described analogously to a symmetric two--mode Bose--Einstein condensate.
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