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Transport characterization of magnetic states in Superconductor/Ferromagnet Nb/Co multilayers

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 Added by Vladimir M. Krasnov
 Publication date 2020
  fields Physics
and research's language is English




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Employment of the non-trivial proximity effect in Superconductor/Ferromagnet (S/F) heterostructures for creation of novel superconducting devices requires an accurate control of magnetic states in complex thin-film multilayers composing such devices. In this work we study experimentally in-plane transport properties of micro-structured Nb/Co multilayers. We apply various experimental techniques for characterization of multilayers, including the anisotropic magnetoresistance, the Hall effect and the first-order-reversal-curves analysis. We demonstrate that a combination of those techniques can provide a detailed knowledge of the magnetic state of the multilayer. In particular, we identify the range of existence of the coherently rotating, monodomain scissor-like state. It is anticipated, that in this noncollinear magnetic state the unconventional odd-frequency spin-triplet order parameter should appear. The non-hystertic nature of this state allows reversible tuning of the magnetic orientation. Thus, we identify the range of parameters and the procedure for controllable operation of devices based on such S/F heterostructures.



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In this work, magnetization dynamics is studied in superconductor/ferromagnet/superconductor three-layered films in a wide frequency, field, and temperature ranges using the broad-band ferromagnetic resonance measurement technique. It is shown that in presence of both superconducting layers and of superconducting proximity at both superconductor/ferromagnet interfaces a massive shift of the ferromagnetic resonance to higher frequencies emerges. The phenomenon is robust and essentially long-range: it has been observed for a set of samples with the thickness of ferromagnetic layer in the range from tens up to hundreds of nanometers. The resonance frequency shift is characterized by proximity-induced magnetic anisotropies: by the positive in-plane uniaxial anisotropy and by the drop of magnetization. The shift and the corresponding uniaxial anisotropy grow with the thickness of the ferromagnetic layer. For instance, the anisotropy reaches 0.27~T in experiment for a sample with 350~nm thick ferromagnetic layer, and about 0.4~T in predictions, which makes it a ferromagnetic film structure with the highest anisotropy and the highest natural resonance frequency ever reported. Various scenarios for the superconductivity-induced magnetic anisotropy are discussed. As a result, the origin of the phenomenon remains unclear. Application of the proximity-induced anisotropies in superconducting magnonics is proposed as a way for manipulations with a spin-wave spectrum.
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We study a high-TC superconducting (YBa2Cu3O7-d) / ferromagnetic (Co/Pt multilayer) hybrid which exhibits resistance switching driven by the magnetic history: depending on the direction of the external field, a pronounced decrease or increase of the mixed-state resistance is observed as magnetization reversal occurs within the Co/Pt multilayer. We demonstrate that stray magnetic fields cause these effects via i) creation of vortices/antivortices and ii) magnetostatic pinning of vortices that are induced by the external field.
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We investigate the charge and spin transport in half-metallic ferromagnet ($F$) and superconductor ($S$) nanojunctions. We utilize a self-consistent microscopic method that can accommodate the broad range of energy scales present, and ensures proximity effects that account for the interactions at the interfaces are accurately determined. Two experimentally relevant half-metallic junction types are considered: The first is a $F_1 F_2 S$ structure, where a half-metallic ferromagnet $F_1$ adjoins a weaker conventional ferromagnet $F_2$. The current is injected through the $F_1$ layer by means of an applied bias voltage. The second configuration involves a $S F_1 F_2 F_3 S$ Josephson junction whereby a phase difference $Deltavarphi$ between the two superconducting electrodes generates the supercurrent flow. In this case, the central half-metallic $F_2$ layer is surrounded by two weak ferromagnets $F_1$ and $F_3$. By placing a ferromagnet with a weak exchange field adjacent to an $S$ layer, we are able to optimize the conversion process in which opposite-spin triplet pairs are converted into equal-spin triplet pairs that propagate deep into the half-metallic regions in both junction types. For the tunnel junctions, we study the bias-induced local magnetization, spin currents, and spin transfer torques for various orientations of the relative magnetization angle $theta$ in the $F$ layers. We find that the bias-induced equal-spin triplet pairs are maximized in the half-metal for $thetaapprox90^circ$ and as part of the conversion process, are anticorrelated with the opposite-spin pairs. We show that the charge current density is maximized, corresponding to the occurrence of a large amplitude of equal-spin triplet pairs, when the exchange interaction of the weak ferromagnet is about $0.1E_F.$
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