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Register a new userTheory of correlated insulators and superconductivity in twisted bilayer graphene
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We introduce and analyze a model that sheds light on the interplay between correlated insulating states, superconductivity, and flavor-symmetry breaking in magic angle twisted bilayer graphene. Using a variational mean-field theory, we determine the normal-state phase diagram of our model as a function of the band filling. The model features robust insulators at even integer fillings, occasional weaker insulators at odd integer fillings, and a pattern of flavor-symmetry breaking at non-integer fillings. Adding a phonon-mediated inter-valley retarded attractive interaction, we obtain strong-coupling superconducting domes, whose structure is in qualitative agreement with experiments. Our model elucidates how the intricate form of the interactions and the particle-hole asymmetry of the electronic structure determine the phase diagram. It also explains how subtle differences between devices may lead to the different behaviors observed experimentally. A similar model can be applied with minor modifications to other moir{e} systems, such as twisted trilayer graphene.
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When bilayer graphene is rotationally faulted to an angle $thetaapprox 1.1^circ$, theory predicts the formation of a flat electronic band and correlated insulating, superconducting, and ferromagnetic states have all been observed at partial band filling. The proximity of superconductivity to correlated insulators has suggested a close relationship between these states, reminiscent of the cuprates where superconductivity arises by doping a Mott insulator. Here, we show that superconductivity can appear without correlated insulating states. While both superconductivity and correlated insulating behavior are strongest near the flat band condition, superconductivity survives to larger detuning of the angle. Our observations are consistent with a competing phases picture, in which insulators and superconductivity arise from disparate mechanisms.
Experiments on graphene bilayers, where the top layer is rotated with respect to the one below, have displayed insulating behavior when the moire bands are partially filled. We calculate the charge distributions in these phases, and estimate the excitation gaps.
Moire systems displaying flat bands have emerged as novel platforms to study correlated electron phenomena. Insulating and superconducting states appear upon doping magic angle twisted bilayer graphene (TBG), and there is evidence of correlation induced effects at the charge neutrality point (CNP) which could originate from spontaneous symmetry breaking. Our theoretical calculations show how optical conductivity measurements can distinguish different symmetry breaking states, and reveal the nature of the correlated states. In the specific case of nematic order, which breaks the discrete rotational symmetry of the lattice, we find that the Dirac cones are displaced, not only in momentum space but also in energy, inducing finite Drude weight at the CNP. We also show that the sign of the dc conductivity anisotropy induced by a nematic order depends on the degree of lattice relaxation, the doping and the nature of the symmetry breaking.
Recent experiments on twisted bilayer graphene have shown a high-temperature parent state with massless Dirac fermions and broken electronic flavor symmetry; superconductivity and correlated insulators emerge from this parent state at lower temperatures. We propose that the superconducting and correlated insulating orders are connected by Wess-Zumino-Witten terms, so that defects of one order contain quanta of another order and skyrmion fluctuations of the correlated insulator are a mechanism for superconductivity. We present a comprehensive listing of plausible low-temperature orders, and the parent flavor symmetry breaking orders. The previously characterized topological nature of the band structure of twisted bilayer graphene plays an important role in this analysis.
Magic-angle twisted bilayer graphene (MATBG) exhibits a range of correlated phenomena that originate from strong electron-electron interactions. These interactions make the Fermi surface highly susceptible to reconstruction when $ pm 1, pm 2, pm 3$ electrons occupy each moir e unit cell and lead to the formation of correlated insulating, superconducting and ferromagnetic phases. While some phases have been shown to carry a non-zero Chern number, the local microscopic properties and topological character of many other phases remain elusive. Here we introduce a set of novel techniques hinging on scanning tunneling microscopy (STM) to map out topological phases in MATBG that emerge in finite magnetic field. By following the evolution of the local density of states (LDOS) at the Fermi level with electrostatic doping and magnetic field, we visualize a local Landau fan diagram that enables us to directly assign Chern numbers to all observed phases. We uncover the existence of six topological phases emanating from integer fillings in finite fields and whose origin relates to a cascade of symmetry-breaking transitions driven by correlations. The spatially resolved and electron-density-tuned LDOS maps further reveal that these topological phases can form only in a small range of twist angles around the magic-angle value. Both the microscopic origin and extreme sensitivity to twist angle differentiate these topological phases from the Landau levels observed near charge neutrality. Moreover, we observe that even the charge-neutrality Landau spectrum taken at low fields is considerably modified by interactions and exhibits an unexpected splitting between zero Landau levels that can be as large as ${sim },3-5$ meV. Our results show how strong electronic interactions affect the band structure of MATBG and lead to the formation of correlation-enabled topological phases.
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