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Register a new userCharge order at high temperature in cuprate superconductors
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The presence of different electronic orders other than superconductivity populating the phase diagram of cuprates suggests that they might be the key to disclose the mysteries of this class of materials. In particular charge order in the form of charge density waves (CDW), i.e., the incommensurate modulation of electron density in the CuO$_2$ planes, is ubiquitous across different families and presents a clear interplay with superconductivity. Until recently, CDW had been found to be confined inside a rather small region of the phase diagram, below the pseudogap temperature and the optimal doping. This occurrence might shed doubts on the possibility that such low temperature phenomenon actually rules the properties of cuprates either in the normal or in the superconducting states. However, recent resonant X-ray scattering (RXS) experiments are overturning this paradigm. It results that very short-ranged charge modulations permeate a much wider region of the phase diagram, coexisting with CDW at lower temperatures and persisting up to temperatures well above the pseudogap opening. Here we review the characteristics of these high temperature charge modulations, which are present in several cuprate families, with similarities and differences. A particular emphasis is put on their dynamical character and on their coupling to lattice and magnetic excitations, properties that can be determined with high resolution resonant inelastic x-ray scattering (RIXS).
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A model of charged hole-pair bosons, with long range Coulomb interactions and very weak interlayer coupling, is used to calculate the order parameter -Phi- of underdoped cuprates. Model parameters are extracted from experimental superfluid densities and plasma frequencies. The temperature dependence -Phi(T)- is characterized by a trapezoidal shape. At low temperatures, it declines slowly due to harmonic phase fluctuations which are suppressed by anisotropic plasma gaps. Above the single layer Berezinski-Kosterlitz-Thouless (BKT) temperature, Phi(T) falls rapidly toward the three dimensional transition temperature. The theoretical curves are compared to c-axis superfluid density data by H. Kitano et al., (J. Low Temp. Phys. 117, 1241 (1999)) and to the -transverse nodal velocity- measured by angular resolved photoemmission spectra on BSCCO samples by W.S. Lee et al., (Nature 450, 81 (2007)), and by A. Kanigel, et al., (Phys. Rev. Lett. 99, 157001 (2007)).
We show that the asymmetric tunneling spectrum observed in the cuprate superconductors stems from the existence of a competing order. The competition between the competing order and superconductivity can create a charge depletion region near the surface. The asymmetric response of the depletion region as the function of the external voltage causes the asymmetric tunneling spectrum. The effect is very general in a system which is near the phase boundary of two competing states favoring different carrier densities. The asymmetry which has recently been observed in the point-contact spectroscopy of the heavy fermion superconductor CeCoIn5 is another example of this effect.
In a multiorbital model of the cuprate high-temperature superconductors soft antiferromagnetic (AF) modes are assumed to reconstruct the Fermi surface to form nodal pockets. The subsequent charge ordering transition leads to a phase with a spatially modulated transfer of charge between neighboring oxygen p_x and p_y orbitals and also weak modulations of the charge density on the copper d_{x^2-y^2} orbitals. As a prime result of the AF Fermi surface reconstruction, the wavevectors of the charge modulations are oriented along the crystalline axes with a periodicity that agrees quantitatively with experiments. This resolves a discrepancy between experiments, which find axial order, and previous theoretical calculations, which find modulation wavevectors along the Brillouin zone (BZ) diagonal. The axial order is stabilized by hopping processes via the Cu4s orbital, which is commonly not included in model analyses of cuprate superconductors.
The spectral energy gap is an important signature that defines states of quantum matter: insulators, density waves, and superconductors have very different gap structures. The momentum resolved nature of angle-resolved photoemission spectroscopy (ARPES) makes it a powerful tool to characterize spectral gaps. ARPES has been instrumental in establishing the anisotropic d-wave structure of the superconducting gap in high-transition temperature (Tc) cuprates, which is different from the conventional isotropic s-wave superconducting gap. Shortly afterwards, ARPES demonstrated that an anomalous gap above Tc, often termed the pseudogap, follows a similar anisotropy. The nature of this poorly understood pseudogap and its relationship with superconductivity has since become the focal point of research in the field. To address this issue, the momentum, temperature, doping, and materials dependence of spectral gaps have been extensively examined with significantly improved instrumentation and carefully matched experiments in recent years. This article overviews the current understanding and unresolved issues of the basic phenomenology of gap hierarchy. We show how ARPES has been sensitive to phase transitions, has distinguished between orders having distinct broken electronic symmetries, and has uncovered rich momentum and temperature dependent fingerprints reflecting an intertwined & competing relationship between the ordered states and superconductivity that results in multiple phenomenologically-distinct ground states inside the superconducting dome. These results provide us with microscopic insights into the cuprate phase diagram.
The symmetry operations of the crystal groups relevant for the high temperature superconductors HgBa2CuO4+x (Hg1201), YBa2Cu3O7-x (YBCO), and Bi2Sr2CaCu2O8+x (BSCCO) are elucidated. The allowable combinations of the superconducting order parameter (OP) components are presented for both the angular momentum and lattice representations. For tetragonal Hg1201, the spin singlet OP components are composed from four sets of compatible basis functions, which combine to give the generalized s-, dx2-y2-, dxy-, and gxy(x2-y2)- wave OPs. In YBCO, elements of s- and dx2-y2- wave sets are compatible, but in BSCCO, elements of s- and dxy- wave sets are compatible. The Josephson critical current density JcJ across c-axis twist junctions in the vicinity of Tc is then evaluated as a function of the twist angle phi0, for each allowable OP combination, for both coherent and incoherent tunneling. Recent experiments of Li et al. demonstrated the independence of JcJ(phi0)/JcS upon phi0 at and below Tc, where JcS is the critical current density of a constituent single crystal. These experiments are shown to be consistent with an OP containing an s-wave component, but inconsistent with an OP containing the purported dx2-y2-wave component. In addition, they demonstrate that the interlayer tunneling across untwisted layers in single crystal BSCCO is entirely incoherent. We propose a new type of tricrystal experiment using single crystal c-axis twist junctions, that does not employ substrate grain boundaries.
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