We study the characteristics of the light generated by few emitters in a cavity at strong light-matter coupling. By means of the Glauber $g^{(2)}$-function we can identify clearly distinguished parameter regimes with super-Poissonian and sub-Poissoni
an photon statistics. We establish a relation between the emission characteristics for one and multiple emitters, and explain its origin in terms of the photon-dressed emitter states. Cooperative effects lead to the generation of nonclassical light already at reduced light-matter coupling if the number of emitters is increased. Our results are obtained with a full input-output formalism and master equation valid also at strong light-matter coupling. We compare the behavior obtained with and without counter-rotating light-matter interaction terms in the Hamiltonian, and find that the generation of nonclassical light is robust against such modifications. Finally, we contrast our findings with the predictions of the quantum optical master equation and find that it fails entirely at predicting regimes with different photon statistics.
We formulate exact generalized nonequilibrium fluctuation relations for the quantum mechanical harmonic oscillator coupled to multiple harmonic baths. Each of the different baths is prepared in its own individual (in general nonthermal) state. Starti
ng from the exact solution for the oscillator dynamics we study fluctuations of the oscillator position as well as of the energy current through the oscillator under general nonequilibrium conditions. In particular, we formulate a fluctuation-dissipation relation for the oscillator position autocorrelation function that generalizes the standard result for the case of a single bath at thermal equilibrium. Moreover, we show that the generating function for the position operator fullfills a generalized Gallavotti-Cohen-like relation. For the energy transfer through the oscillator, we determine the average energy current together with the current fluctuations. Finally, we discuss the generalization of the cumulant generating function for the energy transfer to nonthermal bath preparations.
We study the dissipative quantum harmonic oscillator with general non-thermal preparations of the harmonic oscillator bath. The focus is on equilibration of the oscillator in the long-time limit and the additional requirements for thermalization. Our
study is based on the exact solution of the microscopic model obtained by means of operator equations of motion, which provides us with the time evolution of the central oscillator density matrix in terms of the propagating function. We find a hierarchy of conditions for thermalization, together with the relation of the asymptotic temperature to the energy distribution in the initial bath state. We discuss the presence and absence of equilibration for the example of an inhomogeneous chain of harmonic oscillators, and illustrate the general findings about thermalization for the non-thermal environment that results from a quench.
Atoms, molecules or excitonic quasiparticles, for which excitations are induced by external radiation fields and energy is dissipated through radiative decay, are examples of driven open quantum systems. We explain the use of commutator-free exponent
ial time-propagators for the numerical solution of the associated Schrodinger or master equations with a time-dependent Hamilton operator. These time-propagators are based on the Magnus series but avoid the computation of commutators, which makes them suitable for the efficient propagation of systems with a large number of degrees of freedom. We present an optimized fourth order propagator and demonstrate its efficiency in comparison to the direct Runge-Kutta computation. As an illustrative example we consider the parametrically driven dissipative Dicke model, for which we calculate the periodic steady state and the optical emission spectrum.
We study the quantum phase transition of the Dicke model in the classical oscillator limit, where it occurs already for finite spin length. In contrast to the classical spin limit, for which spin-oscillator entanglement diverges at the transition, en
tanglement in the classical oscillator limit remains small. We derive the quantum phase transition with identical critical behavior in the two classical limits and explain the differences with respect to quantum fluctuations around the mean-field ground state through an effective model for the oscillator degrees of freedom. With numerical data for the full quantum model we study convergence to the classical limits. We contrast the classical oscillator limit with the dual limit of a high frequency oscillator, where the spin degrees of freedom are described by the Lipkin-Meshkov-Glick model. An alternative limit can be defined for the Rabi case of spin length one-half, in which spin frequency renormalization replaces the quantum phase transition.
We consider a quantum dot, affected by a local vibrational mode and contacted to macroscopic leads, in the non-equilibrium steady-state regime. We apply a variational Lang-Firsov transformation and solve the equations of motion of the Green functions
in the Kadanoff-Baym formalism up to second order in the interaction coefficients. The variational determination of the transformation parameter through minimization of the thermodynamic potential allows us to calculate the electron/polaron spectral function and conductance for adiabatic to anti-adiabatic phonon frequencies and weak to strong electron-phonon couplings. We investigate the qualitative impact of the quasi-particle renormalization on the inelastic electron tunneling spectroscopy signatures and discuss the possibility of a polaron induced negative differential conductance. In the high-voltage regime we find that the polaron level follows the lead chemical potential to enhance resonant transport.
To describe the interaction of molecular vibrations with electrons at a quantum dot contacted to metallic leads, we extend an analytical approach that we previously developed for the many-polaron problem. Our scheme is based on an incomplete variatio
nal Lang-Firsov transformation, combined with a perturbative calculation of the electron-phonon self-energy in the framework of generalised Matsubara functions. This allows us to describe the system at weak to strong coupling and intermediate to large phonon frequencies. We present results for the quantum dot spectral function and for the kinetic coefficient that characterises the electron transport through the dot. With these results we critically examine the strengths and limitations of our approach, and discuss the properties of the molecular quantum dot in the context of polaron physics. We place particular emphasis on the importance of corrections to the concept of an antiadiabatic dot polaron suggested by the complete Lang-Firsov transformation.
We investigate charge transport within some background medium by means of an effective lattice model with a novel form of fermion-boson coupling. The bosons describe fluctuations of a correlated background. By analyzing groundstate and spectral prope
rties of this transport model, we show how a metal-insulator quantum phase transition can occur for the half-filled band case. We discuss the evolution of a mass-asymmetric band structure in the insulating phase and establish connections to the Mott and Peierls transition scenarios.
