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Critical point for Bose-Einstein condensation of excitons in graphite

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 Added by Zengwei Zhu
 Publication date 2020
  fields Physics
and research's language is English




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An exciton is an electron-hole pair bound by attractive Coulomb interaction. Short-lived excitons have been detected by a variety of experimental probes in numerous contexts. An excitonic insulator, a collective state of such excitons, has been more elusive. Here, thanks to Nernst measurements in pulsed magnetic fields, we show that in graphite there is a critical temperature (T = 9.2 K) and a critical magnetic field (B = 47 T) for Bose-Einstein condensation of excitons. At this critical field, hole and electron Landau sub-bands simultaneously cross the Fermi level and allow exciton formation. By quantifying the effective mass and the spatial separation of the excitons in the basal plane, we show that the degeneracy temperature of the excitonic fluid corresponds to this critical temperature. This identification would explain why the field-induced transition observed in graphite is not a universal feature of three-dimensional electron systems pushed beyond the quantum limit.



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Correlations of luminescence intensity have been studied under Bose-Einstein condensation of dipolar excitons in the temperature range of 0.45-4.2 K. Photoexcited dipolar excitons were collected in a lateral trap in GaAs/AlGaAs Schottky-diode heterostructure with single wide (25 nm) quantum well under applied electric bias. Two-photon correlations were measured with the use of a classical Hanbury Brown - Twiss intensity interferometer (time resolution ~0.4 ns). Photon bunching has been observed near the Bose condensation threshold of dipolar excitons determined by the appearance of a narrow luminescence line of exciton condensate at optical pumping increase. The two-photon correlation function shows super-poissonian distribution at time scales of system coherence (<~1 ns). No photon bunching was observed at the excitation pumping appreciably below the condensation threshold. At excitation pumping increasing well above the threshold, when the narrow line of exciton condensate grows in the luminescence spectrum, the photon bunching is decreasing and finally vanishes - the two-photon correlator becomes poissonian reflecting the single-quantum-state origin of excitonic Bose condensate. Under the same conditions a first-order spatial correlator, measured by means of the luminescence interference from spatially separated condensate parts, remains significant. The discovered photon bunching is rather sensitive to temperature: it drops several times with temperature increase from 0.45 K up to 4.2 K. If assumed that the luminescence of dipolar excitons collected in the lateral trap reflects directly coherent properties of interacting exciton gas, the observed phenomenon of photon bunching nearby condensation threshold manifests phase transition in interacting exciton Bose gas.
An asymmetric multi-quantum state magnetic lattice is proposed to host excitons formed in a quantum degenerate gas of ultracold fermionic atoms to simulate Bose-Einstein condensation (BEC) of excitons. A Quasi-two dimensional degenerate gas of excitons can be collected in the in-plane asymmetric magnetic bands created at the surface of the proposed magnetic lattice, where the ultracold fermions simulate separately direct and indirect confined electronhole pairs (spin up fermions-spin down fermions) rising to the statistically degenerate Bose gas and eventually through controlled tunnelling to BEC of excitons. The confinement of the coupled magnetic quantum well (CMQWs) system may significantly improve the condition for long lived exciton BEC. The exciton BEC, formed in CMQWs can be regarded as a suitable host for the multi-qubits (multipartite) systems to be used in quantum information processors.
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To investigate the phenomenon of Bose-Einstein condensation in perfect crystals a hierarchy of equations for reduced density matrices that describes a thermodynamically equilibrium quantum system is employed, the hierarchy being obtained earlier by the author. The thermodynamics of a crystal with a condensate and the one of a crystal with no condensate are constructed in parallel, which is required for studying the phase transition involving Bose-Einstein condensation. The transition is analysed also with the help of the Landau theory of phase transitions which shows that a superfluid state can result either from two consecutive phase transitions or from only one. To demonstrate how the general equations obtained can be applied for a concrete crystal the bifurcation method for solving the equations is utilized. New results concerning properties of the condensate crystals at zero temperature are obtained as well. In the concluding section, the physical concept of the condensate is discussed.
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