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Register a new userRotational Quantum Beat Lasing Without Inversion
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In standard lasers, light amplification requires population inversion between an upper and a lower state to break the reciprocity between absorption and stimulated emission. However, in a medium prepared in a specific superposition state, quantum interference may fully suppress absorption while leaving stimulated emission intact, opening the possibility of lasing without inversion. Here we show that lasing without inversion arises naturally during propagation of intense femtosecond laser pulses in air. It is triggered by the combination of molecular ionization and molecular alignment, both unavoidable in intense light fields. The effect could enable inversionless amplification of broadband radiation in many molecular gases, opening unusual opportunities for remote sensing.
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We study the photon generation in a transmission line oscillator coupled to a driven qubit in the presence of a dissipative electromagnetic environment. It has been demonstrated previously that a population inversion in the qubit may lead to a lasing state of the oscillator. Here we show that the circuit can also exhibit the effect of lasing without inversion. This is possible since the coupling to the dissipative environment enhances photon emission as compared to absorption, similar to the recoil effect which was predicted for atomic systems. While the recoil effect is very weak, and so far elusive, the effect described here should be observable with present circuits. We analyze the requirements for the system parameters and environment.
We simulate the pump-probe experiments of lasing in molecular nitrogen ions with particular interest on the effects of rotational wave-packet dynamics. Our computations demonstrate that the coherent preparation of rotational wave packets in N$_2^+$ by an intense short non-resonant pulse results in a modulation of the subsequent emission from $B^2Sigma_u^+ rightarrow X^2Sigma_g^+$ transitions induced by a resonant seed pulse. We model the dynamics of such pumping and emission using density matrix theory to describe the N$_2^+$ dynamics and the Maxwell wave equation to model the seed pulse propagation. We show that the gain and absorption of a delayed seed pulse is dependent on the pump-seed delay, that is, the rotational coherences excited by the pump pulse can modulate the gain and absorption of the delayed seed pulse. Further, we demonstrate that the coherent rotational dynamics of the nitrogen ions can cause lasing without electronic inversion.
We propose a two-magnet design of a drift region for a free-electron laser without inversion (FELWI). By performing direct calculations of the phase shifts for electrons passing the drift region, we prove that the small-signal gain integrated over the detuning is positive and is inversely proportional to the energy spread of the ``hot electron beam. The dispersion and the geometry of the drift region are specified, and the requirements to the electron beam quality, including the transverse size and the angular spread, are found.
We stabilize a chosen radiofrequency beat note between two optical fields derived from the same mode-locked laser pulse train, in order to coherently manipulate quantum information. This scheme does not require access or active stabilization of the laser repetition rate. We implement and characterize this external lock, in the context of two-photon stimulated Raman transitions between the hyperfine ground states of trapped 171-Yb+ quantum bits.
The field of attosecond science was first enabled by nonlinear compression of intense laser pulses to a duration below two optical cycles. Twenty years later, creating such short pulses still requires state-of-the-art few-cycle laser amplifiers to most efficiently exploit instantaneous optical nonlinearities in noble gases for spectral broadening and parametric frequency conversion. Here, we show that nonlinear compression can in fact be much more efficient when driven in molecular gases by pulses substantially longer than a few cycles, due to enhanced optical nonlinearity associated with rotational alignment. We use 80-cycle pulses from an industrial-grade laser amplifier to simultaneously drive molecular alignment and supercontinuum generation in a gas-filled capillary, producing more than two octaves of coherent bandwidth and achieving >45-fold compression to a duration of 1.7 cycles. As the enhanced nonlinearity is linked to rotational motion, the dynamics can be exploited for long-wavelength frequency conversion and compressing picosecond lasers.
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