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Observation of coherent backscattering of light by cold atoms

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 Added by Cord Axel Mueller
 Publication date 2000
  fields Physics
and research's language is English
 Authors G. Labeyrie




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Coherent backscattering (CBS) of light waves by a random medium is a signature of interference effects in multiple scattering. This effect has been studied in many systems ranging from white paint to biological tissues. Recently, we have observed CBS from a sample of laser-cooled atoms, a scattering medium with interesting new properties. In this paper we discuss various effects, which have to be taken into account for a quantitative study of coherent backscattering of light by cold atoms.



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75 - G. Labeyrie 1999
Light propagating in an optically thick sample experiences multiple scattering. It is now known that interferences alter this propagation, leading to an enhanced backscattering, a manifestation of weak localization of light in such diffuse samples. This phenomenon has been extensively studied with classical scatterers. In this letter we report the first experimental evidence for coherent backscattering of light in a laser-cooled gas of Rubidium atoms.
We present a generalization of the diagrammatic pump-probe approach to coherent backscattering (CBS) of intense laser light for atoms with degenerate energy levels. We employ this approach for a characterization of the double scattering signal from optically pumped atoms with the transition $J_grightarrow J_e=J_g+1$ in the helicity preserving polarization channel. We show that, in the saturation regime, the internal degeneracy becomes manifest for atoms with $J_ggeq 1$, leading to a faster decrease of the CBS enhancement factor with increasing saturation parameter than in the non-degenerate case.
We explore the potential of a static electric field to induce Anderson localization of light in a large three-dimensional (3D) cloud of randomly distributed, immobile atoms with a degenerate ground state (total angular momentum $J_g = 0$) and a three-fold degenerate excited state ($J_e = 1$). We study both the spatial structure of quasimodes of the atomic cloud and the scaling of the Thouless number with the size of the cloud. Our results indicate that unlike the static magnetic field, the electric field does not induce Anderson localization of light by atoms. We explain this conclusion by the incomplete removal of degeneracy of the excited atomic state by the field and the relatively strong residual dipole-dipole coupling between atoms which is weaker than in the absence of external fields but stronger than in the presence of a static magnetic field. A joint analysis of these results together with our previous results concerning Anderson localization of scalar waves and light suggests the existence of a critical strength of dipole-dipole interactions that should not be surpassed for Anderson localization to be possible in 3D.
We demonstrate that the transport of coherent quasiresonant light through a dense cloud of immobile two-level atoms subjected to a static external electric field can be described by a simple diffusion process up to atomic number densities of the order of at least $10^2$ atoms per wavelength cubed. Transport mean free paths well below the wavelength of light in the free space can be reached without inducing any sign of Anderson localization of light or of any other mechanism of breakdown of diffusion.
We present the first calculation of coherent backscattering with inelastic scattering by saturated atoms. We consider the scattering of a quasi-monochromatic laser pulse by two distant atoms in free space. By restricting ourselves to scattering of two photons, we employ a perturbative approach, valid up to second order in the incident laser intensity. The backscattering enhancement factor is found to be smaller than two (after excluding single scattering), indicating a loss of coherence between the doubly scattered light emitted by both atoms. Since the undetected photon carries information about the path of the detected photon, the coherence loss can be explained by a which-path argument, in analogy with a double-slit experiment.
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