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Register a new userResonant binding of dielectric particles to metal surface without plasmonics
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High index dielectric spherical particle supports the high-$Q$ resonant Mie modes that results in a regular series of sharp resonances in the radiation pressure. A presence of perfectly conducting metal surface transforms the Mie modes into the extremely high-$Q$ magnetic bonding or electric anti-bonding modes for close approaching of the sphere to the surface. We show that the electromagnetic plane wave with normal incidence results in repulsive or attractive resonant optical forces relative to metal for excitation of the electric bonding or magnetic anti-bonding resonant modes respectively. A magnitude of resonant optical forces reaches order of one nano Newton of magnitude for micron size of silicon particles and power of light $1mW/mu m^2$ that exceeds the gravitational force by four orders. However what is the most remarkable there are steady positions for the sphere between pulling and pushing forces that gives rise to resonant binding of the sphere by metal surface. A frequency of mechanical oscillations of particle around the equilibrium positions reaches a magnitude of order MHz.
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The review is devoted to a discussion of new (and often unexpected) aspects of the old problem of elastic light scattering by small metal particles, whose size is comparable to or smaller than the thickness of the skin layer. The main focus is put on elucidating the physical grounds for these new aspects. It is shown that, in many practically important cases, the scattering of light by such particles, despite their smallness, may have almost nothing in common with the Rayleigh one. The so-called, anomalous scattering and absorption, as well as Fano resonances, including unconventional (associated with the excitation of longitudinal electromagnetic oscillations) and directional Fano resonances, observed only in a small solid angle, are discussed in detail. The review contains a Mathematical Supplement, which includes a summary of the main results of the Mie theory and a discussion of some general properties of the scattering coefficients. In addition to purely academic interest, the phenomena considered in this review can find wide applications in biology, medicine, pharmacology, genetic engineering, imaging of ultra-small objects, ultra-high-resolution spectroscopy, information transmission, recording, and processing, and many other applications and technologies. The reported study was funded by RFBR, project number 19-11-00001 and the project of the Russian Science Foundation No. 19-72-30012, within the framework of which all the original calculations given in this publication were performed.
Raman intensity of Rhodamine B (RhB) is enhanced by inserting a thin high k{appa} dielectric layer which reduces the surface plasmon damping at the gold-graphene interface. The results indicate that the Raman intensity increases sharply by plasmonic resonance enhancement while maintaining efficient fluorescence quenching with optimized dielectric layer thickness.
Evanescent waves in a metal thin film with nonlocality are found to propagate in normal direction to film surface with quenched (to zero) energy dissipation associated with intra-band electron transitions when wave numbers satisfy a resonant condition. It is shown that resonant quenching of energy dissipation (RQED) effect occurs in metal films with thicknesses of less or larger than, but still on the order of, the nonlocality scale length. RQED ceases to exist in metal films whose thickness exceeds a cutoff length or in metal films with local dielectric permittivity. Resonant quenching of energy dissipation is caused by destructive interference of partial contributions to electric displacement field, spatially dispersed over thin film thickness. It is demonstrated that RQED effect can be used for designing a new type of plasmonic waveguides, such as a slit waveguide representing a metal film with a narrow slit filled with a dielectric, to achieve near zero propagation losses for plasmonic modes with few nanometer scale confinement.
Plasmonics allows manipulating light at the nanoscale, but has limitations due to the static nature of nanostructures and lack of tuneability. We propose and theoretically analyse a room-temperature liquid-metal nanodroplet that changes its shape, and therefore tunes the plasmon resonance frequency, due to capillary oscillations. We show the possibility to tune the capillary oscillation frequency of the nanodroplet and to drive the oscillations electrically or mechanically. Employed as a tuneable nanoantenna, the nanodroplet may find applications in sensors, imaging, microscopy, and medicine.
Multivalent particles competing for binding on the same surface can exhibit switch-like behaviour, depending on the concentration of receptors on the surface. When the receptor concentration is low, energy dominates the free energy of binding, and particles having a small number of strongly-binding ligands preferentially bind to the surface. At higher receptor concentrations, multivalent effects become significant, and entropy dominates the binding free energy; particles having many weakly-binding ligands preferentially bind to the surface. Between these two regimes there is a switch-point, at which the surface binds the two species of particles equally strongly. We demonstrate that a simple theory can account for this switch-like behaviour and present numerical calculations that support the theoretical predictions. We argue that binding selectivity based on receptor density, rather than identity, may have practical applications.
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