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Does filling-dependent band renormalization aid pairing in twisted bilayer graphene?

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 Publication date 2021
  fields Physics
and research's language is English




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Twisted bilayer graphene exhibits a panoply of many-body phenomena that are intimately tied to the appearance of narrow and well isolated electronic bands near magic-angle. The microscopic ingredients that are responsible for the complex experimental phenomenology include electron-electron (phonon) interactions and non-trivial Bloch wavefunctions associated with the narrow bands. Inspired by recent experiments, we focus here on an interplay of two independent interaction-induced phenomena on superconductivity. We analyze the combined effects of Coulomb interaction driven band-flattening and phonon-mediated attraction due to the exchange of multiple electron-phonon umklapp processes, as a function of filling and twist angle. The former leads to a filling-dependent enhancement of the renormalized density of states, which contributes to a robust increase in the tendency towards pairing in a range of angles near magic-angle. In addition, the minimal spatial extent associated with the Wannier functions develops a non-trivial enhancement as a result of these many-body renormalizations, which can further contribute towards stabilizing the superconducting state over a wider range of fillings and twist-angles.

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We present a simple model that we believe captures the key aspects of the competition between superconducting and insulating states in twisted bilayer graphene. Within this model, the superconducting phase is primary, and arises at generic fillings, but is interrupted by the insulator at commensurate fillings. Importantly, the insulator forms because of electron-electron interactions, but the model is agnostic as to the superconducting pairing mechanism, which need not originate with electron-electron interactions. The model is composed of a collection of crossed one-dimensional quantum wires whose intersections form a superlattice. At each superlattice point, we place a locally superconducting puddle which can exchange Cooper pairs with the quantum wires. We analyze this model assuming weak wire-puddle and wire-wire couplings. We show that for a range of repulsive intrawire interactions, the system is superconducting at `generic incommensurate fillings, with the superconductivity being `interrupted by an insulating phase at commensurate fillings. We further show that the gapped insulating states at commensurate fillings give way to gapless states upon application of external Zeeman fields. These features are consistent with experimental observations in magic-angle twisted bilayer graphenes despite the distinct microscopic details. We further study the full phase diagram of this model and discover that it contains several distinct correlated insulating states, which we characterize herein.
153 - Chao Ma , Qiyue Wang , Scott Mills 2019
Recently twisted bilayer graphene (t-BLG) emerges as a new strongly correlated physical platform near a magic twist angle, which hosts many exciting phenomena such as the Mott-like insulating phases, unconventional superconducting behavior and emergent ferromagnetism. Besides the apparent significance of band flatness, band topology may be another critical element in determining strongly correlated twistronics yet receives much less attention. Here we report compelling evidence for nontrivial noninteracting band topology of t-BLG moire Dirac bands through a systematic nonlocal transport study, in conjunction with an examination rooted in $K$-theory. The moire band topology of t-BLG manifests itself as two pronounced nonlocal responses in the electron and hole superlattice gaps. We further show that the nonlocal responses are robust to the interlayer electric field, twist angle, and edge termination, exhibiting a universal scaling law. While an unusual symmetry of t-BLG trivializes Berry curvature, we elucidate that two $Z_2$ invariants characterize the topology of the moire Dirac bands, validating the topological edge origin of the observed nonlocal responses. Our findings not only provide a new perspective for understanding the emerging strongly correlated phenomena in twisted van der Waals heterostructures, but also suggest a potential strategy to achieve topologically nontrivial metamaterials from topologically trivial quantum materials based on twist engineering.
Recent experiments have observed possible spin- and valley-polarized insulators and spin-triplet superconductivity in twisted double bilayer graphene, a moire structure consisting of a pair of Bernal-stacked bilayer graphene. Besides the continuously tunable band widths controlled by an applied displacement field and twist angle, these moire bands also possess van Hove singularities near the Fermi surface and a field-dependent nesting which is far from perfect. Here we carry out a perturbative renormalization group analysis to unbiasedly study the competition among all possible instabilities in twisted double bilayer graphene and related systems with a similar van Hove fermiology in the presence of weak but finite repulsive interactions. Our key finding is that there are several competing magnetic, valley, charge, and superconducting instabilities arising from interactions in twisted double bilayer graphene, which can be tuned by controlling the displacement field and the twist angle. In particular, we show that spin- or valley-polarized uniform instabilities generically dominate under moderate interactions smaller than the band width, whereas $p$-wave spin-triplet topological superconductivity and exotic spin-singlet modulated paired state become important as the interactions decrease. Realization of our findings in general moire systems with a similar van Hove fermiology should open up new opportunities for manipulating topological superconductivity and spin- or valley-polarized states in highly tunable platforms.
100 - Gal Shavit , Erez Berg , Ady Stern 2021
We introduce and analyze a model that sheds light on the interplay between correlated insulating states, superconductivity, and flavor-symmetry breaking in magic angle twisted bilayer graphene. Using a variational mean-field theory, we determine the normal-state phase diagram of our model as a function of the band filling. The model features robust insulators at even integer fillings, occasional weaker insulators at odd integer fillings, and a pattern of flavor-symmetry breaking at non-integer fillings. Adding a phonon-mediated inter-valley retarded attractive interaction, we obtain strong-coupling superconducting domes, whose structure is in qualitative agreement with experiments. Our model elucidates how the intricate form of the interactions and the particle-hole asymmetry of the electronic structure determine the phase diagram. It also explains how subtle differences between devices may lead to the different behaviors observed experimentally. A similar model can be applied with minor modifications to other moir{e} systems, such as twisted trilayer graphene.
We calculate the interactions between the Wannier functions of the 8-orbital model for twisted bilayer graphene (TBG). In this model, two orbitals per valley centered at the AA regions, the AA-p orbitals, account for the most part of the spectral weight of the flats bands. Exchange and assisted-hopping terms between these orbitals are found to be small. Therefore, the low energy properties of TBG will be determined by the density-density interactions. These interactions decay with the distance much faster than in the two orbital model, following a 1/r law in the absence of gates. The magnitude of the largest interaction in the model, the onsite term between the flat band orbitals, is controlled by the size of the AA regions and is estimated to be ~ 40 meV. To screen this interaction, the metallic gates have to be placed at a distance smaller than 5 nm. For larger distances only the long-range part of the interaction is substantially screened. The model reproduces the band deformation induced by doping found in other approaches within the Hartree approximation. Such deformation reveals the presence of other orbitals in the flat bands and is sensitive to the inclusion of the interactions involving them.
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