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Register a new userFission fragments intrinsic spins and their correlations
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The intrinsic spins and their correlations are the least understood characteristics of fission fragments from both theoretical and experimental points of view. In many nuclear reactions the emerging fragments are typically excited and acquire an intrinsic excitation energy and an intrinsic spin depending on the type of the reactions and interaction mechanism. Both the intrinsic excitation energies and the fragments intrinsic spins and parities are controlled by the interaction mechanism and conservations laws, which lead to their correlations and determines the character of their de-excitation mechanism. We outline here a framework for the theoretical extraction of the intrinsic spin distributions of the fragments and their correlations within the fully microscopic real-time density functional theory formalism and illustrate it on the example of induced fission of $^{236}$U and $^{240}$Pu, using two nuclear energy density functionals. These fission fragment intrinsic spin distributions display new qualitative features previously not discussed in literature. Within this fully microscopic framework we extract for the first time the intrinsic spin distributions of fission fragments of $^{236}$U and $^{240}$Pu as well as the correlations of their intrinsic spins, which have been debated in literature for more than six decades with no definite conclusions so far.
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We present the first fully unrestricted microscopic calculations of the primary fission fragment intrinsic spins and of the fission fragments relative orbital angular momentum for $^{236}$U$^*$, $^{240}$Pu$^*$, and $^{252}$Cf using the time-dependent density functional theory framework. Within this microscopic approach, free of restrictions and unchecked assumptions and which incorporates the relevant physical observables relevant for describing fission, we evaluate the triple distribution of the fission fragment intrinsic spins and of their fission fragments relative orbital angular momentum and show that their dynamics is dominated by their bending collective modes, in contradistinction to the predictions of the existing phenomenological models and some interpretations of experimental data.
It is shown that the unexpected character of the angular correlation between the angle of the primary fission fragment intrinsic spins, recently evaluated by performing very complex time-dependent density functional simulations, which favors fission fragment intrinsic spins pointing in opposite directions, can be understood using simple general arguments.
Several sources of angular anisotropy for fission fragments and prompt neutrons have been studied in neutron-induced fission reactions. These include kinematic recoils of the target from the incident neutron beam and the fragments from the emission of the prompt neutrons, preferential directions of the emission of the fission fragments with respect to the beam axis due to the population of particular transition states at the fission barrier, and forward-peaked angular distributions of pre-equilibrium neutrons which are emitted before the formation of a compound nucleus. In addition, there are several potential sources of angular anisotropies that are more difficult to disentangle: the angular distributions of prompt neutrons from fully accelerated fragments or from scission neutrons, and the emission of neutrons from fission fragments that are not fully accelerated. In this work, we study the effects of the first group of anisotropy sources, particularly exploring the correlations between the fission fragment anisotropy and the resulting neutron anisotropy. While kinematic effects were already accounted for in our Hauser-Feshbach Monte Carlo code, $mathtt{CGMF}$, anisotropic angular distributions for the fission fragments and pre-equilibrium neutrons resulting from neutron-induced fission on $^{233,234,235,238}$U, $^{239,241}$Pu, and $^{237}$Np have been introduced for the first time. The effects of these sources of anisotropy are examined over a range of incident neutron energies, from thermal to 20 MeV, and compared to experimental data from the Chi-Nu liquid scintillator array. The anisotropy of the fission fragments is reflected in the anisotropy of the prompt neutrons, especially as the outgoing energy of the prompt neutrons increases, allowing for an extraction of the fission fragment anisotropy to be made from a measurement of the neutrons.
Fission of $^{180}$Hg produces mass asymmetric fragments which are expected to be influenced by deformed shell-effects at N=56 in the heavy fragment and Z=34 in the light fragment [G. Scamps and C. Simenel, arXiv:1904.01275 (2019)]. To investigate both shell-effects and to determine which one has the main influence on the asymmetry in the region of the $^{180}$Hg, we produce a systematic of Constraint-Hartree-Fock calculations in nuclei with similar N/Z ratio than the $^{178}$Pt. It is found that N=56 determines the asymmetry of systems in this region of the nuclear chart.
The ternary cluster decay of heavy nuclei has been observed in several experiments with binary coincidences between two fragments using detector telescopes (the FOBOS-detectors, JINR, Dubna) placed on the opposite sides from the source of fissioning nuclei. The binary coincidences at a relative angle of 180$^0$ deg. correspond to binary fission or to the decay into three cluster fragments by registration of two nuclei with different masses (e.g.$^{132}$Sn,$^{52-48}$Ca,$^{68-72}$Ni). This marks a new step in the physics of fission-phenomena of heavy nuclei. These experimental results for the collinear cluster tripartition (CCT), refer to the decay into three clusters of comparable masses. In the present work we discuss the various aspects of this ternary fission (FFF) mode. The question of collinearity is analysed on the basis of recent publications. Further insight into the possible decay modes is obtained by the discussion of the path towards larger deformation, towards hyper-deformation and by inspecting details of the potential energy surfaces (PES). In the path towards the extremely deformed states leading to ternary fission, the concept of deformed shells is most important. At the scission configuration the phase space determined by the PESs leads to the final mass distributions. The possibility of formation of fragments of almost equal size ($Z_i$ = 32, 34, 32, for $Z$=98) and the observation of several other fission modes in the same system can be predicted by the PES. The PESs show pronounced minima and valleys, namely for several mass/charge combinations of ternary fragments, which correspond to a variety of collinear ternary fission (multi-modal) decays. The case of the decay of $^{252}$Cf(sf,fff) turns out to be unique due to the presence of deformed shells in the total system and of closed shells in all three nuclei in the decay.
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