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Register a new userLiquid Xe scintillation calorimetry and Xe optical properties
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Added by
Giovanni Signorelli
Publication date
2004
fields
Physics
and research's language is
English
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The optical properties of LXe in the vacuum ultra violet (VUV), determining the performance of a scintillation calorimeter, are discussed in detail. The available data, measured in a wider spectral region from visible to UV light, and in a large range of Xe densities, from gas to liquid, are examined. It is shown that this information can be used for deriving the LXe optical properties in the VUV. A comparison is made with the few direct measurements in LXe for VUV light resulting from the LXe excitation by ionizing particles. A useful relation is obtained which connects the Rayleigh scattering length to the refractive index in LXe.
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Vacuum ultraviolet light emission from xenon-doped liquid argon is described in the context of liquid noble gas particle detectors. Xenon concentrations in liquid argon from 0.1 ppm to 1000 ppm were studied. The energy transfer from the second excimer continuum of argon ($sim$127 nm) to the second excimer continuum of xenon ($sim$174 nm) is observed by recording optical emission spectra. The transfer almost saturates at a xenon concentration of $sim$10 ppm for which, in addition, an intense emission in the infrared at a peak wavelength of 1.17 $mu$m with (13000$pm$4000) photons per MeV deposited by electrons had been found. The corresponding value for the VUV emission at a peak wavelength of 174 nm (second excimer continuum of xenon) is determined to be (20000$pm$6000) photons per MeV electron energy deposited. Under these excitation conditions pure liquid argon emits (22000$pm$3000) photons per MeV electron energy deposited at a peak wavelength of 127nm. An electron-beam induced emission spectrum for the 10 ppm Ar-Xe liquid mixture ranging from 115 nm to 3.5 $mu$m is presented. VUV emission spectra from xenon-doped liquid argon with exponentially varied xenon concentrations from 0.1 ppm to 1000 ppm are also shown. Time structure measurements of the light emissions at well-defined wavelength positions in the vacuum ultraviolet as well as in the near-infrared are presented.
Liquid argon is used as active medium in a variety of neutrino and Dark Matter experiments thanks to its excellent properties of charge yield and transport and as a scintillator. Liquid argon scintillation photons are emitted in a narrow band of 10~nm centered around 127 nm and with a characteristic time profile made by two components originated by the decay of the lowest lying singlet and triplet state of the excimer Ar$_2^*$ to the dissociative ground state. A model is proposed which takes into account the quenching of the long lived triplet states through the self-interaction with other triplet states or through the interaction with molecular Ar$_2^+$ ions. The model predicts the time profile of the scintillation signals and its dependence on the intensity of an external electric field and on the density of deposited energy, if the relative abundance of the unquenched fast and slow components is know. The model successfully explains the experimentally observed dependence of the characteristic time of the slow component on the intensity of the applied electric field and the increase of photon yield of liquid argon when doped with small quantities of xenon (at the ppm level). The model also predicts the dependence of the pulse shape parameter, F$_{prompt}$, for electron and nuclear recoils on the recoil energy and the behavior of the relative light yield of nuclear recoils in liquid argon, $mathcal{L}_{eff}$
We present the results of our recent studies of a Thick Gaseous Electron Multiplier (THGEM)-based detector, operated in Ar, Xe and Ar:Xe (95:5) at various gas pressures. Avalanche-multiplication properties and energy resolution were investigated with soft x-rays for different detector configurations and parameters. Gains above 10E4 were reached in a double-THGEM detector, at atmospheric pressure, in all gases, in almost all the tested conditions; in Ar:Xe (95:5) similar gains were reached at pressures up to 2 bar. The energy resolution dependence on the gas, pressure, hole geometry and electric fields was studied in detail, yielding in some configurations values below 20% FWHM with 5.9 keV x-rays.
We describe a system to transport and identify barium ions produced in liquid xenon, as part of R&D towards the second phase of a double beta decay experiment, nEXO. The goal is to identify the Ba ion resulting from an extremely rare nuclear decay of the isotope $^{136}$Xe, hence providing a confirmation of the occurrence of the decay. This is achieved through Resonance Ionization Spectroscopy (RIS). In the test setup described here, Ba ions can be produced in liquid xenon or vacuum and collected on a clean substrate. This substrate is then removed to an analysis chamber under vacuum, where laser-induced thermal desorption and RIS are used with time-of-flight (TOF) mass spectroscopy for positive identification of the barium decay product.
Optically hyperpolarized $^{129}$Xe gas has become a powerful contrast agent in nuclear magnetic resonance (NMR) spectroscopy and imaging, with applications ranging from studies of the human lung to the targeted detection of biomolecules. Equally attractive is its potential use to enhance the sensitivity of microfluidic NMR experiments, in which small sample volumes yield poor sensitivity. Unfortunately, most $^{129}$Xe polarization systems are large and non-portable. Here we present a microfabricated chip that optically polarizes $^{129}$Xe gas. We have achieved $^{129}$Xe polarizations greater than 0.5$%$ at flow rates of several microliters per second, compatible with typical microfluidic applications. We employ in situ optical magnetometry to sensitively detect and characterize the $^{129}$Xe polarization at magnetic fields of 1 $mu$T. We construct the device using standard microfabrication techniques, which will facilitate its integration with existing microfluidic platforms. This device may enable the implementation of highly sensitive $^{129}$Xe NMR in compact, low-cost, portable devices.
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