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Register a new userStructural second-order nonlinearity in metamaterials
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Added by
Viktor A. Podolskiy
Publication date
2017
fields
Physics
and research's language is
English
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Nonlinear processes are at the core of many optical technologies including lasers, information processing, sensing, and security, and require optimised materials suitable for nanoscale integration. Here we demonstrate the emergence of a strong bulk second-order nonlinear response in a composite plasmonic nanorod material comprised of centrosymmetric materials. The metamaterial provides equally strong generation of the p-polarized second harmonic light in response to both s- and p-polarized excitation. We develop an effective-medium description of the underlying physics, compare its predictions to the experimental results and analyze the limits of its applicability. We show that while the effective medium theory adequately describes the nonlinear polarization, the process of emission of second harmonic light cannot be described in the same framework. The work provides an understanding of the emergent nonlinear optical response in composites and opens a doorway to new nonlinear optical platform designs for integrated nonlinear photonics.
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We report the observation of second-harmonic generation in stoichiometric silicon nitride waveguides grown via low-pressure chemical vapour deposition. Quasi-rectangular waveguides with a large cross section were used, with a height of 1 {mu}m and various different widths, from 0.6 to 1.2 {mu}m, and with various lengths from 22 to 74 mm. Using a mode-locked laser delivering 6-ps pulses at 1064 nm wavelength with a repetition rate of 20 MHz, 15% of the incoming power was coupled through the waveguide, making maximum average powers of up to 15 mW available in the waveguide. Second-harmonic output was observed with a delay of minutes to several hours after the initial turn-on of pump radiation, showing a fast growth rate between 10$^{-4}$ to 10$^{-2}$ s$^{-1}$, with the shortest delay and highest growth rate at the highest input power. After this first, initial build-up, the second-harmonic became generated instantly with each new turn-on of the pump laser power. Phase matching was found to be present independent of the used waveguide width, although the latter changes the fundamental and second-harmonic phase velocities. We address the presence of a second-order nonlinearity and phase matching, involving an initial, power-dependent build-up, to the coherent photogalvanic effect. The effect, via the third-order nonlinearity and multiphoton absorption leads to a spatially patterned charge separation, which generates a spatially periodic, semi-permanent, DC-field-induced second-order susceptibility with a period that is appropriate for quasi-phase matching. The maximum measured second-harmonic conversion efficiency amounts to 0.4% in a waveguide with 0.9 x 1 {mu}m$^2$ cross section and 36 mm length, corresponding to 53 {mu}W at 532 nm with 13 mW of IR input coupled into the waveguide. The according $chi^{(2)}$ amounts to 3.7 pm/V, as retrieved from the measured conversion efficiency.
Recent studies on fully dielectric multilayered metamaterials have shown that the negligibly small nonlocal effects (spatial dispersion) typically observed in the limit of deeply subwavelength layers may be significantly enhanced by peculiar boundary effects occurring in certain critical parameter regimes. These phenomena, observed so far in periodic and randomly disordered geometries, are manifested as strong differences between the exact optical response of finite-size metamaterial samples and the prediction from conventional effective-theory-medium models based on mixing formulae. Here, with specific focus on the Thue-Morse geometry, we make a first step toward extending the studies above to the middle-ground of aperiodically ordered multilayers, lying in between perfect periodicity and disorder. We show that, also for these geometries, there exist critical parameter ranges that favor the buildup of boundary effects leading to strong enhancement of the (otherwise negligibly weak) nonlocality. However, the underlying mechanisms are fundamentally different from those observed in the periodic case, and exhibit typical footprints (e.g., fractal gaps, quasi-localized states) that are distinctive of aperiodic order. The outcomes of our study indicate that aperiodic order plays a key role in the buildup of the aforementioned boundary effects, and may also find potential applications to optical sensors, absorbers and lasers.
Optical nonlinearity plays a pivotal role in quantum information processing using photons, from heralded single-photon sources to long-sought quantum repeaters. Despite the availability of strong light-atom interaction, an all-optical nonlinearity is highly desired for more scalable quantum protocols. Here, we realize quantum nanophotonic integrated circuits in thin-film InGaP with a record-high second-order optical nonlinearity of $1.5%$---the ratio of the single-photon trimodal coupling strength ($g/2pi=11.2$ MHz) and cavity-photon loss rate. We demonstrate photon-pair generation via degenerate spontaneous parametric down conversion in the InGaP photonic circuit with an ultrahigh rate exceeding 27.5 MHz per 1 $mu$W pump power and large coincidence-to-accidental ratio up to $1.4times 10^4$. Our work shows InGaP as a potentially transcending platform for quantum nonlinear optics and quantum information applications.
We investigate optically reconfigurable dielectric metamaterials at gigahertz frequencies. More precisely, we study the microwave response of a subwavelength grating optically imprinted into a semiconductor slab. In the homogenized regime, we analytically evaluate the ordinary and extraordinary component of the effective permittivity tensor by taking into account the photo-carrier dynamics described by the ambipolar diffusion equation. We analyze the impact of semiconductor parameters on the gigahertz metamaterial response which turns out to be highly reconfigurable by varying the photogenerated grating and which can show a marked anisotropic behavior.
Nonlocal (spatial-dispersion) effects in multilayered metamaterials composed of periodic stacks of alternating, deeply subwavelength dielectric layers are known to be negligibly weak. Counterintuitively, under certain critical conditions, weak nonlocality may build up strong boundary effects that are not captured by conventional (local) effective-medium models based on simple mixing formulas. Here, we show that this phenomenon can be fruitfully studied and understood in terms of error propagation in the iterated maps of the trace and anti-trace of the optical transfer matrix of the multilayer. Our approach effectively parameterizes these peculiar effects via remarkably simple and insightful closed-form expressions, which enable direct identification of the critical parameters and regimes. We also show how these boundary effects can be captured by suitable nonlocal corrections.
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