No Arabic abstract
We report high-precision small angle neutron scattering of the orientation of the skyrmion lattice in a spherical sample of MnSi under systematic changes of the magnetic field direction. For all field directions the skyrmion lattice may be accurately described as a triple-$vec{Q}$ state, where the modulus $vert vec{Q} vert$ is constant and the wave vectors enclose rigid angles of $120^{circ}$. Along a great circle across $langle 100rangle$, $langle 110rangle$, and $langle 111rangle$ the normal to the skyrmion-lattice plane varies systematically by $pm3^{circ}$ with respect to the field direction, while the in-plane alignment displays a reorientation by $15^{circ}$ for magnetic field along $langle 100rangle$. Our observations are qualitatively and quantitatively in excellent agreement with an effective potential, that is determined by the symmetries of the tetrahedral point group $T$ and includes contributions up to sixth-order in spin-orbit coupling, providing a full account of the effect of cubic magnetocrystalline anisotropies on the skyrmion lattice in MnSi.
We investigate the anisotropic nature of magnetocrystalline coupling between the crystallographic and skyrmion crystal (SKX) lattices in the chiral magnet MnSi by magnetic field-angle resolved resonant ultrasound spectroscopy. Abrupt changes are observed in the elastic moduli and attenuation when the magnetic field is parallel to the [011] crystallographic direction. These observations are interpreted in a phenomenological Ginzburg-Landau theory that identifies switching of the SKX orientation to be the result of an anisotropic magnetocrystalline coupling potential. Our paper sheds new light on the nature of magnetocrystalline coupling potential relevant to future spintronic applications.
Using small-angle neutron scattering (SANS), we investigate the deformation of the magnetic skyrmion lattice in bulk single-crystalline MnSi under electric current flow. A significant broadening of the skyrmion-lattice-reflection peaks was observed in the SANS pattern for current densities greater than a threshold value j_t ~ 1 MA/m^2 (10^6 A/m^2). We show this peak broadening to originate from a spatially inhomogeneous rotation of the skyrmion lattice, with an inverse rotation sense observed for opposite sample edges aligned with the direction of current flow. The peak broadening (and the corresponding skyrmion lattice rotations) remain finite even after switching off the electric current. These results indicate that skyrmion lattices under current flow experience significant friction near the sample edges, and plastic deformation due to pinning effects, these being important factors that must be considered for the anticipated skyrmion-based applications in chiral magnets at the nanoscale.
We report an experimental study of the emergence of non-trivial topological winding and long-range order across the paramagnetic to skyrmion lattice transition in the transition metal helimagnet MnSi. Combining measurements of the susceptibility with small angle neutron scattering, neutron resonance spin echo spectroscopy and all-electrical microwave spectroscopy, we find evidence of skyrmion textures in the paramagnetic state exceeding $10^3$AA with lifetimes above several 10$^{-9}$s. Our experimental findings establish that the paramagnetic to skyrmion lattice transition in MnSi is well-described by the Landau soft-mode mechanism of weak crystallization, originally proposed in the context of the liquid to crystal transition. As a key aspect of this theoretical model, the modulation-vectors of periodic small amplitude components of the magnetization form triangles that add to zero. In excellent agreement with our experimental findings, these triangles of the modulation-vectors entail the presence of the non-trivial topological winding of skyrmions already in the paramagnetic state of MnSi when approaching the skyrmion lattice transition.
The magnetic inhomogeneity of the A-phase in MnSi chiral magnet is identified for the first time from the precise measurements of transverse magnetoresistance (MR) anisotropy. The area inside the A-phase (A-phase core) corresponds to isotropic MR having no confinement to the MnSi crystal lattice. Per contra, the MR becomes anisotropic both on the border of the A-phase and in other magnetic phases, the strongest magnetic scattering being observed when external magnetic field applied along [001] or [00-1] directions. We argue here that the established MR features prove the presence of two different types of the skyrmion lattices inside the A-phase, and the dense skyrmion state of the A-phase core is built from individual skyrmions similar to Abrikosov-type magnetic vortexes.
We report the direct measurement of the topological skyrmion energy barrier through a hysteresis of the skyrmion lattice in the chiral magnet MnSi. Measurements were made using small-angle neutron scattering with a custom-built resistive coil to allow for high-precision minor hysteresis loops. The experimental data was analyzed using an adapted Preisach model to quantify the energy barrier for skyrmion formation and corroborated by the minimum-energy path analysis based on atomistic spin simulations. We reveal that the skyrmion lattice in MnSi forms from the conical phase progressively in small domains, each of which consisting of hundreds of skyrmions, and with an activation barrier of several eV.