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Register a new userIdentification and Separation of Radioactive Isotope Beams by the BigRIPS Separator at the RIKEN RI Beam Factory
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We have developed a method for achieving excellent resolving power in in-flight particle identification of radioactive isotope (RI) beams at the BigRIPS fragment separator at the RIKEN Nishina Center RI Beam Factory (RIBF). In the BigRIPS separator, RI beams are identified by their atomic number Z and mass-to-charge ratio A/Q which are deduced from the measurements of time of flight (TOF), magnetic rigidity (Brho) and energy loss (delta-E), and delivered as tagged RI beams to a variety of experiments including secondary reaction measurements. High A/Q resolution is an essential requirement for this scheme, because the charge state Q of RI beams has to be identified at RIBF energies such as 200-300 MeV/nucleon. By precisely determining the Brho and TOF values, we have achieved relative A/Q resolution as good as 0.034% (root-mean-square value). The achieved A/Q resolution is high enough to clearly identify the charge state Q in the Z versus A/Q particle identification plot, where fully-stripped and hydrogen-like peaks are very closely located. The precise Brho determination is achieved by refined particle trajectory reconstruction, while a slew correction is performed to precisely determine the TOF value. Furthermore background events are thoroughly removed to improve reliability of the particle identification. In the present paper we present the details of the particle identification scheme in the BigRIPS separator. The isotope separation in the BigRIPS separator is also briefly introduced.
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We have measured the production rates and production cross sections for a variety of radioactive isotopes which were produced from 124Xe, 48Ca, and 238U beams at an energy of 345 MeV/nucleon using the BigRIPS separator at the RIKEN Nishina Center RI Beam Factory (RIBF). Proton-rich isotopes with atomic numbers Z = 40 to 52 and neutron-rich isotopes with Z = 5 to 16 were produced by projectile fragmentation of the 124Xe and 48Ca beam on Be targets, respectively. Neutron-rich isotopes with Z = 20 to 59 were produced by in-flight fission of the 238U beam, in which both Be and Pb were used as production targets. The measured production rates and production cross sections were compared with those of the LISE++ calculations, and overall fairly good agreement has been obtained. Furthermore, in the measurements with the 124Xe beam, we have discovered four new isotopes on the proton-drip line, 85,86Ru and 81,82Mo, and obtained the clear evidence that 103Sb is particle unbound with an upper limit of 49 ns for the half-life. The measurements of projectile-fragment momentum distributions have been also performed with the 124Xe beam, in which the low-momentum tails of the distributions have been measured for the first time at the energy of 345 MeV/nucleon.
To improve the ability of particle identification of the RIBLL2 separator at the HIRFL-CSR complex, a new high-performance detector for measuring fragment starting time and position at the F1 dispersive plane has been constructed and installed, and a method for achieving precise Br{ho} determination has been developed using the experimentally derived ion-optical transfer matrix elements from the measured position and ToF information. Using the high-performance detectors and the precise Br{ho} determination method, the fragments produced by the fragmentation of 78Kr at 300 MeV/nucleon were identified clearly at the RIBLL2-ETF under full momentum acceptance. The atomic number Z resolution of {sigma}Z~0.19 and the mass-to-charge ratio A/Q resolution of {sigma}A/Q~5.8e-3 were obtained for the 75As33+ fragment. This great improvement will increase the collection efficiency of exotic nuclei, extend the range of nuclei of interest from the A<40 mass region up to the A~80 mass region, and promote the development of radioactive nuclear beam experiments at the RIBLL2 separator.
The design, construction and performance characteristics of a simple axial-field ionization chamber suitable for identifying ions in a radioactive beam are presented. Optimized for use with low-energy radioactive beams (< 5 MeV/A) the detector presents only three 0.5 $mu$m/cm$^2$ foils to the beam in addition to the detector gas. A fast charge sensitive amplifier (CSA) integrated into the detector design is also described. Coupling this fast CSA to the axial field ionization chamber produces an output pulse with a risetime of 60-70 ns and a fall time of 100 ns, making the detector capable of sustaining a relatively high rate. Tests with an $alpha$ source establish the detector energy resolution as $sim$8 $%$ for an energy deposit of $sim$3.5 MeV. The energy resolution with beams of 2.5 and 4.0 MeV/A $^{39}$K ions and the dependence of the energy resolution on beam intensity is measured. At an instantaneous rate of 3 x 10$^5$ ions/s the energy resolution has degraded to 14% with a pileup of 12%. The good energy resolution of this detector at rates up to 3 x 10$^5$ ions/s makes it an effective tool in the characterization of low-energy radioactive beams.
A challenge preventing successful inverse kinematics measurements with heavy nuclei that are not fully stripped is identifying and tagging the beam particles. For this purpose, the HEavy ISotope Tagger (HEIST) has been developed. HEIST utilizes two micro-channel plate timing detectors to measure time of flight, a multi-sampling ion chamber to measure energy loss, and a high purity Ge detector to identify isomer decays and calibrate the isotope identification system. HEIST has successfully identified $^{198}$Pb and other nearby nuclei at energies of about 75 MeV/A. In the experiment discussed, a typical cut containing 89% of all $^{198}$Pb$^{+80}$ in the beam had a purity of 86%. We examine the issues of charge state contamination. The observed charge state populations of these ions are presented and are moderately well described by the charge state model GLOBAL.
Ions with similar charge-to-mass ratios cannot be separated from existing beam profile monitors (BPMs) in nuclear facilities in which low-energy radioactive ions are produced due to nuclear fusion reactions. In this study, we developed a BPM using a microchannel plate and a charge-coupled device to differentiate the beam profiles of alpha-decaying radioactive isotopes from other ions (reaction products) produced in a nuclear reaction. This BPM was employed to optimize the low-energy radioactive francium ion (Fr+) beam developed at the Cyclotron and Radioisotope Center (CYRIC), Tohoku University, for electron permanent electric dipole moment (e-EDM) search experiments using Fr atoms. We demonstrated the performance of the BPM by separating the Fr+ beam from other reaction products produced during the nuclear fusion reaction of an oxygen (18O) beam and gold (197Au) target. However, as the mass of Au is close to that of Fr, separating the ions of these elements using a mass filter is a challenge, and a dominant number of Au+ renders the Fr+ beam profile invisible when using a typical BPM. Therefore, by employing the new BPM, we could successfully observe the Fr+ beam and other ion beams distinctly by measuring the alpha decay of Fr isotopes. This novel technique to monitor the alpha-emitting radioactive beam covers a broad range of lifetimes, for example, from approximately 1 s to 10 min, and can be implemented for other alpha-emitter beams utilized for medical applications.
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