We studied the specific heat and thermal conductivity of the spin-triplet superconductor Sr2RuO4 at low temperatures and under oriented magnetic fields H. We resolved a double peak structure of the superconducting transition under magnetic field for the first time, which provides thermodynamic evidence for the existence of multiple superconducting phases. We also found a clear limiting of the upper critical field Hc2 for the field direction parallel to the RuO2 plane only within 2 degrees. The limiting of Hc2 occurs in the same H-T domain of the second superconducting phase; we suggest that the two phenomena have the same physical origin.
The magnetoresistance and magnetic torque of FeS are measured in magnetic fields $B$ of up to 18 T down to a temperature of 0.03 K. The superconducting transition temperature is found to be $T_c$ = 4.1 K, and the anisotropy ratio of the upper critical field $B_{c2}$ at $T_c$ is estimated from the initial slopes to be $Gamma(T_c)$ = 6.9. $B_{c2}(0)$ is estimated to be 2.2 and 0.36 T for $B parallel ab$ and $c$, respectively. Quantum oscillations are observed in both the resistance and torque. Two frequencies $F$ = 0.15 and 0.20 kT are resolved and assigned to a quasi-two-dimensional Fermi surface cylinder. The carrier density and Sommerfeld coefficient associated with this cylinder are estimated to be 5.8 $times$ 10$^{-3}$ carriers/Fe and 0.48 mJ/(K$^2$mol), respectively. Other Fermi surface pockets still remain to be found. Band-structure calculations are performed and compared to the experimental results.
By means of the magnetocaloric effect, we examine the nature of the superconducting-normal (S-N) transition of Sr2RuO4, a most promising candidate for a spin-triplet superconductor. We provide thermodynamic evidence that the S-N transition of this oxide is of first order below approximately 0.8 K and only for magnetic field directions very close to the conducting plane, in clear contrast to the ordinary type-II superconductors exhibiting second-order S-N transitions. The entropy release across the transition at 0.2 K is 10% of the normal-state entropy. Our result urges an introduction of a new mechanism to break superconductivity by magnetic field.
We present measurements of the superconducting critical temperature Tc and upper critical field Hc2 as a function of pressure in the transition metal dichalcogenide 2H-NbS2 up to 20 GPa. We observe that Tc increases smoothly from 6K at ambient pressure to about 8.9K at 20GPa. This range of increase is comparable to the one found previously in 2H-NbSe2. The temperature dependence of the upper critical field Hc2(T) of 2H-NbS2 varies considerably when increasing the pressure. At low pressures, Hc2(0) decreases, and at higher pressures both Tc and Hc2(0) increase simultaneously. This points out that there are pressure induced changes of the Fermi surface, which we analyze in terms of a simplified two band approach.
We report large enhancement of upper critical field Hc2 observed in superconducting Sr2RuO4 thin films. Through dimensional crossover approaching two dimensions, Hc2 except the in-plane field direction is dramatically enhanced compared to bulks, following a definite relation distinct from bulk one between Hc2 and the transition temperature. The anomalous enhancement of Hc2 is highly suggestive of important changes of the superconducting properties, possibly accompanied with rotation of the triplet d-vector. Our findings will become a crucial step to further explore exotic properties by employing Sr2RuO4 thin films.
We investigate the specific heat of ultra-pure single crystals of Sr2RuO4, a leading candidate of a spin-triplet superconductor. We for the first time obtained specific-heat evidence of the first-order superconducting transition below 0.8 K, namely divergent-like peaks and clear hysteresis in the specific heat at the upper critical field. The first-order transition occurs for all in-plane field directions. The specific-heat features for the first-order transition are found to be highly sensitive to sample quality; in particular, the hysteresis becomes totally absent in a sample with slightly lower quality. These thermodynamic observations provide crucial bases to understand the unconventional pair-breaking effect responsible for the first-order transition.
Kazuhiko Deguchi
,Makariy Tanatar
,Zhiqiang Mao
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(2002)
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"Superconducting Double Transition and the Upper Critical Field Limit of Sr2RuO4 in Parallel Magnetic Fields"
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Kazuhiko Deguchi
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