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Register a new userMagnetic field-assisted spectral decomposition and imaging of charge states of NV centers in diamond
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With the advent of quantum technology, nitrogen vacancy ($NV$) centers in diamond turn out to be a frontier which provides an efficient platform for quantum computation, communication and sensing applications. Due to the coupled spin-charge dynamics of the $NV$ system, knowledge about $NV$ charge state dynamics can help to formulate efficient spin control sequences strategically. Through this paper we report two spectroscopy-based deconvolution methods to create charge state mapping images of ensembles of $NV$ centers in diamond. First, relying on the fact that an off axis external magnetic field mixes the electronic spins and selectively modifies the photoluminescence (PL) of $NV^-$, we perform decomposition of the optical spectrum for an ensemble of $NV$s and extract the spectra for $NV^-$ and $NV^0$ states. Next, we introduce an optical filter based decomposition protocol and perform PL imaging for $NV^-$ and $NV^0$. Earlier obtained spectra for $NV^-$ and $NV^0$ states are used to calculate their transmissivities through a long pass optical filter. These results help us to determine the spatial distribution of the $NV$ charge states in a diamond sample.
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Characterizing the local internal environment surrounding solid-state spin defects is crucial to harnessing them as nanoscale sensors of external fields. This is especially germane to the case of defect ensembles which can exhibit a complex interplay between interactions, internal fields and lattice strain. Working with the nitrogen-vacancy (NV) center in diamond, we demonstrate that local electric fields dominate the magnetic resonance behavior of NV ensembles at low magnetic field. We introduce a simple microscopic model that quantitatively captures the observed spectra for samples with NV concentrations spanning over two orders of magnitude. Motivated by this understanding, we propose and implement a novel method for the nanoscale localization of individual charges within the diamond lattice; our approach relies upon the fact that the charge induces an NV dark state which depends on the electric field orientation.
We investigated the depth dependence of coherence times of nitrogen-vacancy (NV) centers through precisely depth controlling by a moderately oxidative at 580{deg}C in air. By successive nanoscale etching, NV centers could be brought close to the diamond surface step by step, which enable us to trace the evolution of the number of NV centers remained in the chip and to study the depth dependence of coherence times of NV centers with the diamond etching. Our results showed that the coherence times of NV centers declined rapidly with the depth reduction in their last about 22 nm before they finally disappeared, revealing a critical depth for the influence of rapid fluctuating surface spin bath. By monitoring the coherence time variation with depth, we could make a shallow NV center with long coherence time for detecting external spins with high sensitivity.
We show that nitrogen-vacancy (NV) centers in diamond can produce a novel quantum hyperbolic metamaterial. We demonstrate that a hyperbolic dispersion relation in diamond with NV centers can be engineered and dynamically tuned by applying a magnetic field. This quantum hyperbolic metamaterial with a tunable window for the negative refraction allows for the construction of a superlens beyond the diffraction limit. In addition to subwavelength imaging, this NV-metamaterial can be used in spontaneous emission enhancement, heat transport and acoustics, analogue cosmology, and lifetime engineering. Therefore, our proposal interlinks the two hotspot fields, i.e., NV centers and metamaterials.
We report on the systematic characterization of the optical properties of diamond color centers based on Pb impurities. An ensemble photoluminescence analysis of their spectral emission was performed at different excitation wavelengths in the 405-520 nm range and at different temperatures in the 4-300 K range. The series of observed spectral features consist of different emission lines associated with Pb-related defects. Finally, a room-temperature investigation of single-photon emitters under 490.5 nm laser excitation is reported, revealing different spectral signatures with respect to those already reported under 514 nm excitation. This work represents a substantial progress with respect to previous studies on Pb-related color centers, both in the attribution of an articulated series of spectral features and in the understanding of the formation process of this type of defect, thus clarifying the potential of this system for high-impact applications in quantum technologies.
We report on the observation of a topologically protected edge state at the interface between two topologically distinct domains of the Su-Schrieffer-Heeger model, which we implement in arrays of evanescently coupled dielectric-loaded surface plasmon polariton waveguides. Direct evidence of the topological character of the edge state is obtained through several independent experiments: Its spatial localization at the interface as well as the restriction to one sublattice is confirmed by real-space leakage radiation microscopy. The corresponding momentum-resolved spectrum obtained by Fourier imaging reveals the midgap position of the edge state as predicted by theory.
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