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Photonic spin density (PSD) in the near-field gives rise to exotic phenomena such as photonic skyrmions, optical spin-momentum locking and unidirectional topological edge waves. Experimental investigation of these phenomena requires a nanoscale probe that directly interacts with PSD. Here, we propose and demonstrate that the nitrogen-vacancy (NV) center in diamond can be used as a quantum sensor for detecting the spinning nature of photons. This room temperature magnetometer can measure the local polarization of light in ultra-subwavelength volumes through photon-spin-induced virtual transitions. The direct detection of lights spin density at the nanoscale using NV centers in diamond opens a new frontier for studying exotic phases of photons as well as future on-chip applications in spin quantum electrodynamics (sQED).
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Quantum resources can enhance the sensitivity of a device beyond the classical shot noise limit and, as a result, revolutionize the field of metrology through the development of quantum-enhanced sensors. In particular, plasmonic sensors, which are widely used in biological and chemical sensing applications, offer a unique opportunity to bring such an enhancement to real-life devices. Here, we use bright entangled twin beams to enhance the sensitivity of a plasmonic sensor used to measure local changes in refractive index. We demonstrate a 56% quantum enhancement in the sensitivity of state-of-the-art plasmonic sensor with measured sensitivities on the order of $10^{-10}$RIU$/sqrt{textrm{Hz}}$, nearly 5 orders of magnitude better than previous proof-of-principle implementations of quantum-enhanced plasmonic sensors. These results promise significant enhancements in ultratrace label free plasmonic sensing and will find their way into areas ranging from biomedical applications to chemical detection.
Photonic quantum simulators are promising candidates for providing insight into other small- to medium-sized quantum systems. The available photonic quantum technology is reaching the state where significant advantages arise for the quantum simulation of interesting questions in Heisenberg spin systems. Here we experimentally simulate such spin systems with single photons and linear optics. The effective Heisenberg-type interactions among individual single photons are realized by quantum interference at the tunable direction coupler followed by the measurement process. The effective interactions are characterized by comparing the entanglement dynamics using pairwise concurrence of a four-photon quantum system. We further show that photonic quantum simulations of generalized Heisenberg interactions on a four-site square lattice and a six-site checkerboard lattice are in reach of current technology.
Quantum simulation involves engineering devices to implement different Hamiltonians and measuring their quantized spectra to study quantum many-body systems. Recent developments in topological photonics have shown the possibility of studying novel quantum phenomena by controlling the topological properties of such devices. Here, using coupled arrays of upto 16 high Q nano-cavities we experimentally realize quantum photonic baths which are analogs of the Su-Schrieffer-Heeger model. We investigate the effect of fabrication induced disorder on these baths by probing individual super-modes and demonstrate the design mitigation steps required to overcome the disorder effects on the quantum phenomena.
Kinetic models are essential for describing how molecules interact in a variety of biochemical processes. The estimation of a models kinetic parameters by experiment enables researchers to understand how pathogens, such as viruses, interact with other entities like antibodies and trial drugs. In this work, we report a proof-of-principle experiment that uses quantum sensing techniques to give a more precise estimation of kinetic parameters than is possible with a classical approach. The specific interaction we study is that of bovine serum albumin (BSA) binding to gold via an electrostatic mechanism. BSA is an important protein in biochemical research as it can be conjugated with other proteins and peptides to create sensors with a wide range of specificity. We use single photons generated via parametric down-conversion to probe the BSA-gold interaction in a plasmonic resonance sensor. We find that sub-shot-noise level fluctuations in the sensor signal allow us to achieve an improvement in the precision of up to 31.8% for the values of the kinetic parameters. This enhancement can in principle be further increased in the setup. Our work highlights the potential use of quantum states of light for sensing in biochemical research.
The measurement of parameters that describe kinetic processes is important in the study of molecular interactions. It enables a deeper understanding of the physical mechanisms underlying how different biological entities interact with each other, such as viruses with cells, vaccines with antibodies, or new drugs with specific diseases. In this work, we study theoretically the use of quantum sensing techniques for measuring the kinetic parameters of molecular interactions. The sensor we consider is a plasmonic resonance sensor -- a label-free photonic sensor that is one of the most widely used in research and industry. The first type of interaction we study is the antigen BSA interacting with antibody IgG1, which provides a large sensor response. The second type is the enzyme carbonic anhydrase interacting with the tumor growth inhibitor benzenesulfonamide, which produces a small sensor response. For both types of interaction we consider the use of two-mode Fock states, squeezed vacuum states and squeezed displaced states. We find that these quantum states offer an enhancement in the measurement precision of kinetic parameters when compared to that obtained with classical light. The results may help in the design of more precise quantum-based sensors for studying kinetics in the life sciences.
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