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Negative heat capacity in the critical region of nuclear fragmentation: an experimental evidence of the liquid-gas phase transition

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 Added by Dagostino Michela
 Publication date 1999
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and research's language is English




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An experimental indication of negative heat capacity in excited nuclear systems is inferred from the event by event study of energy fluctuations in $Au$ quasi-projectile sources formed in $Au+Au$ collisions at 35 A.MeV. The excited source configuration is reconstructed through a calorimetric analysis of its de-excitation products. Fragment partitions show signs of a critical behavior at about 5 A.MeV excitation energy. In the same energy range the heat capacity shows a negative branch providing a direct evidence of a first order liquid gas phase transition.



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We have observed a bimodal behaviour of the distribution of the asymmetry between the charges of the two heaviest products resulting from the decay of the quasi-projectile released in binary Xe+Sn and Au+Au collisions from 60 to 100 MeV/u. Event sorting has been achieved through the transverse energy of light charged particles emitted on the quasi-target side, thus avoiding artificial correlations between the bimodality signal and the sorting variable. Bimodality is observed for intermediate impact parameters for which the quasi-projectile is identified. A simulation shows that the deexcitation step rather than the geometry of the collision appears responsible for the bimodal behaviour. The influence of mid-rapidity emission has been verified. The two bumps of the bimodal distribution correspond to different excitation energies and similar temperatures. It is also shown that it is possible to correlate the bimodality signal with a change in the distribution of the heaviest fragment charge and a peak in potential energy fluctuations. All together, this set of data is coherent with what would be expected in a finite system if the corresponding system in the thermodynamic limit exhibits a first order phase transition.
Critical temperature Tc for the nuclear liquid-gas phase transition is stimated both from the multifragmentation and fission data. In the first case,the critical temperature is obtained by analysis of the IMF yields in p(8.1 GeV)+Au collisions within the statistical model of multifragmentation (SMM). In the second case, the experimental fission probability for excited 188Os is compared with the calculated one with Tc as a free parameter. It is concluded for both cases that the critical temperature is higher than 16 MeV.
A global protocol for the thermostatistical analysis of hot nuclear sources is discussed. Within our method of minimization of variances we show that the abnormal kinetic energy fluctuation signal recently reported in different experimental data (M.DAgostino et al.-Phys. Lett. B 473 (2000) 219, N. Le Neindre et al.- contr. to the XXXVIII Bormio Winter Meeting on Nucl. Phys. (2001) 404) is a genuine signal of a first order phase transition in a finite system.
190 - A. Lavagno , D. Pigato 2013
We study an effective relativistic mean-field model of nuclear matter with arbitrary proton fraction at finite temperature in the framework of nonextensive statistical mechanics, characterized by power-law quantum distributions. We investigate the presence of thermodynamic instability in a warm and asymmetric nuclear medium and study the consequent nuclear liquid-gas phase transition by requiring the Gibbs conditions on the global conservation of baryon number and electric charge fraction. We show that nonextensive statistical effects play a crucial role in the equation of state and in the formation of mixed phase also for small deviations from the standard Boltzmann-Gibbs statistics.
We present first-principle predictions for the liquid-gas phase transition in symmetric nuclear matter employing both two- and three-nucleon chiral interactions. Our discussion focuses on the sources of systematic errors in microscopic quantum many body predictions. On the one hand, we test uncertainties of our results arising from changes in the construction of chiral Hamiltonians. We use five different chiral forces with consistently derived three-nucleon interactions. On the other hand, we compare the ladder resummation in the self-consistent Greens functions approach to finite temperature Brueckner--Hartree--Fock calculations. We find that systematics due to Hamiltonians dominate over many-body uncertainties. Based on this wide pool of calculations, we estimate that the critical temperature is $T_c=16 pm 2$ MeV, in reasonable agreement with experimental results. We also find that there is a strong correlation between the critical temperature and the saturation energy in microscopic many-body simulations.
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