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Register a new userMagnetic-field-induced delocalization in hybrid electron-nuclear spin ensembles
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Added by
Carlos Meriles Prof
Publication date
2020
fields
Physics
and research's language is
English
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We use field-cycling-assisted dynamic nuclear polarization and continuous radio-frequency (RF) driving over a broad spectral range to demonstrate magnetic-field-dependent activation of nuclear spin transport from strongly-hyperfine-coupled 13C sites in diamond. We interpret our observations with the help of a theoretical framework where nuclear spin interactions are mediated by electron spins. In particular, we build on the results from a 4-spin toy model to show how otherwise localized nuclear spins must thermalize as they are brought in contact with a larger ancilla spin network. Further, by probing the system response to a variable driving field amplitude, we witness stark changes in the RF-absorption spectrum, which we interpret as partly due to contributions from heterogeneous multi-spin sets, whose zero-quantum transitions become RF active thanks to the hybrid electron-nuclear nature of the system. These findings could prove relevant in applications to dynamic nuclear polarization, spin-based quantum information processing, and nanoscale sensing.
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Nuclear magnetism in n-doped semiconductors with positive hyperfine constant is revisited. Two kinds of nuclear magnetic ordering can be induced by resident electrons in a deeply cooled nuclear spin system. At positive nuclear spin temperature below a critical value, randomly oriented nuclear spin polarons similar to that predicted by I. Merkulov [I. Merkulov, Physics of the Solid State 40, 930 (1998)] should emerge. These polarons are oriented randomly and within each polaron nuclear and electron spins are aligned antiferromagnetically. At negative nuclear spin temperature below a critical value we predict another type of magnetic ordering - dynamically induced nuclear ferromagnet. This is a long-range ferromagnetically ordered state involving both electrons and nuclei. It can form if electron spin relaxation is dominated by the hyperfine coupling, rather than by the spin-orbit interaction. Application of the theory to the n-doped GaAs suggests that the ferromagnetic order may be reached at experimentally achievable nuclear spin temperature $Theta_N approx 0.5$ $mu$K and lattice temperature $T_L approx 5$ K.
Recently, magnetic field sensors based on an electron spin of a nitrogen vacancy (NV) center in diamond have been studied both from an experimental and theoretical point of view. This system provides a nanoscale magnetometer, and it is possible to detect a precession of a single spin. In this paper, we propose a sensor consisting of an electron spin and a nuclear spin in diamond. Although the electron spin has a reasonable interaction strength with magnetic field, the coherence time of the spin is relatively short. On the other hand, the nuclear spin has a longer life time while the spin has a negligible interaction with magnetic fields. We show that, through the combination of such two different spins via the hyperfine interaction, it is possible to construct a magnetic field sensor with the sensitivity far beyond that of previous sensors using just a single electron spin.
We report density dependent instabilities in the localised regime of mesoscopic two-dimensional electron systems (2DES) with intermediate strength of background disorder. They are manifested by strong resistance oscillations induced by high perpendicular magnetic fields B_{perp}. While the amplitude of the oscillations is strongly enhanced with increasing B_{perp}, their position in density remains unaffected. The observation is accompanied by an unusual behaviour of the temperature dependence of resistance and activation energies. We suggest the interplay between a strongly interacting electron phase and the background disorder as a possible explanation.
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We demonstrate a method of imaging spatially varying magnetic fields using a thin layer of nitrogen-vacancy (NV) centers at the surface of a diamond chip. Fluorescence emitted by the two-dimensional NV ensemble is detected by a CCD array, from which a vector magnetic field pattern is reconstructed. As a demonstration, AC current is passed through wires placed on the diamond chip surface, and the resulting AC magnetic field patterns are imaged using an echo-based technique with sub-micron resolution over a 140 mu m x 140 mu m field of view, giving single-pixel sensitivity ~100 nT/sqrt{Hz}. We discuss ongoing efforts to further improve sensitivity and potential bioimaging applications such as real-time imaging of activity in functional, cultured networks of neurons.
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