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A scanning quantum cryogenic atom microscope at 6 K

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 Added by Benjamin Lev
 Publication date 2020
  fields Physics
and research's language is English




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The Scanning Quantum Cryogenic Atom Microscope (SQCRAMscope) is a quantum sensor in which a quasi-1D quantum gas images electromagnetic fields emitted from a nearby sample. We report improvements to the microscope. Cryogen usage is reduced by replacing the liquid cryostat with a closed-cycle system and modified cold finger, and cryogenic cooling is enhanced by adding a radiation shield. The minimum accessible sample temperature is reduced from 35 K to 5.8 K while maintaining low sample vibrations. A new sample mount is easier to exchange, and quantum gas preparation is streamlined.



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Microscopic imaging of local magnetic fields provides a window into the organizing principles of complex and technologically relevant condensed matter materials. However, a wide variety of intriguing strongly correlated and topologically nontrivial materials exhibit poorly understood phenomena outside the detection capability of state-of-the-art high-sensitivity, high-resolution scanning probe magnetometers. We introduce a quantum-noise-limited scanning probe magnetometer that can operate from room to cryogenic temperatures with unprecedented DC-field sensitivity and micron-scale resolution. The Scanning Quantum Cryogenic Atom Microscope (SQCRAMscope) employs a magnetically levitated atomic Bose-Einstein condensate (BEC), thereby providing immunity to conductive and blackbody radiative heating. It has a field sensitivity of 1.4 nT per resolution-limited point ($sim$2 $mu$m), or 6 nT/$sqrt{text{Hz}}$ per point at its duty cycle. Compared to point-by-point sensors, the long length of the BEC provides a naturally parallel measurement, allowing one to measure nearly one-hundred points with an effective field sensitivity of 600 pT$/sqrt{text{Hz}}$ for each point during the same time as a point-by-point scanner would measure these points sequentially. Moreover, it has a noise floor of 300 pT and provides nearly two orders of magnitude improvement in magnetic flux sensitivity (down to $10^{-6}$ $Phi_0/sqrt{text{Hz}}$) over previous atomic probe magnetometers capable of scanning near samples. These capabilities are, for the first time, carefully benchmarked by imaging magnetic fields arising from microfabricated wire patterns, in a system where samples may be scanned, cryogenically cooled, and easily exchanged. The SQCRAMscope will provide charge transport images at temperatures from room to 4 K in unconventional superconductors and topologically nontrivial materials.
Combining electron paramagnetic resonance (EPR) with scanning tunneling microscopy (STM) enables detailed insight into the interactions and magnetic properties of single atoms on surfaces. A requirement for EPR-STM is the efficient coupling of microwave excitations to the tunnel junction. Here, we achieve a coupling efficiency of the order of unity by using a radiofrequency antenna placed parallel to the STM tip, which we interpret using a simple capacitive-coupling model. We further demonstrate the possibility to perform EPR-STM routinely above 4 K using amplitude as well as frequency modulation of the radiofrequency excitation. We directly compare different acquisition modes on hydrogenated Ti atoms and highlight the advantages of frequency and magnetic field sweeps as well as amplitude and frequency modulation in order to maximize the EPR signal. The possibility to tune the microwave-excitation scheme and to perform EPR-STM at relatively high temperature and high power opens this technique to a broad range of experiments, ranging from pulsed EPR spectroscopy to coherent spin manipulation of single atom ensembles.
We study the single-particle properties of a system formed by ultracold atoms loaded into the manifold of $l=1$ Orbital Angular Momentum (OAM) states of an optical lattice with a diamond chain geometry. Through a series of successive basis rotations, we show that the OAM degree of freedom induces phases in some tunneling amplitudes of the tight-binding model that are equivalent to a net $pi$ flux through the plaquettes and give rise to a topologically non-trivial band structure and protected edge states. In addition, we demonstrate that quantum interferences between the different tunneling processes involved in the dynamics may lead to Aharanov-Bohm caging in the system. All these analytical results are confirmed by exact diagonalization numerical calculations.
Helium atoms in Rydberg states have been manipulated coherently with microwave radiation pulses near a gold surface and near a superconducting NbTiN surface at a temperature of $3 text{K}$. The experiments were carried out with a skimmed supersonic beam of metastable $(1text{s})^1(2text{s})^1, {}^1text{S}_0$ helium atoms excited with laser radiation to $ntext{p}$ Rydberg levels with principal quantum number $n$ between $30$ and $40$. The separation between the cold surface and the center of the collimated beam is adjustable down to $250 mutext{m}$. Short-lived $ntext{p}$ Rydberg levels were coherently transferred to the long-lived $ntext{s}$ state to avoid radiative decay of the Rydberg atoms between the photoexcitation region and the region above the cold surfaces. Further coherent manipulation of the $ntext{s}$ Rydberg levels with pulsed microwave radiation above the surfaces enabled measurements of stray electric fields and allowed us to study the decoherence of the atomic ensemble. Adsorption of residual gas onto the surfaces and the resulting slow build-up of stray fields was minimized by controlling the temperature of the surface and monitoring the partial pressures of H$_2$O, N$_2$, O$_2$ and CO$_2$ in the experimental chamber during the cool-down. Compensation of the stray electric fields to levels below $100 text{mV}/text{cm}$ was achieved over a region of $6 text{mm}$ along the beam-propagation direction which, for the $1770 text{m}/text{s}$ beam velocity, implies the possibility to preserve the coherence of the atomic sample for several microseconds above the cold surfaces.
We describe the design, construction, and performance of an ultra-high vacuum (UHV) scanning tunneling microscope (STM) capable of imaging at dilution-refrigerator temperatures and equipped with a vector magnet. The primary objective of our design is to achieve a high level of modularity by partitioning the STM system into a set of easily separable, interchangeable components. This naturally segregates the UHV needs of STM instrumentation from the typically non-UHV construction of a dilution refrigerator, facilitating the usage of non-UHV materials while maintaining a fully bakeable UHV chamber that houses the STM. The modular design also permits speedy removal of the microscope head from the rest of the system, allowing for repairs, modifications, and even replacement of the entire microscope head to be made at any time without warming the cryostat or compromising the vacuum. Without using cryogenic filters, we measured an electron temperature of 184 mK on a superconducting Al(100) single crystal.
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