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Register a new userFrequency stabilization of a quantum cascade laser by weak resonant feedback from a Fabry-P{e}rot cavity
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Frequency-stabilized mid-infrared lasers are valuable tools for precision molecular spectroscopy. However, their implementation remains limited by complicated stabilization schemes. Here we achieve optical self-locking of a quantum cascade laser to the resonant leak-out field of a highly mode-matched two-mirror cavity. The result is a simple approach to achieving ultra-pure frequencies from high-powered mid-infrared lasers. For short time scales (<0.1 ms), we report a linewidth reduction factor of $3times10^{-6}$ to a linewidth of 12 Hz. Furthermore, we demonstrate two-photon cavity-enhanced absorption spectroscopy of an N$_{2}$O overtone transition near a wavelength of 4.53 $mu$m.
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The nitrogen-vacancy (NV) center in diamond has been established as a prime building block for quantum networks. However, scaling beyond a few network nodes is currently limited by low spin-photon entanglement rates, resulting from the NV centers low probability of coherent photon emission and collection. Integration into a cavity can boost both values via the Purcell effect, but poor optical coherence of near-surface NV centers has so far prevented their resonant optical control, as would be required for entanglement generation. Here, we overcome this challenge, and demonstrate resonant addressing of individual, fiber-cavity-coupled NV centers, and collection of their Purcell-enhanced coherent photon emission. Utilizing off-resonant and resonant addressing protocols, we extract Purcell factors of up to 4, consistent with a detailed theoretical model. This model predicts that the probability of coherent photon detection per optical excitation can be increased to 10% for realistic parameters - an improvement over state-of-the art solid immersion lens collection systems by two orders of magnitude. The resonant operation of an improved optical interface for single coherent quantum emitters in a closed-cycle cryogenic system at T $sim$ 4 K is an important result towards extensive quantum networks with long coherence.
We report the relative frequency stabilization of a distributed feedback erbium-doped fiber laser on an optical cavity by serrodyne frequency shifting. A correction bandwidth of 2.3 MHz and a dynamic range of 220 MHz are achieved, which leads to a strong robustness against large disturbances up to high frequencies. We demonstrate that serrodyne frequency shifting reaches a higher correction bandwidth and lower relative frequency noise level compared to a standard acousto-optical modulator based scheme. Our results allow to consider promising applications in the absolute frequency stabilization of lasers on optical cavities.
We present homogeneous quantum cascade lasers (QCLs) emitting around 3 THz which display bandwidths up to 950 GHz with a single stable beatnote. Devices are spontaneously operating in a harmonic comb state, and when in a dense mode regime they can be injection locked at the cavity roundtrip frequency with very small RF powers down to -55 dBm. When operated in the electrically unstable region of negative differential resistance, the device displays ultra-broadband operation exceeding 1.83 THz ($Delta f/f=50%$) with high phase noise, exhibiting self-sustained, periodic voltage oscillations. The low CW threshold (115 A$cdot$ cm$^{-2}$) and broadband comb operation ($Delta f/f=25%$) make these sources extremely appealing for on-chip frequency comb applications.
Quantum cascade lasers are proving to be instrumental in the development of compact frequency comb sources at mid-infrared and terahertz frequencies. Here we demonstrate a heterogeneous terahertz quantum cascade laser with two active regions spaced exactly by one octave. Both active regions are based on a four-quantum well laser design and they emit a combined 3~mW peak power at 15~K in pulsed mode. The two central frequencies are 2.3~THz (bandwidth 300~GHz) and 4.6~THz (bandwidth 270~GHz). The structure is engineered in a way that allows simultaneous operation of the two active regions in the comb regime, serving as a double comb source as well as a test bench structure for all waveguide internal self-referencing techniques. Narrow RF beatnotes ($sim$ 15~kHz) are recorded showing the simultaneous operation of the two combs, whose free-running coherence properties are investigated by means of beatnote spectroscopy performed both with an external detector and via self-mixing. Comb operation in a highly dispersive region (4.6~THz) relying only on gain bandwidth engineering shows the potential for broad spectral coverage with compact comb sources.
Quantum cascade laser (QCL)-pumped molecular lasers (QPMLs) have recently been introduced as a new source of powerful (>1 mW), tunable (>1 THz), narrow-band (<10 kHz), continuous-wave terahertz radiation. The performance of these lasers depends critically on molecular collision physics, pump saturation, and on the design of the laser cavity. Using a validated three-level model that captures the essential collision and saturation behaviors of the QPML gas nitrous oxide (N2O),we explore how threshold pump power and output terahertz power depend on pump power, gas pressure, as well as on the diameter, length, and output-coupler transmissivity of a cylindrical cavity.The analysis indicates that maximum power occurs as pump saturation is minimized in a manner that depends much more sensitively on pressure than on cell diameter, length, or transmissivity. A near-optimal compact laser cavity can produce more than 10 mW of power tunable over frequencies above 1 THz when pumped by a multi-watt QCL.
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