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Register a new userHot carrier dynamics and electron-optical phonon coupling in photoexcited graphene via time-resolved ultrabroadband terahertz spectroscopy
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Added by
Masatsugu Yamashita
Publication date
2021
fields
Physics
and research's language is
English
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Electron-electron (e-e) interaction is known as a source of logarithmic renormalizations for Dirac fermions in quantum field theory. The renormalization of electron--optical phonon coupling (EPC) by e-e interaction, which plays a pivotal role in hot carrier and phonon dynamics, has been discussed after the discovery of graphene. We investigate the hot carrier dynamics and the EPC strength using time-resolved ultrabroadband terahertz (THz) spectroscopy combined with numerical simulation based on the Boltzmann transport equation and comprehensive temperature model. The large negative photoconductivity and the non-Drude behavior of THz conductivity spectra appear under high pump fluence and can be attributed to the temporal variation of the hot carrier distribution and scattering rate. We successfully estimate the dimensionless EPC matrix element of the $A_1^{prime}$ optical phonon mode near the $mathbf{K}$ point as $lambda_{mathbf{K}} approx$0.09 from the fitting of THz conductivity spectra and temporal evolution of transient THz reflectivity, which is slightly larger than the prediction of the renormalization group.
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We propose and analyze the concept of the vertical hot-electron terahertz (THz) graphene-layer detectors (GLDs) based on the double-GL and multiple-GL structures with the barrier layers made of materials with a moderate conduction band off-set (such as tungsten disulfide and related materials). The operation of these detectors is enabled by the thermionic emissions from the GLs enhanced by the electrons heated by incoming THz radiation. The electron heating is primarily associated with the intraband absorption (the Drude absorption). We calculate the responsivity and detectivity as functions of the photon energy, GL doping, and the applied voltage for the GL detectors (GLDs) with different number of GLs. The detectors based on the cascade multiple-GL structures can exhibit a substantial photoelectric gain resulting in the elevated responsivity and detectivity. The advantages of the THz detectors under consideration are associated with their high sensitivity to the normal incident radiation and efficient operation at room temperature at the low end of the THz frequency range. Such GLDs with a metal grating, supporting the excitation of plasma oscillations in the GL-structures by the incident THz radiation, can exhibit a strong resonant response at the frequencies of several THz (in the range, where the operation of the conventional detectors based on A$_3$B$_5$ materials, in particular THz quantum-well detectors, is hindered due to a strong optical phonon radiation absorption in such materials).
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