Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userInvestigation of the ferromagnetic transition in the correlated 4d perovskites SrRu$_{1-x}$Rh$_x$O$_3$
85
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
The solid-solution SrRu$_{1-x}$Rh$_x$O$_3$ ($0le x le1$) is a variable-electron-configuration system forming in the nearly-cubic-perovskite basis, ranging from the ferromagnetic 4$d^4$ to the enhanced paramagnetic 4$d^5$. Polycrystalline single-phase samples were obtained over the whole composition range by a high-pressure-heating technique, followed by measurements of magnetic susceptibility, magnetization, specific heat, thermopower, and electrical resistivity. The ferromagnetic order in long range is gradually suppressed by the Rh substitution and vanishes at $x sim 0.6$. The electronic term of specific-heat shows unusual behavior near the critical Rh concentration; the feature does not match even qualitatively with what was reported for the related perovskites (Sr,Ca)RuO$_3$. Furthermore, another anomaly in the specific heat was observed at $x sim 0.9$.
rate research
Read More
The quasi-skutterudite superconductor Sr$_3$Rh$_4$Sn$_{13}$ features a pronounced anomaly in electrical resistivity at $T^*sim$138 K. We show that the anomaly is caused by a second-order structural transition, which can be tuned to 0 K by applying physical pressure and chemical pressure via the substitution of Ca for Sr. A broad superconducting dome is centred around the structural quantum critical point. Detailed analysis of the tuning parameter dependence of $T^*$ as well as insights from lattice dynamics calculations strongly support the existence of a structural quantum critical point at ambient pressure when the fraction of Ca is 0.9 (i.e., $x_c=0.9$). This establishes (Ca$_x$Sr$_{1-x}$)$_3$Rh$_4$Sn$_{13}$ series as an important system for exploring the physics of structural quantum criticality without the need of applying high pressures.
SrAuSi$_3$ is a noncentrosymmetric superconductor (NCS) with $T_c$ = 1.54 K, which to date has been studied only via macroscopic techniques. By combining nuclear magnetic resonance (NMR) and muon-spin rotation ($mu$SR) measurements we investigate both the normal and the superconducting phase of SrAuSi$_3$ at a local level. In the normal phase, our data indicate a standard metallic behavior with weak electron correlations and a Korringa constant $S_mathrm{exp} = 1.31 times 10^{-5}$ sK. The latter, twice the theoretical value, can be justified by the Moriya theory of exchange enhancement. In the superconducting phase, the material exhibits conventional BCS-type superconductivity with a weak-coupling s-wave pairing, a gap value $Delta(0)$ = 0.213(2) meV, and a magnetic penetration depth $lambda(0)$ = 398(2) nm. The experimental proof of weak correlations in SrAuSi$_{3}$ implies that correlation effects can be decoupled from those of antisymmetric spin-orbit coupling (ASOC), thus enabling accurate band-structure calculations in the weakly-correlated NCSs.
We present a systematic investigation of the electrical, structural, and antiferromagnetic properties for the series of Ba(Fe$_{1-x-y}$Co$_{x}$Rh$_{y}$)$_{2}$As$_{2}$ compounds with fixed $x approx$ 0.027 and $ 0 leq y leq 0.035$. We compare our results for the Co-Rh doped Ba(Fe$_{1-x-y}$Co$_{x}$Rh$_{y}$)$_{2}$As$_{2}$ compounds with the Co doped Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ compounds. We demonstrate that the electrical, structural, antiferromangetic, and superconducting properties of the Co-Rh doped compounds are similar to the properties of the Co doped compounds. We find that the overall behaviors of Ba(Fe$_{1-x-y}$Co$_{x}$Rh$_{y}$)$_{2}$As$_{2}$ and Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ compounds are very similar when the total number of extra electrons per Fe/$TM$ ($TM$ = transition metal) site is considered, which is consistent with the rigid band model. Despite the similarity, we find that the details of the transitions, for example, the temperature difference between the structural and antiferromagnetic transition temperatures and the incommensurability of the antiferromangetic peaks, are different between Ba(Fe$_{1-x-y}$Co$_{x}$Rh$_{y}$)$_{2}$As$_{2}$ and Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ compounds.
The interplay between different ordered phases, such as superconducting, charge or spin ordered phases, is of central interest in condensed matter physics. The very recent discovery of superconductivity with a remarkable T$_c$= 26 K in Fe-based oxypnictide La(O$_{1-x}$F$_x$)FeAs is a surprise to the scientific communitycite{Kamihara08}. The pure LaOFeAs itself is not superconducting but shows an anomaly near 150 K in both resistivity and dc magnetic susceptibility. Here we provide combined experimental and theoretical evidences showing that the anomaly is caused by the spin-density-wave (SDW) instability, and electron-doping by F suppresses the SDW instability and recovers the superconductivity. Therefore, the La(O$_{1-x}$F$_x$)FeAs offers an exciting new system showing competing orders in layered compounds.
Perovskite oxides ABO$_3$ containing heavy B-site elements are a class of candidate materials to host topological metals with a large spin-orbit interaction. In contrast to the band insulator BaSnO$_3$, the semimetal BaPbO$_3$ is proposed to be a typical example with an inverted band structure, the conduction band of which is composed of mainly the O-2p orbital. In this study, we exemplify a band-gap modification by systematic structural, optical, and transport measurements in BaSn$_{1-x}$Pb$_x$O$_3$ films. A sudden suppression of the conductivity and an enhancement of the weak antilocalization effect at $x$ = 0.9 indicate the presence of a singular point in the electronic structure as a signature of the band inversion. Our findings provide an intriguing platform for combining topological aspects and electron correlation in perovskite oxides based on band-gap engineering.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
