Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userInfluence of host matrices on krypton electron binding energies and KLL Auger transition energies
449
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
The low-energy electron spectra emitted in the radioactive decay of the $^{83}$Rb and $^{83}$Sr isotopes were measured with a combined electrostatic electron spectrometer. Radioactive sources used were prepared by ion implantation of $^{83}$Sr into a high purity polycrystalline platinum foil at 30 keV and by vacuum-evaporation deposition of $^{83}$ Rb on the same type of foil. From the measured conversion electron spectra, the electron binding energies (referenced to the Fermi level) for the K, L$_1$ , L$_2$ , L$_3$ , M$_1$ , M$_2$, and M$_3$ shell/subshells of krypton in the platinum host were determined to be 14 316.4(12), 1 914.3(9), 1 720.3(9), 1 667.6(9), 281.5(9), 209.6(13), and 201.2(15) eV, respectively, and those for the evaporated layer were observed to be lower by 0.7(1) eV. For both host matrices, values of 2.3(2), 4.6(2), 1.7(2), 1.3(2), and 3.2(3) eV were obtained for the krypton K, L$_1$ , L$_2$ , L$_3$ , and M$_1$ natural atomic level widths, respectively. The absolute energies of 10 838.5(9) and 10 839.5(10) eV were measured for the KL$_2$L$_3$ ($^{1}$D$_2$) Auger transition in krypton implanted in Pt and generated in the evaporated rubidium layer, respectively. A value of 601.0(8) eV was measured for the energy difference of the KL$_2$L$_3$ ($^{1}$D$_2$) transitions in Rb and Kr in the Pt host. Multiconfiguration Dirac-Fock calculations of the krypton KLL transition energies and intensities were also performed.
rate research
Read More
Nuclear mass contains a wealth of nuclear structure information, and has been widely employed to extract the nuclear effective interactions. The known nuclear mass is usually extracted from the experimental atomic mass by subtracting the masses of electrons and adding the binding energy of electrons in the atom. However, the binding energies of electrons are sometimes neglected in extracting the known nuclear masses. The influence of binding energies of electrons on nuclear mass predictions are carefully investigated in this work. If the binding energies of electrons are directly subtracted from the theoretical mass predictions, the rms deviations of nuclear mass predictions with respect to the known data are increased by about $200$ keV for nuclei with $Z, Ngeqslant 8$. Furthermore, by using the Coulomb energies between protons to absorb the binding energies of electrons, their influence on the rms deviations is significantly reduced to only about $10$ keV for nuclei with $Z, Ngeqslant 8$. However, the binding energies of electrons are still important for the heavy nuclei, about $150$ keV for nuclei around $Z=100$ and up to about $500$ keV for nuclei around $Z=120$. Therefore, it is necessary to consider the binding energies of electrons to reliably predict the masses of heavy nuclei at an accuracy of hundreds of keV.
Nuclear deformation effects on the binding energies in heavy ions are investigated. Approximate formulas for the nuclear-size correction and the isotope shift for deformed nuclei are derived. Combined with direct numerical evaluations, these formulas are employed to reanalyse experimental data on the nuclear-charge-distribution parameters in $^{238}textrm{U}$ and to revise the nuclear-size corrections to the binding energies in H- and Li-like $^{238}textrm{U}$. As a result, the theoretical uncertainties for the ground-state Lamb shift in $^{238}textrm{U}^{91+}$ and for the $2p_{1/2}-2s$ transition energy in $^{238}textrm{U}^{89+}$ are significantly reduced. The isotope shift of the $2p_{j}-2s$ transition energies for $^{142}textrm{Nd}^{57+}$ and $^{150}textrm{Nd}^{57+}$ is also evaluated including nuclear size and nuclear recoil effects within a full QED treatment.
The most precise to-date evaluation of the nuclear recoil effect on the $n=1$ and $n=2$ energy levels of He-like ions is presented in the range $Z=12-100$. The one-electron recoil contribution is calculated within the framework of the rigorous QED approach to first order in the electron-to-nucleus mass ratio $m/M$ and to all orders in the parameter $alpha Z$. The two-electron $m/M$ recoil term is calculated employing the $1/Z$ perturbation theory. The recoil contribution of the zeroth order in $1/Z$ is evaluated to all orders in $alpha Z$, while the $1/Z$ term is calculated using the Breit approximation. The recoil corrections of the second and higher orders in $1/Z$ are taken into account within the nonrelativistic approach. The obtained results are compared with the previous evaluation of this effect [A. N. Artemyev et al., Phys. Rev. A 71, 062104 (2005)].
Energies of two-electron one-photon transitions from initial double K-hole states were computed using the Dirac-Fock model. The transition energies of competing processes, the K$alpha$ hypersatellites, were also computed. The results are compared to experiment and to other theoretical calculations.
The KLL Auger spectrum of rubidium following the electron capture decay of $^{83}$Sr and $^{85}$Sr isotopes was experimentally studied in detail for the first time using one $^{83}$Sr source and three $^{85}$Sr sources in different host matrices. Energies, relative intensities, and natural widths of all the nine well-resolved basic spectrum components were determined and compared with both predictions and experimental data for krypton. Results of our multiconfiguration Dirac-Fock calculations demonstrated an influence of the atomic structure effect on absolute energies of the KLL transitions following the creation of initial vacancies by the electron capture decay. Environmental effects on the KLL Auger spectrum were distinctly observed only for the absolute transition energies.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
