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Microscopic imaging of local magnetic fields provides a window into the organizing principles of complex and technologically relevant condensed matter materials. However, a wide variety of intriguing strongly correlated and topologically nontrivial materials exhibit poorly understood phenomena outside the detection capability of state-of-the-art high-sensitivity, high-resolution scanning probe magnetometers. We introduce a quantum-noise-limited scanning probe magnetometer that can operate from room to cryogenic temperatures with unprecedented DC-field sensitivity and micron-scale resolution. The Scanning Quantum Cryogenic Atom Microscope (SQCRAMscope) employs a magnetically levitated atomic Bose-Einstein condensate (BEC), thereby providing immunity to conductive and blackbody radiative heating. It has a field sensitivity of 1.4 nT per resolution-limited point ($sim$2 $mu$m), or 6 nT/$sqrt{text{Hz}}$ per point at its duty cycle. Compared to point-by-point sensors, the long length of the BEC provides a naturally parallel measurement, allowing one to measure nearly one-hundred points with an effective field sensitivity of 600 pT$/sqrt{text{Hz}}$ for each point during the same time as a point-by-point scanner would measure these points sequentially. Moreover, it has a noise floor of 300 pT and provides nearly two orders of magnitude improvement in magnetic flux sensitivity (down to $10^{-6}$ $Phi_0/sqrt{text{Hz}}$) over previous atomic probe magnetometers capable of scanning near samples. These capabilities are, for the first time, carefully benchmarked by imaging magnetic fields arising from microfabricated wire patterns, in a system where samples may be scanned, cryogenically cooled, and easily exchanged. The SQCRAMscope will provide charge transport images at temperatures from room to 4 K in unconventional superconductors and topologically nontrivial materials.
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The Scanning Quantum Cryogenic Atom Microscope (SQCRAMscope) is a quantum sensor in which a quasi-1D quantum gas images electromagnetic fields emitted from a nearby sample. We report improvements to the microscope. Cryogen usage is reduced by replacing the liquid cryostat with a closed-cycle system and modified cold finger, and cryogenic cooling is enhanced by adding a radiation shield. The minimum accessible sample temperature is reduced from 35 K to 5.8 K while maintaining low sample vibrations. A new sample mount is easier to exchange, and quantum gas preparation is streamlined.
Combining electron paramagnetic resonance (EPR) with scanning tunneling microscopy (STM) enables detailed insight into the interactions and magnetic properties of single atoms on surfaces. A requirement for EPR-STM is the efficient coupling of microwave excitations to the tunnel junction. Here, we achieve a coupling efficiency of the order of unity by using a radiofrequency antenna placed parallel to the STM tip, which we interpret using a simple capacitive-coupling model. We further demonstrate the possibility to perform EPR-STM routinely above 4 K using amplitude as well as frequency modulation of the radiofrequency excitation. We directly compare different acquisition modes on hydrogenated Ti atoms and highlight the advantages of frequency and magnetic field sweeps as well as amplitude and frequency modulation in order to maximize the EPR signal. The possibility to tune the microwave-excitation scheme and to perform EPR-STM at relatively high temperature and high power opens this technique to a broad range of experiments, ranging from pulsed EPR spectroscopy to coherent spin manipulation of single atom ensembles.
Quantum computing has been attracting tremendous efforts in recent years. One prominent application is to perform quantum simulations of electron correlations in large molecules and solid-state materials, where orbital degrees of freedom are crucial to quantitatively model electronic properties. Electron orbitals unlike quantum spins obey crystal symmetries, making the atomic orbital in optical lattices a natural candidate to emulate electron orbitals. Here, we construct atom-orbital qubits by manipulating $s$- and $d$-orbitals of atomic Bose-Einstein condensation in an optical lattice. Noise-resilient quantum gate operations are achieved by performing holonomic quantum control, which admits geometrical protection. We find it is critical to eliminate the orbital leakage error in the system. The gate robustness is tested by varying the intensity of the laser forming the lattice. Our work opens up wide opportunities for atom-orbital based quantum information processing, of vital importance to programmable quantum simulations of multi-orbital physics in molecules and quantum materials.
The light-matter interaction can be utilized to qualitatively alter physical properties of materials. Recent theoretical and experimental studies have explored this possibility of controlling matter by light based on driving many-body systems via strong classical electromagnetic radiation, leading to a time-dependent Hamiltonian for electronic or lattice degrees of freedom. To avoid inevitable heating, pump-probe setups with ultrashort laser pulses have so far been used to study transient light-induced modifications in materials. Here, we pursue yet another direction of controlling quantum matter by modifying quantum fluctuations of its electromagnetic environment. In contrast to earlier proposals on light-enhanced electron-electron interactions, we consider a dipolar quantum many-body system embedded in a cavity composed of metal mirrors, and formulate a theoretical framework to manipulate its equilibrium properties on the basis of quantum light-matter interaction. We analyze hybridization of different types of the fundamental excitations, including dipolar phonons, cavity photons, and plasmons in metal mirrors, arising from the cavity confinement in the regime of strong light-matter interaction. This hybridization qualitatively alters the nature of the collective excitations and can be used to selectively control energy-level structures in a wide range of platforms. Most notably, in quantum paraelectrics, we show that the cavity-induced softening of infrared optical phonons enhances the ferroelectric phase in comparison with the bulk materials. Our findings suggest an intriguing possibility of inducing a superradiant-type transition via the light-matter coupling without external pumping. We also discuss possible applications of the cavity-induced modifications in collective excitations to molecular materials and excitonic devices.
Using low-temperature high-magnetic-field scanning tunneling microscopy and spectroscopy (STM/STS), we systematically study a graphene quantum dot (GQD) defined by a circular graphene p-p junction. Inside the GQD, we observe a series of quasi-bound states arising from whispering-gallery-mode (WGM) confinement of the circular junction and directly visualize these quasi-bound states down to atomic dimensions. By applying a strong magnetic field, a large jump in energy of the quasi-bound states, which is about one-half the energy spacing between the quasi-bound states, is observed. Such a behavior results from turning on a {pi} Berry phase of massless Dirac fermions in graphene by a magnetic field. Moreover, our experiment demonstrates that a quasi-bound state splits into two peaks with an energy separation of about 26 meV when the Fermi level crosses the quasi-bound state, indicating that there are strong electron-electron interactions in the GQD.
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