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Register a new userColossal anomalous Nernst effect in a correlated noncentrosymmetric kagome ferromagnet
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Analogous to the Hall effect, the Nernst effect is the generation of a transverse voltage due to a temperature gradient in the presence of a perpendicular magnetic field. The Nernst effect has promise for thermoelectric applications and as a probe of electronic structure. In magnetic materials, a so-called anomalous Nernst effect (ANE) is possible in zero magnetic field. Here we report a colossal ANE reaching 23 $mu$V/K in the ferromagnetic metal UCo$_{0.8}$Ru$_{0.2}$Al. Uraniums $5f$ electrons provide strong electronic correlations that lead to narrow bands, which are a known route to producing a large thermoelectric response. Additionally, the large nuclear charge of uranium generates strong spin-orbit coupling, which produces an intrinsic transverse response in this material due to the Berry curvature associated with the relativistic electronic structure. Theoretical calculations show that at least 148 Weyl nodes and two nodal lines exist within $pm$ 60 meV of the Fermi level in UCo$_{0.8}$Ru$_{0.2}$Al. This work demonstrates that magnetic actinide materials can host strong Nernst and Hall responses due to their combined correlated and topological nature.
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We present magnetotransport data on the ferrimagnet GdMn$_6$Sn$_6$. From the temperature dependent data we are able to extract a large instrinsic contribution to the anomalous Hall effect $sigma_{xz}^{int} sim$ 32 $Omega^{-1}cm^{-1}$ and $sigma_{xy}^{int} sim$ 223 $Omega^{-1}cm^{-1}$, which is comparable to values found in other systems also containing kagome nets of transition metals. From our transport anisotropy, as well as our density functional theory calculations, we argue that the system is electronically best described as a three dimensional system. Thus, we show that reduced dimensionality is not a strong requirement for obtaining large Berry phase contributions to transport properties. In addition, the coexistence of rare-earth and transition metal magnetism makes the hexagonal MgFe$_6$Ge$_6$ structure type a promising system to tune the electronic and magnetic properties in future studies.
We report a detailed investigation of the Ni$_{2}$MnGa shape memory alloy through magnetic, electronic, and thermal measurements. Our measurements of the anomalous Nernst effect (ANE) reveal that this technique is very sensitive to the onset of the pre-martensitic transition in sharp contrast to other transport measurements. With the ANE being sensitive to changes at the Fermi surface, we infer on the link between the structural modulations and the modulation of the Fermi surface via its nesting features, with the magnetic field induced strain being the mediating mechanism.
The field of topological electronic materials has seen rapid growth in recent years, in particular with the increasing number of weakly interacting systems predicted and observed to host topologically non-trivial bands. Given the broad appearance of topology in such systems, it is expected that correlated electronic systems should also be capable of hosting topologically non-trivial states. Interest in correlated platforms is heightened by the prospect that collective behavior therein may give rise to new types of topological states and phenomena not possible in non-interacting systems. However, to date only a limited number of correlated topological materials have been definitively reported due to both the challenge in calculation of their electronic properties and the experimental complexity of correlation effects imposed on the topological aspects of their electronic structure. Here, we report a de Haas-van Alphen (dHvA) study of the recently discovered kagome metal Fe$_3$Sn$_2$ mapping the massive Dirac states strongly coupled to the intrinsic ferromagnetic order. We observe a pair of quasi-two-dimensional Fermi surfaces arising from the massive Dirac states previously detected by spectroscopic probes and show that these band areas and effective masses are systematically modulated by the rotation of the ferromagnetic moment. Combined with measurements of Berry curvature induced Hall conductivity, we find that along with the Dirac fermion mass, velocity, and energy are suppressed with rotation of the moment towards the kagome plane. These observations demonstrate that strong coupling of magnetic order to electronic structure similar to that observed in elemental ferromagnets can be extended to topologically non-trivial electronic systems, suggesting pathways for connecting topological states to robust spintronic technologies.
We report magnetic and electrical properties for single crystals of NdMn$_6$Sn$_6$ and SmMn$_6$Sn$_6$. They crystallize into a structure which has distorted, Mn-based kagome lattices, compared to the pristine kagome lattices in heavy-rare-earth-bearing RMn$_6$Sn$_6$ compounds. They are hightemperature ferromagnets of which the R moment is parallel with the Mn moment. We observed a large intrinsic anomalous Hall effect (AHE) that is comparable to the ferrimagnetic, heavy-R siblings in a wide range of temperature. We conclude that their intrinsic AHE is stemming from the Mn-based kagome lattice, just as in the heavy RMn$_6$Sn$_6$.
The origin of anomalous Hall effect (AHE) in magnetic materials is one of the most intriguing aspect in condensed matter physics and has been controversial for a long time. Recent studies indicate that the intrinsic AHE is closely related to the Berry curvature of occupied electronic states. In a magnetic Weyl semimetal with broken time-reversal symmetry, there are significant contributions on Berry curvature around Weyl nodes, which would lead to a large intrinsic AHE. Here, we report the large intrinsic AHE in the half-metallic ferromagnet Co3Sn2S2 single crystal. By systematically mapping out the electronic structure of Co3Sn2S2 theoretically and experimentally, the large intrinsic AHE should originate from the Weyl fermions near the Fermi energy. Furthermore, the intrinsic anomalous Hall conductivity depends linearly on the magnetization and this can be attributed to the sharp decrease of magnetization and the change of topological characteristics.
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