Do you want to publish a course? Click here

Resonant quenching of plasmon energy dissipation in a metal film with nonlocal dielectric response

142   0   0.0 ( 0 )
 Added by Vladimir Grigoryan
 Publication date 2017
  fields Physics
and research's language is English




Ask ChatGPT about the research

Evanescent waves in a metal thin film with nonlocality are found to propagate in normal direction to film surface with quenched (to zero) energy dissipation associated with intra-band electron transitions when wave numbers satisfy a resonant condition. It is shown that resonant quenching of energy dissipation (RQED) effect occurs in metal films with thicknesses of less or larger than, but still on the order of, the nonlocality scale length. RQED ceases to exist in metal films whose thickness exceeds a cutoff length or in metal films with local dielectric permittivity. Resonant quenching of energy dissipation is caused by destructive interference of partial contributions to electric displacement field, spatially dispersed over thin film thickness. It is demonstrated that RQED effect can be used for designing a new type of plasmonic waveguides, such as a slit waveguide representing a metal film with a narrow slit filled with a dielectric, to achieve near zero propagation losses for plasmonic modes with few nanometer scale confinement.



rate research

Read More

81 - A. Y. Bekshaev 2021
We study the energy and momentum of the surface plasmon-polariton (SPP) excited in a symmetric 3-layer insulator-metal-insulator structure, which is known to support the symmetric (S) mode with the negative group velocity as well as the antisymmetric (AS) mode with only positive energy flow. The electric and magnetic field vectors are calculated via both the phenomenological and the microscopic approach; the latter involves the hydrodynamic model accounting for the quantum statistical effects for the electron gas in metal. Explicit representation for the energy and momentum constituents in the dielectric and in the metal film are obtained, and the wavenumber dependences of the energy and momentum contributions for the whole SPP are analyzed numerically. The various energy and momentum constituents are classified with respect to their origin: field or material, and the physical nature: orbital (canonical) and spin (Belinfante) momentum contributions. The pictures characteristic for the S and AS modes are systematically compared. The results can be useful for the studies and applications of the SPP-induced thin-film effects, in particular, for the charge and spin dynamics in thin-film plasmonic systems.
High index dielectric spherical particle supports the high-$Q$ resonant Mie modes that results in a regular series of sharp resonances in the radiation pressure. A presence of perfectly conducting metal surface transforms the Mie modes into the extremely high-$Q$ magnetic bonding or electric anti-bonding modes for close approaching of the sphere to the surface. We show that the electromagnetic plane wave with normal incidence results in repulsive or attractive resonant optical forces relative to metal for excitation of the electric bonding or magnetic anti-bonding resonant modes respectively. A magnitude of resonant optical forces reaches order of one nano Newton of magnitude for micron size of silicon particles and power of light $1mW/mu m^2$ that exceeds the gravitational force by four orders. However what is the most remarkable there are steady positions for the sphere between pulling and pushing forces that gives rise to resonant binding of the sphere by metal surface. A frequency of mechanical oscillations of particle around the equilibrium positions reaches a magnitude of order MHz.
We study the effect of off-resonant plasmon modes on spaser threshold in nanoparticle-based spasers. We develop an analytical semiclassical model and derive spaser threshold condition accounting for gain coupling to higher-order plasmons. We show that such a coupling originates from inhomogeneity of gain distribution near the metal surface and leads to an upward shift of spaser frequency and population inversion threshold. This effect is similar, albeit significantly weaker, to quenching of plasmon-enhanced fluorescence near metal nanostructures due to excitation of off-resonant modes with wide spectral band. We also show that spaser quenching is suppressed for high gain concentrations and establish a simple criterion for quenching onset, which we support by numerical calculations for spherical geometry.
We describe an effective resonant interaction between two localized wave modes of different nature: a plasmon-polariton at a metal surface and a self-focusing beam (spatial soliton) in a non-linear dielectric medium. Propagating in the same direction, they represent an exotic coupled-waveguide system, where the resonant interaction is controlled by the soliton amplitude. This non-linear system manifests hybridized plasmon-soliton eigenmodes, mutual conversion, and non-adiabatic switching, which offer exciting opportunities for manipulation of plasmons via spatial solitons.
Harmonic generation mechanisms are of great interest in nanoscience and nanotechnology, since they allow generating visible light by using near-infrared radiation, which is particularly suitable for its endless applications in bio-nanophotonics and opto-electronics. In this context, multilayer metal-dielectric nanocavities are widely used for light confinement and waveguiding at the nanoscale. They exhibit intense and localized resonances that can be conveniently tuned in the near-infrared and are therefore ideal for enhancing nonlinear effects in this spectral range. In this work, we experimentally investigate the nonlinear optical response of multilayer metal-dielectric nanocavities. By engineering their absorption efficiency and exploiting their intrinsic interface-induced symmetry breaking, we achieve one order of magnitude higher second-harmonic generation efficiency compared to gold nanostructures featuring the same geometry and resonant behavior. In particular, while the third order nonlinear susceptibility is comparable with that of bulk Au, we estimate a second order nonlinear susceptibility of the order of 1 pm/V, which is comparable with that of typical nonlinear crystals. We envision that our system, which combines the advantages of both plasmonic and dielectric materials, might enable the realization of composite and multi-functional nano-systems for an efficient manipulation of nonlinear optical processes at the nanoscale.
comments
Fetching comments Fetching comments
Sign in to be able to follow your search criteria
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا