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Register a new userEntangling Nuclear Spins by Dissipation in a Solid-state System
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Entanglement is a fascinating feature of quantum mechanics and a key ingredient in most quantum information processing tasks. Yet the generation of entanglement is usually hampered by undesired dissipation owing to the inevitable coupling of a system with its environment. Here, we report an experiment on how to entangle two $^{13}$C nuclear spins via engineered dissipation in a nitrogen-vacancy system. We utilize the electron spin as an ancilla, and combine unitary processes together with optical pumping of the ancilla to implement the engineered dissipation and deterministically produce an entangled state of the two nuclear spins, independent of their initial states. Our experiment demonstrates the power of engineered dissipation as a tool for generation of multi-qubit entanglement in solid-state systems.
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Generating robust entanglement among solid-state spins is key for applications in quantum information processing and precision sensing. We show here a dissipative approach to generate such entanglement among the hyperfine coupled electron nuclear spins using the rapid optical decay of electronic excited states. The combined dark state interference effects of the optical and microwave driving fields in the presence of spontaneous emission from the short-lived excited state leads to a dissipative formation of an entangled steady state. We show that the dissipative entanglement is generated for any initial state conditions of the spins and is resilient to external field fluctuations. We analyze the scheme both for continuous and pulsed driving fields in the presence of realistic noise sources.
We study the depolarization dynamics of a dense ensemble of dipolar interacting spins, associated with nitrogen-vacancy centers in diamond. We observe anomalously fast, density-dependent, and non-exponential spin relaxation. To explain these observations, we propose a microscopic model where an interplay of long-range interactions, disorder, and dissipation leads to predictions that are in quantitative agreement with both current and prior experimental results. Our results pave the way for controlled many-body experiments with long-lived and strongly interacting ensembles of solid-state spins.
Bells theorem states that no local hidden variable model is compatible with quantum mechanics. Surprisingly, even if we release the locality constraint, certain nonlocal hidden variable models, such as the one proposed by Leggett, may still be at variance with the predictions of quantum physics. Here, we report an experimental test of Leggetts nonlocal model with solid-state spins in a diamond nitrogen-vacancy center. We entangle an electron spin with a surrounding weakly coupled $^{13}C$ nuclear spin and observe that the entangled states violate Leggett-type inequalities by more than four and seven standard deviations for six and eight measurement settings, respectively. Our experimental results are in full agreement with quantum predictions and violate Leggetts nonlocal hidden variable inequality with a high level of confidence.
We demonstrate that efficient optical pumping of nuclear spins in semiconductor quantum dots (QDs) can be achieved by resonant pumping of optically forbidden transitions. This process corresponds to one-to-one conversion of a photon absorbed by the dot into a polarized nuclear spin, which also has potential for initialization of hole spin in QDs. Pumping via the forbidden transition is a manifestation of the optical solid effect, an optical analogue of the effect previously observed in electron spin resonance experiments in the solid state. We find that by employing this effect, nuclear polarization of 65% can be achieved, the highest reported so far in optical orientation studies in QDs. The efficiency of the spin pumping exceeds that employing the allowed transition, which saturates due to the low probability of electron-nuclear spin flip-flop.
We review progress on the use of electron spins to store and process quantum information, with particular focus on the ability of the electron spin to interact with multiple quantum degrees of freedom. We examine the benefits of hybrid quantum bits (qubits) in the solid state that are based on coupling electron spins to nuclear spin, electron charge, optical photons, and superconducting qubits. These benefits include the coherent storage of qubits for times exceeding seconds, fast qubit manipulation, single qubit measurement, and scalable methods for entangling spatially separated matter-based qubits. In this way, the key strengths of different physical qubit implementations are brought together, laying the foundation for practical solid-state quantum technologies.
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