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Register a new userObservation of the Fulde-Ferrell-Larkin-Ovchinnikov state in the quasi-two-dimensional organic superconductor $kappa$-(BEDT-TTF)$_2$Cu(NCS)$_2$
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Single crystals of the layered organic type II superconductor, $kappa$-(BEDT-TTF)$_{2}$Cu(NCS)$_{2}$, have been studied in magnetic fields of up to 33 T and at temperatures between 0.5 K and 11 K using a compact differential susceptometer. When the magnetic field lies precisely in the quasi-two-dimensional planes of the material, there is strong evidence for a phase transition from the superconducting mixed state into a Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state, manisfested as a change in the rigidity of the vortex system. The behaviour of the transition as a function of temperature is in good agreement with theoretical predictions.
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The specific heat of the layered organic superconductor $kappa$-% (BEDT-TTF)$_2$Cu(NCS)$_2$, where BEDT-TTF is bisethylenedithio-% tetrathiafulvalene, has been studied in magnetic fields up to 28 T applied perpendicular and parallel to the superconducting layers. In parallel fields above 21 T, the superconducting transition becomes first order, which signals that the Pauli-limiting field is reached. Instead of saturating at this field value, the upper critical field increases sharply and a second first-order transition line appears within the superconducting phase. Our results give strong evidence that the phase, which separates the homogeneous superconducting state from the normal state is a realization of a Fulde-Ferrell-Larkin-Ovchinnikov state.
We consider a two-component Fermi gas in the presence of spin imbalance, modeling the system in terms of a one-dimensional attractive Hubbard Hamiltonian initially in the presence of a confining trap potential. With the aid of the time-evolving block decimation method, we investigate the dynamics of the initial state when the trap is switched off. We show that the dynamics of a gas initially in the Fulde-Ferrel-Larkin-Ovchinnikov (FFLO) state is decomposed into the independent expansion of two fluids, namely the paired and the unpaired particles. In particular, the expansion velocity of the unpaired cloud is shown to be directly related to the FFLO momentum. This provides an unambiguous signature of the FFLO state in a remarkably simple way.
Low temperature scanning tunneling spectroscopy reveals the local density of states of the organic superconductor $kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br, that was cut in-situ in ultra-high vacuum perpendicular to the superconducting BEDT-TTF layers. The spectra confirm that superconductivity is confined to the conducting BEDT-TTF layers, while the Cu[N(CN)$_2$]Br anion layers are insulating. The density of states comprises a twofold superconducting gap, which is attributed to the two separated bands crossing the Fermi surface.
Nuclear magnetic resonance measurements were performed on CeCu$_{2}$Si$_{2}$ in the presence of a magnetic field close to the upper critical field $mu_{0} H_{rm c2}$ in order to investigate its superconducting (SC) properties near pair-breaking fields. In lower fields, the Knight shift and nuclear spin-lattice relaxation rate divided by temperature $1/T_1T$ abruptly decreased below the SC transition temperature $T_{rm c}(H)$, a phenomenon understood within the framework of conventional spin-singlet superconductivity. In contrast, $1/T_1T$ was enhanced just below $T_{rm c}(H)$ and exhibited a broad maximum when magnetic fields close to $mu_0H_{rm c2}(0)$ were applied parallel or perpendicular to the $c$ axis, although the Knight shift decreased just below $T_{rm c}(H)$. This enhancement of $1/T_1T$, which was recently observed in the organic superconductor $kappa$-(BEDT-TTF)$_{2}$Cu(NCS)$_{2}$, suggests the presence of high-density Andreev bound states in the inhomogeneous SC region, a hallmark of the Fulde-Ferrell-Larkin-Ovchinnikov phase.
The density of states of the organic superconductor $kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br, measured by scanning tunneling spectroscopy on textit{in-situ} cleaved surfaces, reveals a logarithmic suppression near the Fermi edge persisting above the critical temperature $T_mathrm{c}$. A soft Hubbard gap as predicted by the Anderson-Hubbard model for systems with disorder exactly describes the experimentally observed suppression. The electronic disorder also explains the diminished coherence peaks of the quasiparticle density of states below $T_mathrm{c}$.
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