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Register a new userStrong local moment antiferromagnetic spin fluctuations in V-doped LiFeAs
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We use neutron scattering to study vanadium (hole)-doped LiFe$_{1-x}$V$_x$As. In the undoped state, LiFeAs exhibits superconductivity at $T_c=18$ K and transverse incommensurate spin excitations similar to electron overdoped iron pnictides. Upon vanadium-doping to form LiFe$_{0.955}$V$_{0.045}$, the transverse incommensurate spin excitations in LiFeAs transform into longitudinally elongated in a similar fashion as that of potassium (hole) doped Ba$_{0.7}$K$_{0.3}$Fe$_2$As$_2$, but with dramatically enhanced magnetic scattering and elimination of superconductivity. This is different from the suppression of the overall magnetic excitations in hole doped BaFe$_2$As$_2$ and the enhancement of superconductivity near optimal hole doping. These results are consistent with density function theory plus dynamic mean field theory calculations, suggesting that vanadium-doping in LiFeAs may induce an enlarged effective magnetic moment $S_{eff}$ with a spin crossover ground state arising from the inter-orbital scattering of itinerant electrons.
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We present a detailed study of 75As NMR Knight shift and spin-lattice relaxation rate in the normal state of stoichiometric polycrystalline LiFeAs. Our analysis of the Korringa relation suggests that LiFeAs exhibits strong antiferromagnetic fluctuations, if transferred hyperfine coupling is a dominant interaction between 75As nuclei and Fe electronic spins, whereas for an on-site hyperfine coupling scenario, these are weaker, but still present to account for our experimental observations. Density-functional calculations of electric field gradient correctly reproduce the experimental values for both 75As and 7Li sites.
We present an inelastic neutron scattering study on single-crystalline LiFeAs devoted to the characterization of the incommensurate antiferromagnetic fluctuations at $mathbf{Q}=(0.5pmdelta, 0.5mpdelta, q_l)$. Time-of-flight measurements show the presence of these magnetic fluctuations up to an energy transfer of 60 meV, while polarized neutrons in combination with longitudinal polarization analysis on a triple-axis spectrometer prove the pure magnetic origin of this signal. The normalization of the magnetic scattering to an absolute scale yields that magnetic fluctuations in LiFeAs are by a factor eight weaker than the resonance signal in nearly optimally Co-doped BaFe$_2$As$_2$, although a factor two is recovered due to the split peaks owing to the incommensurability. The longitudinal polarization analysis indicates weak spin space anisotropy with slightly stronger out-of-plane component between 6 and 12 meV. Furthermore, our data suggest a fine structure of the magnetic signal most likely arising from superposing nesting vectors.
The longitudinal in-plane magnetoresistance (LMR) has been measured in different Ba(Fe_(1-x)Co_x)2As2 single crystals and in LiFeAs. For all these compounds, we find a negative LMR in the paramagnetic phase whose magnitude increases as H^2. We show that this negative LMR can be readily explained in terms of suppression of the spin fluctuations by the magnetic field. In the Co-doped samples, the absolute value of the LMR coefficient is found to decrease with doping content in the paramagnetic phase. The analysis of its T dependence in an itinerant nearly antiferromagnetic Fermi liquid model evidences that the LMR displays a qualitative change of T variation with increasing Co content. The latter occurs at optimal doping for which the antiferromagnetic ground state is suppressed. The same type of analysis for the negative LMR measured in LiFeAs suggests that this compound is on the verge of magnetism.
BaMn2As2 is a local-moment antiferromagnetic insulator with a Neel temperature of 625 K and a large ordered moment of 3.9 Bohr magneton per Mn. Remarkably, this compound can be driven metallic by the substitution of as little as 1.6% K for Ba while retaining essentially the same ordered magnetic moment and Neel temperature, as previously reported. Here, using both powder and single crystal neutron diffraction we show that the local moment antiferromagnetic order in Ba(1-x)KxMn2As2 remains robust up to x = 0.4. The ordered moment is nearly independent of x for 0 < x < 0.4 and the Neel transition temperature decreases to 480 K at x = 0.4.
We report 75As-NMR/NQR results on new iron-arsenide compounds (La0.5-xNa0.5+x)Fe2As2. The parent compound x=0 exhibits a stripe-type antiferromagnetic (AFM) order below T_N=130 K. The measurement of nuclear spin relaxation rate at hole-doped x=+0.3 and heavily electron-doped x=-0.5 revealed that the normal-state properties are dominated by AFM spin fluctuations (AFMSFs), which are more significant at x=+0.3 than at x=-0.5. Their superconducting (SC) phases are characterized by unconventional multi-gap SC state, where the smaller SC gaps are particularly weaken in common. The experimental results indicate the close relationship between the AFMSFs and the SC from the hole-doped state to heavily electron-doped state, which shed light on a unique SC phase emerged in the heavily electron-doped regime being formally equivalent to non-SC compound Ba(Fe0.5Co0.5)Fe2As2.
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