No Arabic abstract
Spectrally intrinsically uncorrelated biphoton states generated from nonlinear crystals are very important but rare resources for quantum photonics and quantum information applications. Previously, such biphoton states were generated from several kinds of crystals, however, their wavelength ranges and nonlinear efficiencies were still limited for various applications. In order to explore new crystal for wider wavelength range and higher nonlinear efficiency, here we theoretically study the generation of spectrally uncorrelated biphoton states from 14 crystals in the `BBO family, including BBO, CLBO, KABO, KBBF, RBBF, CBBF, BABF, BiBO, LBO, CBO, LRB4, LCB, YCOB, and GdCOB. They satisfy three kinds of group-velocity matching condition from near-infrared to telecom wavelengths. Furthermore, heralded single photons can be generated with a purity as high as 0.98, which is achieved without any narrow filtering. The indistinguishability of photons from independent sources is examined by the Hong-Ou-Mandel interference, which results in a visibility of 98% also without any further filtering, i.e., photons from different heralded single-photon sources are highly indistinguishable. Our study may provide single-photon sources with good performance for quantum information processing at near-infrared and telecom wavelengths.
We theoretically investigate the preparation of mid-infrared (MIR) spectrally-uncorrelated biphotons from a spontaneous parametric down-conversion process using doped LN crystals, including MgO doped LN, ZnO doped LN, and In2O3 doped ZnLN with doping ratio from 0 to 7 mol%. The tilt angle of the phase-matching function and the corresponding poling period are calculated under type-II, type-I, and type-0 phase-matching conditions. We also calculate the thermal properties of the doped LN crystals and their performance in Hong-Ou-Mandel interference. It is found that the doping ratio has a substantial impact on the group-velocity-matching (GVM) wavelengths. Especially, the GVM2 wavelength of co-doped InZnLN crystal has a tunable range of 678.7 nm, which is much broader than the tunable range of less than 100 nm achieved by the conventional method of adjusting the temperature. It can be concluded that the doping ratio can be utilized as a degree of freedom to manipulate the biphoton state. The spectrally uncorrelated biphotons can be used to prepare pure single-photon source and entangled photon source, which may have promising applications for quantum-enhanced sensing, imaging, and communications at the MIR range.
We theoretically investigated spectrally uncorrelated biphotons generated in a counter-propagating spontaneous parametric downconversion (CP-SPDC) from periodically poled MTiOXO4 (M = K, Rb, Cs; X = P, As) crystals. By numerical calculation, it was found that the five crystals from the KTP family can be used to generate heralded single photons with high spectral purity and wide tunability. Under the type-0 phase-matching condition, the purity at 1550 nm was between 0.91 and 0.92, and the purity can be maintained over 0.90 from 1500 nm to 2000 nm wavelength. Under the type-II phase-matching condition, the purity at 1550 nm was 0.96, 0.97, 0.97, 0.98, and 0.98 for PPKTP, PPRTP, PPKTA, PPRTA, and PPCTA, respectively; furthermore, the purity can be kept over 0.96 for more than 600 nm wavelength range. We also simulated the Hong-Ou-Mandel interference between independent photon sources for PPRTP crystals at 1550 nm, and interference visibility was 92% (97%) under type-0 (type-II) phase-matching condition. This study may provide spectrally pure narrowband single-photon sources for quantum memories and quantum networks at telecom wavelengths.
We consider a double Gaussian approximation to describe the wavefunction of twin photons (also called a biphoton) created in a nonlinear crystal via a type-I spontaneous parametric downconversion (SPDC) process. We find that the wavefunction develops a Gouy phase while it propagates, being dependent of the two-photon correlation through the Rayleigh length. We evaluate the covariance matrix and show that the logarithmic negativity, useful in quantifying entanglement in Gaussian states, although Rayleigh-dependent, does not depend on the propagation distance. In addition, we show that the two-photon entanglement can be connected to the biphoton Gouy phase as these quantities are Rayleigh-length-related. Then, we focus the double Gaussian biphoton wavefunction using a thin lens and calculate a Gouy phase that is in reasonable agreement with the experimental data of D. Kawase et al. published in Ref. [1].
We report the experimental verification of nonclassical correlations for a four-wave-mixing process in an ensemble of cold two-level atoms, confirming theoretical predictions by Du et al. in 2007 for the violation of a Cauchy-Schwarz inequality in the system, and obtaining $R = (1.98pm0.03) leq 1$. Quantum correlations are observed in a nano-seconds timescale, in the interference between the central exciting frequency and sidebands dislocated by the detuning to the atomic resonance. They prevail without filters over the noise background coming from linear scattering from the same optical transition. These correlations are fragile with respect to processes that disturb the phase of the atomic excitation, but are robust to variations in number of atoms and to increasing light intensities.
We present results of a bright polarization-entangled photon source operating at 1552 nm via type-II collinear degenerate spontaneous parametric down-conversion in a periodically poled potassium titanyl phosphate crystal. We report a conservative inferred pair generation rate of 123,000 pairs/s/mW into collection modes. Minimization of spectral and spatial entanglement was achieved by group velocity matching the pump, signal and idler modes and through properly focusing the pump beam. By utilizing a pair of calcite beam displacers, we are able to overlap photons from adjacent down-conversion processes to obtain polarization-entanglement visibility of 94.7 +/- 1.1% with accidentals subtracted.