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Register a new userUltrafast All Optical Magnetization Control for Broadband Terahertz Spin Wave Generation
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Terahertz spin waves could be generated on-demand via all-optical manipulation of magnetization by femtosecond laser pulse. Here, we present an energy balance model, which explains the energy transfer rates from laser pulse to electron bath coupled with phonon, spin, and magnetization of five different magnetic metallic thin films: Iron, Cobalt, Nickel, Gadolinium and Ni$_{2}$MnSn Heusler alloy. Two types of transient magnetization dynamics emerge in metallic magnetic thin films based on their Curie temperatures (T$_{C}$): type I (Fe, Co, and Ni with T$_{C}$ > room temperature, RT) and type II films (Gd and Ni$_{2}$MnSn with T$_{C}$ $approx$ RT). We study the effect of laser fluence and pulse width for single Gaussian laser pulses and the effect of metal film thickness on magnetization dynamics. Spectral dynamics show that broadband spin waves up to 24 THz could be generated by all-optical manipulation of magnetization in these nanofilms.
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All-optical pump-probe detection of magnetization precession has been performed for ferromagnetic EuO thin films at 10 K. We demonstrate that the circularly-polarized light can be used to control the magnetization precession on an ultrafast time scale. This takes place within the 100 fs duration of a single laser pulse, through combined contribution from two nonthermal photomagnetic effects, i.e., enhancement of the magnetization and an inverse Faraday effect. From the magnetic field dependences of the frequency and the Gilbert damping parameter, the intrinsic Gilbert damping coefficient is evaluated to be {alpha} approx 3times10^-3.
Identifying materials with an efficient spin-to-charge conversion is crucial for future spintronic applications. The spin Hall effect is a central mechanism as it allows for the interconversion of spin and charge currents. Spintronic material research aims at maximizing its efficiency, quantified by the spin Hall angle $Theta_{textrm{SH}}$ and the spin-current relaxation length $lambda_{textrm{rel}}$. We develop an all-optical method with large sample throughput that allows us to extract $Theta_{textrm{SH}}$ and $lambda_{textrm{rel}}$. Employing terahertz spectroscopy, we characterize magnetic metallic heterostructures involving Pt, W and Cu$_{80}$Ir$_{20}$ in terms of their optical and spintronic properties. We furthermore find indications that the interface plays a minor role for the spin-current transmission. Our analytical model is validated by the good agreement with literature DC values. These findings establish terahertz emission spectroscopy as a reliable tool complementing the spintronics workbench.
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