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Register a new userModelling dynamics of samples exposed to free-electron-laser radiation with Boltzmann equations
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We apply Boltzmann equations for modelling the radiation damage in samples irradiated by photons from free electron laser (FEL). We test this method in a study case of a spherically symmetric xenon cluster irradiated with VUV FEL photons. The results obtained demonstrate the potential of the Boltzmann method for describing the complex and non-equilibrium dynamics of samples exposed to FEL radiation.
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We compute molecular continuum orbitals in the single center expansion scheme. We then employ these orbitals to obtain molecular Auger rates and single-photon ionization cross sections to study the interaction of N2 with Free-Electron-Laser (FEL) pulses. The nuclei are kept fixed. We formulate rate equations for the energetically allowed molecular and atomic transitions and we account for dissociation through additional terms in the rate equations. Solving these equations for different parameters of the FEL pulse, allows us to identify the most efficient parameters of the FEL pulse for obtaining the highest contribution of double core hole states (DCH) in the final atomic ion fragments. Finally we identify the contribution of DCH states in the electron spectra and show that the DCH state contribution is more easily identified in the photo-ionization rather than the Auger transitions.
The dynamics of energetic particles in strong electromagnetic fields can be heavily influenced by the energy loss arising from the emission of radiation during acceleration, known as radiation reaction. When interacting with a high-energy electron beam, todays lasers are sufficiently intense to explore the transition between the classical and quantum radiation reaction regimes. We report on the observation of radiation reaction in the collision of an ultra-relativistic electron beam generated by laser wakefield acceleration ($varepsilon > 500$ MeV) with an intense laser pulse ($a_0 > 10$). We measure an energy loss in the post-collision electron spectrum that is correlated with the detected signal of hard photons ($gamma$-rays), consistent with a quantum (stochastic) description of radiation reaction. The generated $gamma$-rays have the highest energies yet reported from an all-optical inverse Compton scattering scheme, with critical energy $varepsilon_{rm crit} > $ 30 MeV.
A nanometer-sized dielectric particle lying on a dielectric substrate is exposed to the flux of low-energy electrons, ion and electron fluxes from a cold plasma and the fluxes from the combination of these two sources with the help of particle-in-cell simulation to investigate the particle lofting phenomenon. The results are of interest for dust mitigation in the semiconductor industry, the lunar exploration, and the explanation of the dust levitation.
Using the Madelung transformation we show that in a quantum Free Electron Laser (QFEL) the beam obeys the equations of a quantum fluid in which the potential is the classical potential plus a quantum potential. The classical limit is shown explicitly.
All carbon materials, e.g., amorphous carbon (a-C) coatings and C60 fullerene thin films, play an important role in short-wavelength free-electron laser (FEL) research motivated by FEL optics development and prospective nanotechnology applications. Responses of a-C and C60 layers to the extreme ultraviolet (SPring-8 Compact SASE Source in Japan) and soft x-ray (free-electron laser in Hamburg) free-electron laser radiation are investigated by Raman spectroscopy, differential interference contrast, and atomic force microscopy. A remarkable difference in the behavior of covalent (a-C) and molecular (C60) carbonaceous solids is demonstrated under these irradiation conditions. Low thresholds for ablation of a fullerene crystal (estimated to be around 0.15 eV/atom for C60 vs 0.9 eV/atom for a-C in terms of the absorbed dose) are caused by a low cohesive energy of fullerene crystals. An efficient mechanism of the removal of intact C60 molecules from the irradiated crystal due to Coulomb repulsion of fullerene-cage cation radicals formed by the ionizing radiation is revealed by a detailed modeling.
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