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Spectroscopy of Rydberg States in Erbium using Electromagnetically Induced Transparency

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 Added by Manfred Mark
 Publication date 2021
  fields Physics
and research's language is English




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We present a study of the Rydberg spectrum in ts{166}Er for series connected to the $4f^{12} (^3H_6) 6s$, $J_c=13/2 $ and $J_c=11/2 $ ionic core states using an all-optical detection based on electromagnetically induced transparency in an effusive atomic beam. Identifying approximately 550 individual states, we find good agreement with a multi-channel quantum defect theory (MQDT) which allows assignment of most states to $ns$ or $nd$ Rydberg series. We provide an improved accuracy for the lowest two ionization thresholds to $E_{textrm{IP}, J_c = 13/2 } = 49260.750(1),$cm$^{-1}$ and $E_{textrm{IP}, J_c = 11/2 } = 49701.184(1),$cm$^{-1}$ as well as the corresponding quantum defects for all observed series. We identify Rydberg states in five different isotopes, and states between the two lowest ionization thresholds. Our results open the way for future applications of Rydberg states for quantum simulation using erbium and exploiting its special open-shell structure.



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We present combined measurements of the spatially-resolved optical spectrum and the total excited-atom number in an ultracold gas of three-level atoms under electromagnetically induced transparency conditions involving high-lying Rydberg states. The observed optical transmission of a weak probe laser at the center of the coupling region exhibits a double peaked spectrum as a function of detuning, whilst the Rydberg atom number shows a comparatively narrow single resonance. By imaging the transmitted light onto a charge-coupled-device camera, we record hundreds of spectra in parallel, which are used to map out the spatial profile of Rabi frequencies of the coupling laser. Using all the information available we can reconstruct the full one-body density matrix of the three-level system, which provides the optical susceptibility and the Rydberg density as a function of spatial position. These results help elucidate the connection between three-level interference phenomena, including the interplay of matter and light degrees of freedom and will facilitate new studies of many-body effects in optically driven Rydberg gases.
We report on the all-optical detection of Rydberg states in a effusive atomic beam of strontium atoms using electromagnetically induced transparency (EIT). Using narrow-linewidth CW lasers we obtain an EIT linewidth of 5 MHz. To illustrate the high spectroscopic resolution offered by this method, we have measured isotope shifts of the 5s18d ^1D_2 and 5s19s ^1S_0 Rydberg states. This technique could be applied to high-resolution, non-destructive measurements of ultra-cold Rydberg gases and plasmas.
142 - Qi Zhang , Zhengyang Bai , 2018
We investigate the transient optical response property of an electromagnetically induced transparency (EIT) in a cold Rydberg atomic gas. We show that both the transient behavior and the steady-state EIT spectrum of the system depend strongly on Rydberg interaction. Especially, the response speed of the Rydberg-EIT can be five-times faster (and even higher) than the conventional EIT without the Rydberg interaction. For comparison, two different theoretical approaches (i.e. two-atom model and many-atom model) are considered, revealing that Rydberg blockade effect plays a significant role for increasing the response speed of the Rydberg-EIT. The fast-responding Rydberg-EIT by using the strong, tunable Rydberg interaction uncovered here is not only helpful for enhancing the understanding of the many-body dynamics of Rydberg atoms but also useful for practical applications in quantum information processing by using Rydberg atoms.
We present an experimental study of cavity assisted Rydberg atom electromagnetically induced transparency (EIT) using a high-finesse optical cavity ($F sim 28000$). Rydberg atoms are excited via a two-photon transition in a ladder-type EIT configuration. A three-peak structure of the cavity transmission spectrum is observed when Rydberg EIT is generated inside the cavity. The two symmetrically spaced side peaks are caused by bright-state polaritons, while the central peak corresponds to a dark-state polariton. Anti-crossing phenomenon and the effects of mirror adsorbate electric fields are studied under different experimental conditions. We determine a lower bound on the coherence time for the system of $7.26 pm 0.06 ,mu$s, most likely limited by laser dephasing. The cavity-Rydberg EIT system can be useful for single photon generation using the Rydberg blockade effect, studying many-body physics, and generating novel quantum states amongst many other applications.
We observe and investigate, both experimentally and theoretically, electromagnetically-induced transparency experienced by evanescent fields arising due to total internal reflection from an interface of glass and hot rubidium vapor. This phenomenon manifests itself as a non-Lorentzian peak in the reflectivity spectrum, which features a sharp cusp with a sub-natural width of about 1 MHz. The width of the peak is independent of the thickness of the interaction region, which indicates that the main source of decoherence is likely due to collisions with the cell walls rather than diffusion of atoms. With the inclusion of a coherence-preserving wall coating, this system could be used as an ultra-compact frequency reference.
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