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Register a new userDynamical detailed balance and local KMS condition for non-equilibrium states
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The principle of detailed balance is at the basis of equilibrium physics and is equivalent to the Kubo-Martin-Schwinger (KMS) condition (under quite general assumptions). In the present paper we prove that a large class of open quantum systems satisfies a dynamical generalization of the detailed balance condition ({it dynamical detailed balance}) expressing the fact that all the micro-currents, associated to the Bohr frequencies are constant. The usual (equilibrium) detailed balance condition is characterized by the property that this constant is identically zero. From this we deduce a simple and experimentally measurable relation expressing the microcurrent associated to a transition between two levels $epsilon_mtoepsilon_n$ as a linear combination of the occupation probabilities of the two levels, with coefficients given by the generalized susceptivities (transport coefficients). Finally, using a master equation characterization of the dynamical detailed balance condition, we show that this condition is equivalent to a local generalization of the usual KMS condition.
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As the core ingredient for spin polarization, the local equilibrium spin distribution function is derived from the detailed balance principle. The kinetic theory for interacting fermionic systems is applied to the Nambu--Jona-Lasinio model at quark level. Under the semi-classical expansion with respect to $hbar$ and non-perturbative expansion with respect to $N_c$, the kinetic equations for the vector and axial-vector distribution functions are derived with collision terms. It is found that, for an initially unpolarized system, non-zero spin polarization can be generated at the order of $hbar$ from the coupling between the vector and axial-vector charges. The local equilibrium spin polarization is derived from the requirement of detailed balance. It arises from the thermal vorticity and is orthogonal to the particle momentum.
We develop an open-system dynamical theory of the Casimir interaction between coherent atomic waves and a material surface. The system --- the external atomic waves --- disturbs the environment --- the electromagnetic field and the atomic dipole degrees of freedom --- in a non- local manner by leaving footprints on distinct paths of the atom interferometer. This induces a non-local dynamical phase depending simultaneously on two distinct paths, beyond usual atom-optics methods, and comparable to the local dynamical phase corrections. Non-local and local atomic phase coherences are thus equally important to capture the interplay between the external atomic motion and the Casimir interaction. Such dynamical phases are obtained for finite-width wavepackets by developing a diagrammatic expansion of the disturbed environment quantum state.
Quantum detailed balance conditions and quantum fluctuation relations are two important concepts in the dynamics of open quantum systems: both concern how such systems behave when they thermalize because of interaction with an environment. We prove that for thermalizing quantum dynamics the quantum detailed balance conditions yield the validity of a quantum fluctuation relation (where only forward-time dynamics is considered). This implies that to have such a quantum fluctuation relation (which in turn enables a precise formulation of the second law of thermodynamics for quantum systems) it suffices to fulfill the quantum detailed balance conditions. We, however, show that the converse is not necessarily true; indeed, there are cases of thermalizing dynamics which feature the quantum fluctuation relation without satisfying detailed balance. We illustrate our results with three examples.
Even photosynthesis -- the most basic natural phenomenon underlying Life on Earth -- involves the non-trivial processing of excitations at the pico- and femtosecond scales during light-harvesting. The desire to understand such natural phenomena, as well as interpret the output from ultrafast experimental probes, creates an urgent need for accurate quantitative theories of open quantum systems. However it is unclear how best to generalize the well-established assumptions of an isolated system, particularly under non-equilibrium conditions. Here we compare two popular approaches: a description in terms of a direct product of the states of each individual system (i.e. a local approach) versus the use of new states resulting from diagonalizing the whole Hamiltonian (i.e. a global approach). We show that their equivalence fails when the system is open, in particular under the experimentally ubiquitous condition of a temperature gradient. By solving for the steady-state populations and calculating the heat flux as a test observable, we uncover stark differences between the formulations. This divergence highlights the need to establish rigorous ranges of applicability for such methods in modeling nanoscale transfer phenomena -- including during the light-harvesting process in photosynthesis.
We extend the new perturbation formula of equilibrium states by Hastings to KMS states of general $W^*$-dynamical systems.
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