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Register a new userControl of Plasmons in Topological Insulators via Local Perturbations
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We use a fully quantum mechanical approach to demonstrate control of plasmonic excitations in prototype models of topological insulators by molecule-scale perturbations. Strongly localized surface plasmons are present in the host systems, arising from the topologically non-trivial single-particle edge states. A numerical evaluation of the RPA equations for the perturbed systems reveals how the positions and the internal electronic structure of the added molecules affect the degeneracy of the locally confined collective excitations, i.e., shifting the plasmonic energies of the host system and changing their spatial charge density profile. In particular, we identify conditions under which significant charge transfer from the host system to the added molecules occurs. Furthermore, the induced field energy density in the perturbed topological systems due to external electric fields is determined.
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Collective excitations in topologically non-trivial systems have attracted considerable attention in recent years. Here we study plasmons in the Su-Schrieffer-Heeger model whose low-energy electronic band is only partially filled, such that the system is metallic. Using the random phase approximation, we calculate the intra- and inter-band polarization functions and determine the bulk plasmonic dispersion from the dielectric function within the random phase approximation. We find that the sub-lattice basis states strongly affect the polarization functions and therefore control the systems plasmonic excitations. By varying the real-space separation of these local orbitals, one can thus selectively enhance or suppress the plasmonic energies via a tunable trade-off between intra-band and inter-band screening processes. Specifically, this mechanism can be used to stabilize undamped high energy plasmons that have already been reported in related models. We propose scenarios on how to control and observe these effects in experiments.
We investigate in a fully quantum-mechanical manner how the many-body excitation spectrum of topological insulators is affected by the presence of long-range Coulomb interactions. In the one-dimensional Su-Schrieffer-Heeger model and its mirror-symmetric variant strongly localized plasmonic excitations are observed which originate from topologically non-trivial single-particle states. These textit{topological plasmons} inherit some of the characteristics of their constituent topological single-particle states, but they are not equally well protected against disorder due to the admixture of non-topological bulk single-particle states in the polarization function. The strength of the effective Coulomb interactions is also shown to have strong effects on the plasmonic modes. Furthermore, we show how external modifications via dielectric screening and applied electric fields with distinct symmetries can be used to study topological plasmons, thus allowing for experimental verification of our atomistic predictions.
Topological insulators (TIs) host unusual surface states with Dirac dispersion and helical spin texture and hold high potentials for novel applications in spintronics and quantum computing. Control of the chemical potential in these materials is challenging but crucial to realizing the hotly pursued exotic physics, including efficient spin generation1,2, Majorana Fermions3-5, and exciton condensation6,7. Here we report a simple and effective method that can in-situ tune the chemical potential of single-crystal Bi2-xSbxSe3 nanoribbons, with a magnitude significantly larger than traditional electrostatic gating. An electric field parallel to a device channel can shift the chemical potential across the Dirac point, both inside and outside the channel. We attribute this non-local reversible modulation of chemical potential to electric-field-induced charge hopping among defect states, further supported by photocurrent mapping. Our approach enables engineering chemical potential distributions in TIs and opens up tremendous opportunities for investigating fundamental transport mechanisms of charge and composite particles in these materials.
We show that the bulk winding number characterizing one-dimensional topological insulators with chiral symmetry can be detected from the displacement of a single particle, observed via losses. Losses represent the effect of repeated weak measurements on one sublattice only, which interrupt the dynamics periodically. When these do not detect the particle, they realize negative measurements. Our repeated measurement scheme covers both time-independent and periodically driven (Floquet) topological insulators, with or without spatial disorder. In the limit of rapidly repeated, vanishingly weak measurements, our scheme describes non-Hermitian Hamiltonians, as the lossy Su-Schrieffer-Heeger model of Phys. Rev. Lett. 102, 065703 (2009). We find, contrary to intuition, that the time needed to detect the winding number can be made shorter by decreasing the efficiency of the measurement. We illustrate our results on a discrete-time quantum walk, and propose ways of testing them experimentally.
We propose a two-dimensional plasmonic platform - periodically patterned monolayer graphene - which hosts topological one-way edge states operable up to infrared frequencies. We classify the band topology of this plasmonic system under time-reversal-symmetry breaking induced by a static magnetic field. At finite doping, the system supports topologically nontrivial bandgaps with mid-gap frequencies up to tens of terahertz. By the bulk-edge correspondence, these bandgaps host topologically protected one-way edge plasmons, which are immune to backscattering from structural defects and subject only to intrinsic material and radiation loss. Our findings reveal a promising approach to engineer topologically robust chiral plasmonic devices and demonstrate a realistic example of high-frequency topological edge state.
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