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Improving radioactive contaminant identification through the analysis of delayed coincidences with an $alpha$-spectrometer

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 Added by Davide Chiesa
 Publication date 2021
  fields Physics
and research's language is English




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In the framework of rare event searches, the identification of radioactive contaminants in ultra-pure samples is a challenging task, because the signal is often at the same level of the instrumental background. This is a rather common situation for $alpha$-spectrometers and other detectors used for low-activity measurements. In order to obtain the target sensitivity without extending the data taking live-time, analysis strategies that highlight the presence of the signal sought should be developed. In this paper, we show how to improve the contaminant tagging capability relying on the time-correlation of radioactive decay sequences. We validate the proposed technique by measuring the impurity level of both contaminated and ultra-pure copper samples, demonstrating the potential of this analysis tool in disentangling different background sources and providing an effective way to mitigate their impact in rare event searches.



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Localization and modeling of radioactive contaminations is a challenge that ultra-low background experiments are constantly facing. These are fundamental steps both to extract scientific results and to further reduce the background of the detectors. Here we present an innovative technique based on the analysis of $alpha-alpha$ delayed coincidences in $^{232}$Th and $^{238}$U decay chains, developed to investigate the contaminations of the ZnSe crystals in the CUPID-0 experiment. This method allows to disentangle surface and bulk contaminations of the detectors relying on the different probability to tag delayed coincidences as function of the $alpha$ decay position.
To improve the ability of particle identification of the RIBLL2 separator at the HIRFL-CSR complex, a new high-performance detector for measuring fragment starting time and position at the F1 dispersive plane has been constructed and installed, and a method for achieving precise Br{ho} determination has been developed using the experimentally derived ion-optical transfer matrix elements from the measured position and ToF information. Using the high-performance detectors and the precise Br{ho} determination method, the fragments produced by the fragmentation of 78Kr at 300 MeV/nucleon were identified clearly at the RIBLL2-ETF under full momentum acceptance. The atomic number Z resolution of {sigma}Z~0.19 and the mass-to-charge ratio A/Q resolution of {sigma}A/Q~5.8e-3 were obtained for the 75As33+ fragment. This great improvement will increase the collection efficiency of exotic nuclei, extend the range of nuclei of interest from the A<40 mass region up to the A~80 mass region, and promote the development of radioactive nuclear beam experiments at the RIBLL2 separator.
The design, construction and performance characteristics of a simple axial-field ionization chamber suitable for identifying ions in a radioactive beam are presented. Optimized for use with low-energy radioactive beams (< 5 MeV/A) the detector presents only three 0.5 $mu$m/cm$^2$ foils to the beam in addition to the detector gas. A fast charge sensitive amplifier (CSA) integrated into the detector design is also described. Coupling this fast CSA to the axial field ionization chamber produces an output pulse with a risetime of 60-70 ns and a fall time of 100 ns, making the detector capable of sustaining a relatively high rate. Tests with an $alpha$ source establish the detector energy resolution as $sim$8 $%$ for an energy deposit of $sim$3.5 MeV. The energy resolution with beams of 2.5 and 4.0 MeV/A $^{39}$K ions and the dependence of the energy resolution on beam intensity is measured. At an instantaneous rate of 3 x 10$^5$ ions/s the energy resolution has degraded to 14% with a pileup of 12%. The good energy resolution of this detector at rates up to 3 x 10$^5$ ions/s makes it an effective tool in the characterization of low-energy radioactive beams.
Profiting from previous works done with the emph{INDRA} multidetector on the description of the light response $mathcal L$ of the CsI(emph{Tl}) crystals to different impinging nuclei, we propose an improved $Delta E - mathcal L$ identification-calibration procedure for Silicon-Cesium Iodide (Si-CsI) telescopes, namely an Advanced Mass Estimate (emph{AME}) method. emph{AME} is compared to the usual, %$Delta E - E$ simple visual analysis of the corresponding two-dimensional map of $Delta E - E$ type, by using emph{INDRA} experimental data from nuclear reactions induced by heavy ions in the Fermi energy regime. We show that the capability of such telescopes to identify both the atomic $Z$ and the mass $A$ numbers of light and heavy reaction products, can be quantitatively improved thanks to the proposed approach. This conclusion opens new possibilities to use emph{INDRA} for studying these reactions especially with radioactive beams. Indeed, the determination of the mass for charged reaction products becomes of paramount importance to shed light on the role of the isospin degree of freedom in the nuclear equation of state.
298 - N. Fukuda , T. Kubo , T. Ohnishi 2013
We have developed a method for achieving excellent resolving power in in-flight particle identification of radioactive isotope (RI) beams at the BigRIPS fragment separator at the RIKEN Nishina Center RI Beam Factory (RIBF). In the BigRIPS separator, RI beams are identified by their atomic number Z and mass-to-charge ratio A/Q which are deduced from the measurements of time of flight (TOF), magnetic rigidity (Brho) and energy loss (delta-E), and delivered as tagged RI beams to a variety of experiments including secondary reaction measurements. High A/Q resolution is an essential requirement for this scheme, because the charge state Q of RI beams has to be identified at RIBF energies such as 200-300 MeV/nucleon. By precisely determining the Brho and TOF values, we have achieved relative A/Q resolution as good as 0.034% (root-mean-square value). The achieved A/Q resolution is high enough to clearly identify the charge state Q in the Z versus A/Q particle identification plot, where fully-stripped and hydrogen-like peaks are very closely located. The precise Brho determination is achieved by refined particle trajectory reconstruction, while a slew correction is performed to precisely determine the TOF value. Furthermore background events are thoroughly removed to improve reliability of the particle identification. In the present paper we present the details of the particle identification scheme in the BigRIPS separator. The isotope separation in the BigRIPS separator is also briefly introduced.
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