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Register a new userTemperature dependence of the anomalous Nernst effect in Ni$_{2}$MnGa shape memory alloy
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We report a detailed investigation of the Ni$_{2}$MnGa shape memory alloy through magnetic, electronic, and thermal measurements. Our measurements of the anomalous Nernst effect (ANE) reveal that this technique is very sensitive to the onset of the pre-martensitic transition in sharp contrast to other transport measurements. With the ANE being sensitive to changes at the Fermi surface, we infer on the link between the structural modulations and the modulation of the Fermi surface via its nesting features, with the magnetic field induced strain being the mediating mechanism.
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Magneto-structural instability in the ferromagnetic shape memory alloy of composition Ni$_2$Mn$_{1.4}$Sn$_{0.6}$ is investigated by transport and magnetic measurements. Large negative magnetoresistance is observed around the martensitic transition temperature (90-210 K). Both magnetization and magnetoresistance data indicate that upon the application of an external magnetic field at a constant temperature, the sample attains a field-induced arrested state which persists even when the field is withdrawn. We observe an intriguing behavior of the arrested state that it can remember the last highest field it has experienced. The field-induced structural transition plays the key role for the observed anomaly and the observed irreversibility can be accounted by the Landau-type free energy model for the first order phase transition.
Magnetic shape memory Heusler alloys are multiferroics stabilized by the correlations between electronic, magnetic and structural order. To study these correlations we use time resolved x-ray diffraction and magneto-optical Kerr effect experiments to measure the laser induced dynamics in a Heusler alloy Ni$_2$MnGa film and reveal a set of timescales intrinsic to the system. We observe a coherent phonon which we identify as the amplitudon of the modulated structure and an ultrafast phase transition leading to a quenching of the incommensurate modulation within 300~fs with a recovery time of a few ps. The thermally driven martensitic transition to the high temperature cubic phase proceeds via nucleation within a few ps and domain growth limited by the speed of sound. The demagnetization time is 320~fs, which is comparable to the quenching of the structural modulation.
We report on the observation of temperature and field dependent anomalous Nernst effect (ANE) in Ni-rich bulk Ni-Co-Mn-Sn full Heusler alloy. A large change in the transverse Nernst coefficient (N) is obtained across the first order magnetostructural transition from a tetragonal martensite to a cubic austenite phase. The saturation of ANE and magnetic data appear to depend largely on the magnetic anisotropy of the device. Such change in the Nernst co-efficient may prove to be useful for switching applications controlled by temperature and magnetic field changes.
The ground state properties of the ferromagnetic shape memory alloy of nominal composition Ni2Mn1.36Sn0.64 have been studied by dc magnetization and ac susceptibility measurements. Like few other Ni-Mn based alloys, this sample exhibits exchange bias phenomenon. The observed exchange bias pinning was found to originate right from the temperature where a step-like anomaly is present in the zero-field-cooled magnetization data. The ac susceptibility study indicates the onset of spin glass freezing near this step-like anomaly with clear frequency shift. The sample can be identified as a reentrant spin glass with both ferromagnetic and glassy phases coexisting together at low temperature at least in the field-cooled state. The result provides us an comprehensive view to identify the magnetic character of various Ni-Mn-based shape memory alloys with competing magnetic interactions.
Ti50 Pd50-xCrx is a high temperature shape memory alloy with a martensitic transformation temperature strongly dependent on the Cr composition. Prior to the transformation a premartensitic phase is present with an incommensurate modulated cubic lattice with wave vector of q0=(0.22, 0.22, 0). The temperature dependence of the diffuse scattering in the cubic phase is measured as a function temperature for x=6.5, 8.5, and 10 at. %. The lattice dynamics has been studied and reveals anomalous temperature and q-dependence of the [110]-TA2 transverse phonon branch. The phonon linewidth is broad over the entire Brillouin zone and increases with decreasing temperature, contrary to the behavior expected for anharmonicity. No anomaly is observed at q0. The results are compared with first principles calculation of the phonon structure.
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